Our demonstration of multiple-photon resonant cycling between the 1/sup 3/S and 2/sup 3/P states of ortho-Positronium (oPs) makes possible the production of cold positronium (Ps) through the technique of laser cooling. A simplified analysis of magnetic mixing in excited-state Ps is given. This effect is important both as a diagnostic of resonant cycling and Ps cooling. The significance of cold Ps in fine structure measurements and the formation of a Bose-Einstein condensate is discussed. 13 refs., 3 figs.
Our demonstration of multiple-photon resonant cycling between the 1/sup 3/S and 2/sup 3/P states of ortho-Positronium (oPs) makes possible the production of cold positronium (Ps) through the technique of laser cooling. A simplified analysis of magnetic mixing in excited-state Ps is given. This effect is important both as a diagnostic of resonant cycling and Ps cooling. The significance of cold Ps in fine structure measurements and the formation of a Bose-Einstein condensate is discussed. 13 refs., 3 figs.
Zeeman mixing of singlet and triplet 2P states of positronium (Ps) atoms, followed by decay back to the ground state, can effectively turn a long-lived triplet atom into a short-lived singlet state, which would seem to preclude laser cooling of Ps in a magnetic field. Here we report experiments which show that, in fact, because of the large splitting of the n=2 states in a high magnetic field (the Paschen-Back regime), the amount of such mixing diminishes approximately exponentially with an increasing magnetic field >0.01 T and is essentially eliminated above ∼2 T. Thus, laser cooling of Ps should be feasible at high fields, which will facilitate the production of a Ps Bose-Einstein condensate.
A new method to realize Bose-Einstein condensation (BEC) of positronium (Ps) is proposed and a Monte-Carlo simulation was performed to evaluate the cooling efficiency of Ps atoms. Ps-BEC was found to be possible by a method including laser cooling of Ps. Laser specifications for Ps cooling are challenging and development is ongoing. A new temperature measurement method for cold Ps and development of an intense, pulsed, slow-positron microbeam are also necessary. They are under study as outlined in this contribution.
On the basis of three dimensional (3-D) Monte Carlo simulation, we studied details of laser cooling (Doppler cooling) of ortho-Positronium ( o -Ps) which would be applied to the achievement of Bose–Einstein condensation of positronium. The cooling is carried out by an ultraviolet laser with a wavelength of 243 nm being equivalent to the 1 S –2 P transition energy of o -Ps. For this purpose, we have constructed a laser cooling apparatus which consists of a slow positron generator and a long pulse, wide linewidth laser. A 3-D Monte Carlo calculation, which incorporated various parameters of laser beam and positronium distributions expected in the current laser cooling apparatus, revealed that 7% of o -Ps was able to be cool down to 1 K and to be confined in a relatively small volume without employing a special trap.
Abstract A proposed new method of cooling positronium is to realize the Bose–Einstein condensation (BEC) of positronium. We perform detailed studies of three processes: (1) thermalization processes between positronium and the silica walls of a cavity, (2) Ps–Ps scattering and (3) laser cooling. The thermalization process is shown to be not sufficient for BEC. Ps–Ps collision is shown to have a big effect on the cooling performance. We combine both methods and establish an efficient cooling process for BEC. We also propose a new optical laser system for the cooling.
Methods and techniques in the production, manipulation, and accumulation of positrons in a `Surko-type' buffer-gas trap are presented. The pulsed output of the trap is optimised for laser excitation of positronium (Ps). The techniques of positron time compression and single-shot positron annihilation lifetime spectroscopy (SSPALS) are discussed in detail and used throughout the study. A small array or Ps converter materials have been characterised at various temperatures. Ps cooling as a function of positron implantation is presented and discussed. Direct laser irradiation of the samples, and the effect on the Ps yield has also been studied. In some cases, particularly at cryogenic temperatures, laser induced paramagnetic centres are formed and this has a detrimental effect on the Ps yield as they cause triplet Ps to convert to the shorter-lived singlet state. Whereas in single crystal semiconductors, the laser has an enhancing effect due to an exciton-like positron-electron surface state. Many of the Ps converter materials studied here are formed from porous structures. The long term confinement of Ps within isolated cavities has also been observed, where a lifetime measurement technique using an excitation laser is presented. General methods of Ps-laser spectroscopy are also presented and the applications of which are discussed including laser-enhanced time-of-flight spectroscopy (LEPTOF), and the production, and electrostatic guiding of highly excited Rydberg Ps. Using these techniques a crossed beam scattering experiment involving Rydberg Ps, electrons, and Argon ions was carried out. This work presents important considerations for experiments to create a laser-cooled Bose-Einstein condensate (BEC) of Ps in an engineered porous material at cryogenic temperatures.
Realization of Bose-Einstein Condensate (BEC) of positronium (Ps), a purely leptonic particle-antiparticle bound system, is a challenging subject [1, 2]. Recently, Ivanov et al. [3] theoretically investigated the Ps-Ps scattering and showed theoretically that the scattering length for the o-Ps atoms is positive, indicating that a stable o-Ps BEC is actually possible. The condition for the BEC of the ideal Bose gas is λth > (2.612/n)1/3, where λth = h/ √ 2πmkT is the thermal de Broglie wavelength of the atom and n is the number density. This gives the critical temperature for the Ps BEC as Tc = 1.46×10−15n2/3, where Tc is in K and n is in m−3. This condition is much less severe than for the usual alkali atom BEC because λth is longer by five orders of magnitude. However, Ps has a finite lifetime: the lifetime of singlet state, para-positronium (p-Ps), is 125 ps and that of triplet state, ortho-positronium (o-Ps), is 142 ns. Thus a many-Ps system must be cooled within the lifetime of o-Ps. The short lifetime of Ps demands quick cooling and high density. The laser cooling which is employed for the accomplishment of alkali atom BEC is likely to be impractical because it takes longer time. It is also subject to relatively large recoil of the Ps atom when hit by a photon. Moreover, unless an effective method for trapping Ps in free space is developed, the system of Ps atoms diffuses and lowers its density. Platzmann and Mills [1] suggested to confine Ps in a small cavity of insulating material and let the Ps atoms give away their kinetic energy to the walls of the cavity. If one injects an intense polarized positron beam onto a material which has a micro cavity near surface, some of the positrons form Ps and are emitted into the cavity and stay there. This is expected because the work function of most of the material for Ps is negative, i.e., Ps atoms emitted into the cavity after thermalization in the material will never penetrate back into the material. They just hit the cavity walls and approach thermal equilibrium by exciting phonons. The probability of the annihilation of o-Ps with a surface electron is small if there are no paramagnetic centers on the cavity walls. It is necessary to use a polarized positron beam to make Ps. Otherwise all the o-Ps atoms are lost through mutual spin conversion into p-Ps [1, 4]. In this report we would like to discuss prospect of a Ps BEC with special attention to the following aspects [4]: (1) use of 18F for a source of an intense spin-polarized positron beams [5], (2) development of high efficiency Wmesh positron moderator, (3) emission of Ps from solid surface (4) the cooling of Ps in a cavity, and (5) the detection of a Ps BEC.