High-order adiabatic representations of quantum systems through a perturbative construction of dynamical invariants
T. T. Nguyen‐Dang, Evgueni Sinelnikov, Arne Keller +1 more
A perturbative series is derived for the systematic construction of a dynamical invariant (Lewis invariant) for a time-dependent Hamiltonian which is characterized by a time-scale parameter $\ensuremath{\tau}$, as appears in the usual formulation of the adiabatic theorem. The derivations make efficient use of the quantum averaging method, and the perturbative series obtained permits the construction of the invariant in successive orders in $ϵ\ensuremath{\sim}1/\ensuremath{\tau}$, corresponding to high-order adiabatic approximations. The series can be considered and resummed analytically to all orders, yielding an exact invariant for an harmonic oscillator linearly driven by an external field. For a nondegenerate two-level system, approximate invariants have been obtained up to the fifth order and illustrate how the adiabatic approximations of increasing orders successively approach the exact dynamics. The construct is applicable also to Floquet Hamiltonians and, in this context, it furnishes high-order adiabatic representations for the time evolution of Floquet states associated with a material system in an aperiodic laser pulse. We illustrate in particular how an exact Floquet dynamical invariant, defining exact adiabatic transports of Floquet states, is obtained for a laser-driven harmonic vibrational mode.
Physical Review A•Nov 30, 2007•8 citations