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Advances in quantum chemistry

Coherence Effects in Laser-Induced Continuum Structure

Ioannis Thanopulos, Moshe Shapiro

Published Jan 1, 2010• 2 citations
Publisher
DOI
10.1016/s0065-3276(10)60003-2

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Laser induced continuum structures (LICS) can be produced by a strong laser embedding an excited atomic bound state into a flat atomic continuum, leading to a tunable resonance of adjustable width that can be probed by a second laser. If this second laser is of similar intensity to the embedding laser then the distinction between the two becomes artificial and saturation effects become important. In this paper the effect on LICS of transitions caused by both lasers between the original atomic continuum and a second atomic continuum are studied in the Markoff approximation by means of Laplace transform methods and allowing for the ionization of each atomic state by both laser fields. Formal results correct to all orders are also given in terms of a T-matrix approach. Numerical calculations are presented showing the effects on the LICS resonant structures of continuum-continuum coupling processes. Significant changes to the Fano profiles (second laser weak) and to coherence holes (second laser strong) occur. Analytical results are also given.
We present results from a study of the coherence properties of a system involving three discrete states coupled to each other by two-photon processes via a common continuum. This tripod linkage is an extension of the standard laser-induced continuum structure (LICS), which involves two discrete states and two lasers. We show that in the tripod scheme, there exist two population trapping conditions; in some cases these conditions are easier to satisfy than the single trapping condition in a two-state LICS. Depending on the pulse timing, various effects can be observed. We derive some basic properties of the tripod scheme, such as the solution for coincident pulses, the behavior of the system in the adiabatic limit for delayed pulses, the conditions for no ionization and for maximal ionization, and the optimal conditions for population transfer between the discrete states via the continuum. In the case when one of the discrete states is strongly coupled to the continuum, the population dynamics reduces to a standard two-state LICS problem (involving the other two states) with modified parameters; this provides the opportunity to customize the parameters of a given two-state LICS system.