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arXiv:2611.01515

Superradiance fingerprints of moiré exciton-biexciton condensates: path-entangled biphoton vs. supercurrent-enabled one-photon channel

Haochen Wang, Shengxian Li, Hongyu Lu, Mingxing Chen, Wang Yao

cond-mat.mes-hallcond-mat.quant-gasquant-phSubmitted Nov 1, 2026• Announced Nov 3, 2026
arXivHTMLPDF

Abstract

Hybrid moiré excitons form a dense array of electrically tunable single-photon emitters, entailing cooperative optical responses with intriguing consequences. With the strong dipole-dipole interaction, they also realize Bose-Hubbard quantum simulators of emergent correlated matter such as Bose-Einstein condensates (BEC). Here we reveal the characteristic cooperative radiation from condensates of hybrid moiré excitons in twisted MoTe$_2$ bilayers. In each individual moiré trap, the layer hybridization selection rule dictates that the ground-state exciton is a quantum emitter of orbital-angular-momentum photons, with an exceptionally long radiative lifetime. Ground-state emission becomes pronounced only upon forming condensates, where inter-sublattice dipole attraction and intra-sublattice repulsion together lead to the coexistence of exciton and biexciton BEC with comparable weights. The biexciton (molecular-type) BEC decays through superradiance of path-entangled biphotons, whereas the exciton (atomic-type) BEC is dark at rest and becomes superradiant when it carries a supercurrent. Our findings not only uncover a novel source of entangled light but also establish unique fingerprints for exploring the cold chemistry of atomic-molecular condensates with moiré excitons.

Comments
4 pages, 4 figures

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Hybrid moiré excitons form a dense array of electrically tunable single-photon emitters, entailing cooperative optical responses with intriguing consequences. With the strong dipole-dipole interaction, they also realize Bose-Hubbard quantum simulators of emergent correlated matter such as Bose-Einstein condensates (BEC). Here we reveal the characteristic cooperative radiation from condensates of hybrid moiré excitons in twisted MoTe2_22​ bilayers. In each individual moiré trap, the layer hybridization selection rule dictates that the ground-state exciton is a quantum emitter of orbital-angular-momentum photons, with an exceptionally long radiative lifetime. Ground-state emission becomes pronounced only upon forming condensates, where inter-sublattice dipole attraction and intra-sublattice repulsion together lead to the coexistence of exciton and biexciton BEC with comparable weights. The biexciton (molecular-type) BEC decays through superradiance of path-entangled biphotons, whereas the exciton (atomic-type) BEC is dark at rest and becomes superradiant when it carries a supercurrent. Our findings not only uncover a novel source of entangled light but also establish unique fingerprints for exploring the cold chemistry of atomic-molecular condensates with moiré excitons.
The unique properties of two-dimensional moiré systems have been widely studied from many perspectives. However, relatively little work has investigated how the real-space structure of moiré systems can directly engender novel properties and functionalities. In this Letter, we explore how intriguing cooperative optical effects can emerge from the real-space superlattice formed by moiré excitons. Particularly, we show that the collective moiré exciton states can have either strongly enhanced (superradiant) or suppressed (subradiant) radiative decay rates, depending on their in-plane wave vector. These super- and subradiant states can be efficiently switched by a gate-induced electric field gradient. Moreover, the cooperative transmittance T of the atomically thin moiré system can be switched from T≈0T\approx 0T≈0 (opaque) to T≈1T \approx 1T≈1 (transparent) with ≲ 1%\lesssim ~1\%≲ 1% heterostrain or a 1∘1^{\circ}1∘ adjustment in the twist angle θθθ. These features are robust against nonradiative losses and disorders, making the moiré system a highly versatile platform for cooperative quantum optics with potential applications in, e.g., single photon storage and switching.
Moiré related physics in twisted bilayer two-dimensional (2D) materials has attracted widespread interest in condensed matter physics. Simulation of moiré related physics in cold atom platform is expected to outperform the 2D materials thanks to its advantage of higher tunablility. Here, we demonstrate that, the cold atom platform enables a new mechanism of moiré lattice formation, induced by interlayer interaction with intrinsic "dynamical" character, in contrast to conventional moiré lattice induced by "static" ways such as single-particle interlayer tunneling. Specifically, we consider a twisted bilayer Bose-Hubbard model with vanishing interlayer tunneling, and the bilayer is solely coupled through interlayer interaction that originates from contact interaction of atoms. We find that this system hosts a plethora of novel phases unique to this dynamical lattice, including a variety of Mott insulator (MI) and superfluid (SF) phases either preserving or breaking moiré lattice symmetry, phases with one layer in SF and the other in MI, "interlocked" MI, and self-localized phases at commensurate twist angles, which exhibits the characteristics of Bose glass and quasi-many-body localization in the absence of (quasi)disorder or quasicrystalline lattices. Our prediction can be readily observed in current experimental setup of twisted bilayer optical lattices, opening up new avenues for exploring the rich physics of interaction induced moiré systems in cold atoms.
Recently, the simulation of moiré physics using cold atom platforms has gained significant attention. These platforms provide an opportunity to explore novel aspects of moiré physics that go beyond the limits of traditional condensed matter systems. Building on recent experimental advancements in creating twisted bilayer spin-dependent optical lattices for pseudospin-1/2 Bose gases, we extend this concept to a trilayer optical lattice for spin-1 Bose gases. Unlike conventional moiré patterns, which are typically induced by interlayer tunneling or interspin coupling, the moiré pattern in this trilayer system arises from inter-species atomic interactions. We investigate the ground state of Bose-Einstein condensates loaded in this spin-1 twisted optical lattice under both ferromagnetic and antiferromagnetic interactions. We find that the ground state forms a periodic pattern of distinct phases in the homogeneous case, including ferromagnetic, antiferromagnetic, polar, and broken axial symmetry phases. Additionally, by quenching the optical lattice potential strength, we examine the quench dynamics of the system above the ground state and observe the emergence of topological excitations such as vortex pairs. This study provides a pathway for exploring the rich physics of spin-1 twisted optical lattices and expands our understanding of moiré systems in synthetic quantum platforms.
Moiré excitons promise a new platform with which to generate and manipulate hybrid quantum phases of light and matter in unprecedented regimes of interaction strength. We explore the properties in this regime, through studies of a Bose-Hubbard model of excitons coupled to cavity photons. We show that the steady states exhibit a rich phase diagram with pronounced bistabilities governed by multiphoton resonances reflecting the strong interexciton interactions. In the presence of an incoherent pumping of excitons we find that the system can realize single- and multiphoton lasers.
Introduction. Polaritons and Semiconductor Microcavities As we have mentioned previously, BEC of excitons or biexcitons and lasing can be seen as two limits of the same theory. Lasing occurs in the case of strong electron-photon coupling (recombination rate fast compared with interparticle-scattering rate) while excitonic BEC occurs in the case of weak electron-photon coupling (recombination rate slow compared with the interparticle-scattering rate.) A laser can be seen as a Bose condensate in which the long-range phase coherence exists in the photon states [1], while in the exciton condensate the coherence exists in the electronic states. This is one of the reasons for some of the confusing debates in the early history of excitonic Bose condensation – in many systems there is not a sharp distinction between an excitonic condensate and supperradiance, i.e., luminescence with enhanced intensity due to stimulated emission [2-4]. In the previous chapters, we have so far considered a laser light source only as a source of excitons by means of quantum transitions. In Chapter 6, the laser radiation was taken into account as a given external factor. This chapter is dedicated to phenomena related to a strong and noticeable exciton-photon interaction, when the light significantly influences the energy spectrum of the high-density excitons [5-9]. As we will see, this leads to many fascinating effects related to instabilities. A strong exciton-photon interaction implies a strong polariton effect, in which photon and exciton states are mixed (as in Fig. 1.3). When this mixing is strong, it is not obvious how to define the ground state of the system.
Abstract Observation of strong correlations and superconductivity in twisted-bilayer-graphene have stimulated tremendous interest in fundamental and applied physics. In this system, the superposition of two twisted honeycomb lattices, generating a Moire pattern, is the key to the observed flat electronic bands, slow electron velocity and large density of states. Despite these observations, a full understanding of the emerging superconductivity from the coupled layers and the appearance of a small magic angle remain a hot topic of research. Here, we demonstrate a quantum simulation platform to study superfluids in twisted bilayer lattices based on Bose-Einstein condensates loaded into spin-dependent optical lattices. The lattices are made of two sets of laser beams that independently address atoms in different spin states, which form the synthetic dimension accommodating the two layers. The twisted angle of the two lattices is controlled by the relative angle of the laser beams. We show that atoms in each spin state only feel one set of the lattice and the interlayer coupling can be controlled by microwave coupling between the spin states. Our system allows for flexible control of both the inter- and intralayer couplings. Furthermore we directly observe the spatial Moire pattern and the momentum diffraction, which confirm the presence of atomic superfluid in the bilayer lattices. Our system constitutes a powerful platform to investigate the physics underlying the superconductivity in twisted-bilayer-graphene and to explore other novel quantum phenomena difficult to realize in materials.