This thesis introduces the linear and nonlinear properties of photonic crystal fibre (PCF), describes the fabrication and characterisation of different PCFs, and demonstrates their applications to supercontinuum (SC) generation and single-photon sources. The linear properties of PCF include endlessly single-mode transmission, highly controllable dispersion and birefringence. These unique properties have made PCFs the best media to demonstrate all kinds of nonlinear effects such as self-phase modulation (SPM), cross-phase modulation (XPM), Raman effects, four-wave mixing and modulation instability (FWM and MI), and soliton effects. The combination of these nonlinear effects has led to impressive spectral broadening known as SC generation in PCFs. The intrinsic correlation of signal and idler photons from FWM has brought PCF to the application of single-photon generation. Four projects about SC generation were demonstrated. The first was visible continuum generation in a monolithic PCF device, which gave a compact, bright (-20 dBm/nm), flat and single-mode visible continuum source extending to short wavelength at 400 nm. The second was polarised SC generation in a highly bire-fringent PCF. A well linearly polarised continuum source spanning 450-1750 nm was achieved with >99% power kept in a single linear polarisation. This polarised continuum source was then applied to tuneable visible/UV generation in a BIBO crystal. The third was residual pump peak removal for SC generation in PCFs. The fourth was to design an all-fibre dual-wavelength pumping for spectrally localised continuum generation. Two projects about photon pair generation using FWM were then demonstrated. One was an all-fibre photon pair source designed in the telecom band for quantum communication. This source achieved >50% heralding efficiency which is the highest in fibre photon pair sources reported so far. Another one was to design birefringent PCFs for naturally narrow band photon pair generation in the Si SPAD high detection efficiency range. 0.122 nm bandwidth signal photons at 596.8 nm were generated through cross polarisation phase matched FWM in a weakly birefringent PCF pumped by a picosecond Ti:Sapphire laser at 705 nm in the normal dispersion regime.
This thesis introduces the linear and nonlinear properties of photonic crystal fibre (PCF), describes the fabrication and characterisation of different PCFs, and demonstrates their applications to supercontinuum (SC) generation and single-photon sources. The linear properties of PCF include endlessly single-mode transmission, highly controllable dispersion and birefringence. These unique properties have made PCFs the best media to demonstrate all kinds of nonlinear effects such as self-phase modulation (SPM), cross-phase modulation (XPM), Raman effects, four-wave mixing and modulation instability (FWM and MI), and soliton effects. The combination of these nonlinear effects has led to impressive spectral broadening known as SC generation in PCFs. The intrinsic correlation of signal and idler photons from FWM has brought PCF to the application of single-photon generation. Four projects about SC generation were demonstrated. The first was visible continuum generation in a monolithic PCF device, which gave a compact, bright (-20 dBm/nm), flat and single-mode visible continuum source extending to short wavelength at 400 nm. The second was polarised SC generation in a highly bire-fringent PCF. A well linearly polarised continuum source spanning 450-1750 nm was achieved with >99% power kept in a single linear polarisation. This polarised continuum source was then applied to tuneable visible/UV generation in a BIBO crystal. The third was residual pump peak removal for SC generation in PCFs. The fourth was to design an all-fibre dual-wavelength pumping for spectrally localised continuum generation. Two projects about photon pair generation using FWM were then demonstrated. One was an all-fibre photon pair source designed in the telecom band for quantum communication. This source achieved >50% heralding efficiency which is the highest in fibre photon pair sources reported so far. Another one was to design birefringent PCFs for naturally narrow band photon pair generation in the Si SPAD high detection efficiency range. 0.122 nm bandwidth signal photons at 596.8 nm were generated through cross polarisation phase matched FWM in a weakly birefringent PCF pumped by a picosecond Ti:Sapphire laser at 705 nm in the normal dispersion regime.
The preparation of single photons in a pure quantum state is a subject of great interest in physics, enabling the control of light at an unprecedented level. The ease with which certain degrees of freedom of photon states, such as polarisation, can be manipulated, along with the inherent resilience of photons to decoherence, makes them well suited for use as qubits. Recent rapid developments in the transmission and processing of quantum information, as well as the likely technological impact of potential real-world applications such as quantum cryptography and quantum computation, mean that the demand for high performance single photon sources is likely to increase in the near future. One approach to producing single photon states, which are known to be in a well-defined spatio-temporal mode without destructively measuring them, is to take advantage of nonlinear optics. Nonlinear processes can be used to realise frequency conversion by generating a single, correlated pair of photons from an intense pump laser source. The detection of one of the photons from a pair can then be used to indicate the presence of the other photon in the pair, a procedure known as heralding. This thesis describes the development of a source of heralded single photons at 1550 nm, generated directly in the core of a photonic crystal fibre (PCF). By taking advantage of low loss fibre components for the required spectral filtering of the generated photon state, a heralding fidelity of 52% was achieved. The source was designed to be used with a picosecond pulsed fibre laser, making it relatively low cost and maintenance free. With 148 mW of average pump power a heralded output photon rate of 6.4 × 104 s-1 was observed, demonstrating the brightness of the source. The purity of the generated single photons was established by measuring non-classical interference, with a visibility of 70%, between the photons output from this source and a source based on a PPLN waveguide. The fabrication of a series of birefringent PCFs for the generation of spectrally pure state photons at 1550 nm is also discussed. These PCFs will be useful for incorporation in the next generation of high performance, fibre-based photon sources.
The paper reviews a new source of time-correlated photon pairs based on phase matched four-wave mixing in an optical fiber. This source has the potential to replace sources based on a non-linear birefringent crystals and waveguides. It generates linear polarised photon pairs in a narrow bandwidth, single circular mode which can be efficiently coupled into single mode fibres. We generate the parametric gain by pumping with a laser wavelength slightly below the zero dispersion wavelength, in the normal dispersion regime.
Pure state single photons are at the heart of optical quantum technologies. We have previously reported the generation of photon pairs by four-wave mixing in a single-mode photonic crystal fibre (PCF) and the use of a new birefringent phase matching scheme which results in the generation of narrowband signal photons, around 0.2 nm in bandwidth, and a factorizable photon pair state with no requirement for spectral filtering, leading to increased count rates. Our source is bright, polarized, and tuneable by variable laser wavelength and fibre parameters. Hong-Ou-Mandel (HOM) interference is observed between photons from two of these sources, a requirement for optical quantum information tasks.
The interplay between chromatic dispersion and nonlinear effects is patent. Once a photonic crystal fiber (PCF) preform has been prepared, changing the parameters that control the fabrication process it is possible to adjust the dispersion properties of the fiber. In addition, it is very useful to develop postprocessing techniques that enable a fine adjustment of the dispersion along a section of PCF. The tapering of PCF, using a fusion and pulling technique, has been established as a rather useful technique to engineer the dispersion properties along tens of centimeters. Some of our recent experiments demonstrate that the use of erbium doped PCF enables an optical control of the dispersion through optical pumping of the rare earth ions. Our interest is focused on the exploitation of nonlinear PCF for the development of fiber light sources. Thus, we will present several experiments on supercontinuum and photon pairs generation, through degenerated four-wave mixing (FWM), in order to illustrate the control that one can achieve on the optical spectra of these light sources as a function of different dispersion control approaches.
Summary form only given. Generation of correlated photon pairs by spontaneous parametric four-wave mixing (FWM) in photonic crystal fibres (PCF) opens the way for many applications, particularly for fibre-based quantum communication devices. In degenerate FWM, two pump photons at frequency ωρare annihilated to produce simultaneously a signal photon at ωsand an idler photon at ωi, such as ωs+ ωi= 2ωp(energy conservation). This process occurs with high efficiency only if the phase-matching condition (i.e. momentum conservation) is satisfied [1].The group-velocity dispersion (GVD) of the silica-core PCF used in our experiments (fig.1.a, inset) has been experimentally determined by a time-of-flight measurement for wavelengths from 740 nm to 930 nm. The result is consistent with the analytical calculation provided by Saitoh and Koshiba [2]. Particularly, we estimate the zero-dispersion wavelength of the PCF: λZDW = 834 nm. From this GVD measurement, we deduce the phasematching curve given in fig.1.a, on which we note that there is a vertical asymptote at λp - 832 nm. Thus, FWM should not be observed if the pump wavelength λp is lower than this limit value. Our experimental observations are very different from this prediction. Indeed, by injecting inside the fundamental mode of a 1.3-m-long PCF hyperbolic secant picosecond pulses (with an intensity-FWHM duration of about 2 ps) at λinj = 815 nm with a 80-MHz repetition rate, we actually observe a spontaneous parametric FWM phenomenon (with sidebands generated around 925 nm and 745 nm), and moreover with a clear frequency dissymmetry with respect to the injected pulse frequency (ωinj = 2ππc/λinj) (fig.1.b): generated signal and idler frequencies ωs and ωi do not satisfy ωs + ωi = 2ωinj.A systematic study of this frequency-dissymmetric phenomenon shows that it occurs only when the injected pulse peak power (Pinj) is higher than a threshold value Pth, and that Pth increases when λinj decreases from λZDW. This variation of Pth as a function of λinj can be understood by considering the key role played by self-phase modulation (SPM) in the observed phenomenon. Indeed, the frequency-dissymmetric signal and idler waves are generated only when the spectral broadening (due to SPM) of the injected pulses is sufficient to reach a threshold wavelength λth (i.e. a threshold frequency ωth) of the order of 832 nm. This value corresponds to the position of the vertical asymptote in the phase-matching curve. Finally, we observe that ωs + ωi - 2ωth when Pinj Pth. All these observations highlight the fact that, when the injected pulse peak power Pinj is high enough, spectral broadening by SPM is sufficient to get a part of the injected pulse spectrum higher than the threshold value λth, and thus this part of the spectrum can play the role of pump in an efficient FWM process (i.e. with the phasematching condition satisfied). It is important to note that this phenomenon advantageously presents an extension of the spectral range on which an efficient FWM process can occur: instead of being restricted to injected pulse wavelengths higher than the zero-dispersion wavelength λZDW of the fibre (or at least, higher than a threshold wavelength λth of the order of λZDW), experimenters can work with lower wavelengths, providing the availability of a high enough peak power and/or interaction length to sufficiently broaden (by SPM) the injected pulse spectrum.
In this paper, we study the tailoring of photon spectral properties generated by four-wave mixing in a birefringent photonic crystal fibre (PCF). The aim is to produce intrinsically narrow-band photons and hence to achieve high non-classical interference visibility and generate high-fidelity entanglement without any requirement for spectral filtering, leading to high effective detection efficiencies. We show unfiltered Hong–Ou–Mandel interference visibilities of 77% between photons from the same PCF and 80% between separate sources. We compare results from modelling the PCF to these experiments and analyse photon purities.