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Optics and Spectroscopy

Two-photon absorption controlled by the resonance optical Stark effect in crystals and quantum nanostructures

E. Yu. Perlin, Федоров Анатолий Валентинович

Published Mar 1, 1995• 4 citations
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Related papers

Nonlinear switching mechanism in nanostructures doped in photonic crystals

Mahi R. Singh

We have investigated the nonlinear switching mechanism in nanostructures doped in photonic crystals. The nonlinear phenomenon studied in this paper is the two-photon absorption process. A probe laser field is applied between the ground state and the next excited state of the nanoparticles to measure the two-photon absorption spectrum. A coupling field is applied between the two excited states of nanoparticles to control the two-photon process. It is found that when the decay resonance energy lies away from the photonic band edge the inhibition of two-photon absorption is observed. However, when the probe field is not resonance, the inhibition of two photons absorption is not observed. An interesting result is observed when the decay resonance energy lies near the band edge. It is found that the inhibition of the two-photon absorption disappears. It means that the phenomenon of two-photon absorption can be switched on and off by tuning the resonance energy within the lower band of the crystal. This mechanism can be used to make a new type of photonic switching devices using photonic crystals.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jun 21, 2007•0 citations

Two-photon absorption in atoms and solids

A. Quattropani, B. Girlanda

Rivista Del Nuovo Cimento•Sep 1, 1983•23 citations

Optical Stark effect in double-resonance conditions in semiconductor nanostructures

E. Yu. Perlin, Федоров Анатолий Валентинович

The theory of the optical Stark effect is developed for quantum-size structures. The effect is due to the interaction of the electron system with intense light, whose frequency, (omega) , is in resonance between two subbands in the conduction band. The probe light of the frequency (Omega) falls in resonance with the adjacent transition between the ground state and the state with an electron-hole pair. In the quasi-steady-state mode, the singularities in the interband (Omega) -light absorption spectra are related to the critical points of the bands, rearranged by the (omega) - light. The shape of the higher conduction band can be evaluated from the spectral positions of the singularities. In the case of two-photon interband transitions, a sharp dependence of the absorption on the light intensity is predicted. In the non-steady-state mode, the probe beam consists of two femtosecond (Omega) -light pulses following each other with the delay time, (tau) d. The dependence of energy, absorbed from the second pulse, on the (tau) d value is calculated. Under the (omega) -pumping, one of the two phenomena should be observed, depending on the type of band structure, namely, the decay of the induced polarization with the characteristic time approximately 1/(omega) R or oscillations with the frequency approximately (omega) R, where (omega) R is the Rabi frequency. The principal effect, controlling the decay of the Rabi oscillations, is the spreading of the packet of states generated by the (Omega) -light pulse.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jun 10, 1996•1 citation

Two-photon absorption in atomic or molecular systems

G. Fornaca, Mario Iannuzzi, ERSEO POLACCO

Il Nuovo Cimento•Apr 1, 1965•7 citations

A study of the ac Stark effect in doped photonic crystals

I. Haque, Mahi R. Singh

In this paper we present calculations of level populations and susceptibility for an ensemble of five-level atoms doped in a photonic crystal, using the master equation method. The atoms in the ensemble interact with the crystal which acts as a reservoir and are coupled with two strong pump fields and a weak probe field. It is found that, by manipulating the resonance energy associated with one of the decay channels of the atom, the system can be switched between an inverted and a non-inverted state. We have also observed the ac Stark effect in these atoms and have shown that due to the role played by the band structure of the photonic crystal, it is possible to switch between an absorption state and a non-absorption state of the atomic system. This is a very important finding as techniques of rendering material systems transparent to resonant laser radiation are very desirable in the fabrication of novel optical and photonic devices.

Journal of Physics Condensed Matter•Mar 27, 2007•29 citations

Theory of coherent two-photon absorption

NILOY KUMAR DUTTA

Physics Letters A•Nov 1, 1978•5 citations
We have investigated the nonlinear switching mechanism in nanostructures doped in photonic crystals. The nonlinear phenomenon studied in this paper is the two-photon absorption process. A probe laser field is applied between the ground state and the next excited state of the nanoparticles to measure the two-photon absorption spectrum. A coupling field is applied between the two excited states of nanoparticles to control the two-photon process. It is found that when the decay resonance energy lies away from the photonic band edge the inhibition of two-photon absorption is observed. However, when the probe field is not resonance, the inhibition of two photons absorption is not observed. An interesting result is observed when the decay resonance energy lies near the band edge. It is found that the inhibition of the two-photon absorption disappears. It means that the phenomenon of two-photon absorption can be switched on and off by tuning the resonance energy within the lower band of the crystal. This mechanism can be used to make a new type of photonic switching devices using photonic crystals.
The theory of the optical Stark effect is developed for quantum-size structures. The effect is due to the interaction of the electron system with intense light, whose frequency, (omega) , is in resonance between two subbands in the conduction band. The probe light of the frequency (Omega) falls in resonance with the adjacent transition between the ground state and the state with an electron-hole pair. In the quasi-steady-state mode, the singularities in the interband (Omega) -light absorption spectra are related to the critical points of the bands, rearranged by the (omega) - light. The shape of the higher conduction band can be evaluated from the spectral positions of the singularities. In the case of two-photon interband transitions, a sharp dependence of the absorption on the light intensity is predicted. In the non-steady-state mode, the probe beam consists of two femtosecond (Omega) -light pulses following each other with the delay time, (tau) d. The dependence of energy, absorbed from the second pulse, on the (tau) d value is calculated. Under the (omega) -pumping, one of the two phenomena should be observed, depending on the type of band structure, namely, the decay of the induced polarization with the characteristic time approximately 1/(omega) R or oscillations with the frequency approximately (omega) R, where (omega) R is the Rabi frequency. The principal effect, controlling the decay of the Rabi oscillations, is the spreading of the packet of states generated by the (Omega) -light pulse.
In this paper we present calculations of level populations and susceptibility for an ensemble of five-level atoms doped in a photonic crystal, using the master equation method. The atoms in the ensemble interact with the crystal which acts as a reservoir and are coupled with two strong pump fields and a weak probe field. It is found that, by manipulating the resonance energy associated with one of the decay channels of the atom, the system can be switched between an inverted and a non-inverted state. We have also observed the ac Stark effect in these atoms and have shown that due to the role played by the band structure of the photonic crystal, it is possible to switch between an absorption state and a non-absorption state of the atomic system. This is a very important finding as techniques of rendering material systems transparent to resonant laser radiation are very desirable in the fabrication of novel optical and photonic devices.