The ability to efficiently control optical quantum interference by the same device is a challenging task that promises to enable key operations in quantum information processing. Here, we tackle this problem by presenting a composite quantum plasmonic metasurface operating as an ultrathin non-unitary beamsplitter capable of achieving both single photon bosonic bunching and fermionic anti-bunching interference just by varying the incident photons frequency or changing the design dimensions. The presented metasurface combines a plasmonic grating corrugated by periodic nanoslits that can achieve extraordinary optical transmission with additional nanostripes on top forming nanocavities characterized by localized gap plasmon resonances. The photon-photon interactions are analyzed based on calculating the quantum coalescence metric which accurately portrays the obtained bunching or anti-bunching quantum interference. The presented quantum interference operation is applicable to both fundamental non-classical light interactions and in the design of more applied quantum optical logic gates used in quantum computing and communications.
The ability to efficiently control optical quantum interference by the same device is a challenging task that promises to enable key operations in quantum information processing. Here, we tackle this problem by presenting a composite quantum plasmonic metasurface operating as an ultrathin non-unitary beamsplitter capable of achieving both single photon bosonic bunching and fermionic anti-bunching interference just by varying the incident photons frequency or changing the design dimensions. The presented metasurface combines a plasmonic grating corrugated by periodic nanoslits that can achieve extraordinary optical transmission with additional nanostripes on top forming nanocavities characterized by localized gap plasmon resonances. The photon-photon interactions are analyzed based on calculating the quantum coalescence metric which accurately portrays the obtained bunching or anti-bunching quantum interference. The presented quantum interference operation is applicable to both fundamental non-classical light interactions and in the design of more applied quantum optical logic gates used in quantum computing and communications.
Surface plasmon polaritons (SPPs) result from collective oscillations of free electrons coupled to an electromagnetic field at a plane interface between a metal and a dielectric medium. As photons, SPPs can be considered either as waves or as bosonic particles [1] and they can experience striking quantum interferences such as Hong-Ou-Mandel (HOM) effect [2]. We use in this paper a plasmonic platform (Fig.1) that can convert photons into plasmons, and separate or recombine them on a plasmonic beamsplitter [3]. Single SPPs are excited using single photons created by parametric down conversion into a periodically-poled KTP crystal. The platform is placed in a Mach-Zehnder interferometer in order to vary the path difference between SPPs before impinging on the beamsplitter. The setup allows us to revisit quantum optics experiments using SPP as carriers of the quantum of energy. Using the same device, we can test the wave-particle duality, two-particle (HOM) interference and non-local control of single plasmon interference using the entanglement between a photon and a SPP [4]. In the case of the HOM experiment, we demonstrate that the losses can be used as a new degree of freedom [5]. Playing with the dephasing between transmission and reflection coefficient of the beamsplitter, we can observe a peak instead of the usually expected dip in the HOM interference (Fig.2), i.e. an anti-coalescence effect of SPP. In this talk, we will introduce the plasmonic device main features as well as the different quantum plasmonics experiments that have been performed thanks to the SPP beamsplitter. These results are essential to understand the SPP quantum behavior or to develop hybrid plasmon-photon systems for potential future applications in quantum communication mediated by SPP. [1] JM Elson and R.H. Ritchie, Phys. Rev. B 4, 4129 (1971) [2] J.S. Fakonas et al., Nat. Phot. 8, 317 (2014) [3] M.C. Dheur et al. , Sc. Advances 2, e151574 (2016) [4] M.C. Dheur et al. ArXiv 1610.07493, B. Vest et al. ArXiv 1610.07479 [5] S. Barnett et al., Phys. Rev. A 57, 2134 (1998) Fig.1: Plasmonic platform used for the quantum optics experiment (B). It consists in two SPP launchers (A), a plasmonic beamsplitter, and two slits to convert SPP to photons in the glass substrate. The plasmonic interference can thus be probed using single photon counting modules. Fig2: HOM experiment on a lossy plasmonic beamsplitter, whose complex amplitude reflection and transmission factors are denoted r and t respectively. The usual HOM dip is observed when r = it (left), a peak in the coincidence rate is shown when r = t.
Beamsplitters represent fundamental components in both classical and quantum optical systems, enabling the distribution of light, as well as the generation of interference, superposition and entanglement. However, optical networks constructed from conventional bulk 2x2-beamsplitters encounter inherent scalability issues, as the number of required beamsplitters scales quadratically with the number of optical modes for a fully connected network. Metasurfaces offer a promising route to overcome these constraints. By manipulating light at the wavelength scale compact optical components with advanced functionalities can be constructed, which address several modes simultaneously. In this work, we design and experimentally utilize a metasurface as a multiport beamsplitter. Furthermore, we realize a multimode interferometer composed of two cascaded metasurfaces. We characterize the individual and cascaded metasurfaces using classical light, showing controllable splitting ratios through tunable phase relations. We then expand the approach to quantum light, employing single photons to demonstrate second- and third-order photon correlations, as well as single photon interference across multiple spatial paths. These results establish metasurface-based multiport beamsplitters as a scalable and reconfigurable platform bridging classical and quantum photonics.
Beamsplitters represent fundamental components in both classical and quantum optical systems, enabling the distribution of light, as well as the generation of interference, superposition, and entanglement. However, optical networks constructed from conventional bulk 2 × 2-beamsplitters encounter inherent scalability issues, as the number of required beamsplitters scales quadratically with the number of optical modes for a fully connected network. Metasurfaces offer a promising route to overcome these constraints. By manipulating light at the wavelength scale, compact optical components with advanced functionalities can be constructed, which address several modes simultaneously. In this work, we design and experimentally utilize a metasurface as a multiport beamsplitter. Furthermore, we realized a multimode interferometer composed of two cascaded metasurfaces. We characterize the individual and cascaded metasurfaces by using classical light, showing controllable splitting ratios through tunable phase relations. We then expand the approach to quantum light, employing single photons to demonstrate second- and third-order photon correlations as well as single photon interference across multiple spatial paths. These results establish metasurface-based multiport beamsplitters as a scalable and reconfigurable platform bridging classical and quantum photonics.
The ability of phase-change materials to reversibly and rapidly switch between two stable phases has driven their use in a number of applications such as data storage and optical modulators. Incorporating such materials into metasurfaces enables new approaches to the control of optical fields. In this article we present the design of novel switchable metasurfaces that enable the control of the nonclassical two-photon quantum interference. These structures require no static power consumption, operate at room temperature, and have high switching speed. For the first adaptive metasurface presented in this article, tunable nonclassical two-photon interference from -97.7% (anti-coalescence) to 75.48% (coalescence) is predicted. For the second adaptive geometry, the quantum interference switches from -59.42% (anti-coalescence) to 86.09% (coalescence) upon a thermally driven crystallographic phase transition. The development of compact and rapidly controllable quantum devices is opening up promising paths to brand-new quantum applications as well as the possibility of improving free space quantum logic gates, linear-optics bell experiments, and quantum phase estimation systems.
Metasurfaces have proven themselves an exotic ability to harness light at nano-scale, being important not only for classical but also for quantum optics. Dynamic manipulation of the quantum states is at the heart of quantum information processing; however, such function has been rarely realized with metasurfaces so far. Here, we report an all-optical dynamic modulation of the photonic quantum states using the nonlinear metasurface. The metasurface consists of a metallic nanostructure combined with a photoisomerizable azo layer. By tuning the plasmonic resonance through optically switching the azo molecules between their binary isomeric states, we have realized dynamic control of transmission efficiencies of orthogonally polarized photons and also the phase delay between them, thereby an entangled state was efficiently controlled. As an illustration, a quantum state distillation has been demonstrated to recover a Bell state from a non-maximally entangled one to that with fidelities higher than 98%. Our work would enrich the functions of the metasurface in the quantum world, from static to dynamic modulation, making the quantum metasurface going practical.