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arXiv:2610.38832

Gravitational Interactions in Nuclear Clocks

Konstantin Beyer, Niklas E. Önne, Shimon Kolkowitz, Dolev Bluvstein, Mikhail Lukin, Jun Ye, Igor Pikovski

quant-phgr-qcphysics.atom-phSubmitted Oct 28, 2026• Announced Oct 30, 2026
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Abstract

Atomic clocks achieve extraordinary precision through quantum control over large ensembles of atoms, with precision increasing and atom number advancing steadily. Emerging nuclear clock technology encodes clock states in nuclear rather than electronic transitions, offering a new frontier for precision measurement. Here we study whether a large ensemble of such clock nuclei could be used to observe their mutual gravitational interaction. We investigate the gravitational redshift induced by neighboring atoms, including nuclear energy superpositions as sources of gravity, giving rise to a genuinely quantum gravitational interaction between pairs of nuclei. We find that the resulting clock frequency shift due to mutual gravity may become non-negligible for a macroscopic number of nuclei, for instance in a solid-state thorium clock, and we propose approaches to mitigate electromagnetic field effects by exploiting spatial symmetry and high-precision spectroscopy. We further discuss how energy-induced mass superpositions could be directly probed using external gravitational field sensors. By contrast, observing gravity-induced entanglement involving clocks would require substantially greater experimental advances due to decoherence from spontaneous emission. Taken together, our results suggest that nuclear clocks, either alone or in combination with complementary sensors such as optomechanical systems, may offer a future route toward probing gravity at short distances and testing gravitating quantum source masses beyond the Newtonian limit.

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Atomic clocks achieve extraordinary precision through quantum control over large ensembles of atoms, with precision increasing and atom number advancing steadily. Emerging nuclear clock technology encodes clock states in nuclear rather than electronic transitions, offering a new frontier for precision measurement. Here we study whether a large ensemble of such clock nuclei could be used to observe their mutual gravitational interaction. We investigate the gravitational redshift induced by neighboring atoms, including nuclear energy superpositions as sources of gravity, giving rise to a genuinely quantum gravitational interaction between pairs of nuclei. We find that the resulting clock frequency shift due to mutual gravity may become non-negligible for a macroscopic number of nuclei, for instance in a solid-state thorium clock, and we propose approaches to mitigate electromagnetic field effects by exploiting spatial symmetry and high-precision spectroscopy. We further discuss how energy-induced mass superpositions could be directly probed using external gravitational field sensors. By contrast, observing gravity-induced entanglement involving clocks would require substantially greater experimental advances due to decoherence from spontaneous emission. Taken together, our results suggest that nuclear clocks, either alone or in combination with complementary sensors such as optomechanical systems, may offer a future route toward probing gravity at short distances and testing gravitating quantum source masses beyond the Newtonian limit.
This thesis examines how atomic quantum systems can be utilized to probe spacetime effects in regimes where quantum mechanics and general relativity intersect, and how gravitational phenomena imprint on experimentally accessible observables. The work is based on two complementary studies. In Article I, we propose an experimental scheme that combines trapped-atom interferometry with Ramsey interrogation to realize a clock held in a spatial superposition at two heights in Earth’s gravitational field. Using a path-integral treatment of interferometric phases and incorporating the internal-energy contribution to mass, we derive leading relativistic corrections and identify two signatures of proper-time superposition: (i) oscillations of interferometric visibility and (ii) an effective shift of the clock transition frequency. We argue that this frequency-shift signature may be within reach of current or near-term technology, even when visibility changes are too small to resolve. In Article II, we develop a general framework for spontaneous emission in curved spacetime and apply it to a gravitational-wave background. We demonstrate that gravitational waves can induce spectral sidebands and directional modulations in the emitted radiation, and formulate parameter estimation via Fisher-information-based sensitivity bounds, yielding order-of-magnitude requirements for detectability under idealized measurement conditions.
The creation of delocalized coherent superpositions of quantum systems experiencing different relativistic effects is an important milestone in future research at the interface of gravity and quantum mechanics.This milestone could be achieved by generating a superposition of quantum clocks that follow paths with different gravitational time dilation and investigating the consequences on the interference signal when they are eventually recombined.Light-pulse atom interferometry with elements employed in optical atomic clocks is a promising candidate for that purpose, but it suffers from major challenges including its insensitivity to the gravitational redshift in a uniform field.All of these difficulties can be overcome with the novel scheme presented here, which is based on initializing the clock when the spatially separate superposition has already been generated and performing a doubly differential measurement where the differential phase shift between the two internal states is compared for different initialization times.This scheme can be exploited to test the universality of the gravitational redshift with delocalized coherent superpositions of quantum clocks, and it is argued that its experimental implementation should be feasible with a new generation of 10-meter atomic fountains that will soon become available.Interestingly, the approach also offers significant advantages for more compact setups based on guided interferometry or hybrid configurations.Furthermore, in order to provide a solid foundation for the analysis of the various interferometry schemes and the effects that can be measured with them, a general formalism for a relativistic description of atom interferometry in curved spacetime is developed.It can describe freely falling atoms as well as the effects of external forces and guiding potentials, and it can be applied to a very wide range of situations.As an important ingredient for quantum-clock interferometry, suitable diffraction mechanisms for atoms in internal-state superpositions are investigated too.Finally, the relation of the proposed doubly differential measurement scheme to other experimental approaches and to tests of the universality of free fall is discussed in detail.
Atomic interference experiments can probe the gravitational redshift via the internal energy splitting of atoms and thus give direct access to test the universality of the coupling between matter-energy and gravity at different spacetime points. By including possible violations of the equivalence principle in a fully quantized treatment of all atomic degrees of freedom, we characterize how the sensitivity to gravitational redshift violations arises in atomic clocks and atom interferometers, as well as their underlying limitations. Specifically, we show that: (i) Contributions beyond linear order to trapping potentials lead to such a sensitivity of trapped atomic clocks. (ii) Bragg-type interferometers, even with a superposition of internal states, with state-independent, linear interaction potentials are at first insensitive to gravitational redshift tests. However, modified configurations, for example by relaunching the atoms, can mimic such tests under certain conditions and may constitute a competitive alternative. (iii) Guided atom interferometers are comparable to atomic clocks. (iv) Internal transitions lead to state-dependent interaction potentials through which light-pulse atom interferometers can become sensitive to gravitational redshift violations.
The creation of delocalized coherent superpositions of quantum systems experiencing di erent relativistic e ects is an important milestone in future research at the interface of gravity and quantum mechanics. This could be achieved by generating a superposition of quantum clocks that follow paths with di erent gravitational time dilation and investigating the consequences on the interference signal when they are eventually recombined. Light-pulse atom interferometry with elements employed in optical atomic clocks is a promising candidate for that purpose, but su ers from major challenges including its insensitivity to the gravitational redshift in a uniform eld. All these di- culties can be overcome with a novel scheme presented here which is based on initializing the clock when the spatially separate superposition has already been generated and performing a doubly differential measurement where the di erential phase shift between the two internal states is compared for di erent initialization times. This can be exploited to test the universality of the gravitational redshift (UGR) with delocalized coherent superpositions of quantum clocks and it is argued that its experimental implementation should be feasible with a new generation of 10-meter atomic fountains that will soon become available. Interestingly, the approach also o ers signi cant advantages for more compact set-ups based on guided interferometry or hybrid con gurations. Furthermore, in order to provide a solid foundation for the analysis of the various interferometry schemes and the e ects that can be measured with them, a general formalism for a relativistic description of atom interferometry in curved spacetime is developed. It can deal with freely falling atoms, but also include the e ects of external forces and guiding potentials, and can be applied to a very wide range of situations. As an important ingredient for quantum-clock interferometry, suitable difraction mechanisms for atoms in internal-state superpositions are investigated too. Finally, the relation of the proposed doubly-di erential measurement scheme to other experimental approaches and to tests of the universality of free fall (UFF) is discussed in detail.
Remarkable advances in atom interferometry have enabled the creation of macroscopically delocalized quantum superpositions with atomic wave packets separated up to half a meter. Nevertheless, in all cases realized so far the differences in the dynamics of the two wave packets of the superposition can be entirely described in terms of Newtonian mechanics. Therefore, the creation of delocalized coherent superpositions of quantum systems experiencing different relativistic effects is an important milestone in future research at the interface of gravity and quantum mechanics. This could be achieved by generating a superposition of quantum clocks that follow paths with different gravitational time dilation and investigating the consequences on the interference signal when they are eventually recombined. After explaining the major challenges that quantum-clock interferometry based on light-pulse atom interferometers is confronted with (including their insensitivity to gravitational redshift in a uniform field), I will present a promising scheme capable of measuring the effects of gravitational time dilation in interfering quantum clocks. Its experimental implementation should be within reach of the 10-meter atomic fountains of Sr and Yb atoms that will soon become available in Stanford and HITec (Hanover) respectively.
A promising route to testing quantum gravity in the laboratory is to look for gravitationally induced entanglement (GIE) between two or more quantum matter systems. To date, proposed tests have primarily focused on microsolid platforms prepared in highly nonclassical states, such as N00N states or strongly squeezed states. Here, we instead consider measuring GIE in atom interferometry as evidence of quantum gravity. We propose placing two atom interferometers next to each other in parallel and looking for correlations in the atom-number statistics at their output ports. Importantly, GIE is possible without challenging macroscopic superposition states, such as N00N or Schrödinger-cat states. Instead, GIE can arise using coherent, near-classical atomic states, substantially reducing the experimental complexity. Observing the effect in this regime would require the total mass of the atom interferometers to be near the Planck mass scale. However, we show that state-of-the-art quantum squeezing techniques in cold-atom systems can significantly lower this mass requirement, and outline realistic pathways by which the necessary mass scales could be achieved in the near future, placing laboratory tests of GIE with atom interferometers within reach.