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arXiv:2610.18401

Orbital Angular Momentum Transfer and Beam-Quality Limits in Fork-Grating Electron Diffraction

P. K. Tsiopa, S. S. Baturin

physics.opticsquant-phSubmitted Oct 13, 2026• Announced Oct 14, 2026
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Abstract

We analyze fork-grating generation of electron vortex beams beyond the ideal single-mode approximation. The incident beam is described as a paraxial Gaussian ensemble with finite transverse momentum spread and a first electromagnetic Hartree phase accumulated before the grating. Within Fresnel propagation we derive an analytical expression for each diffraction order and determine the corresponding orbital-angular-momentum statistics. The mean OAM of a selected order remains fixed by the topological rule, $\langle L_z\rangle_m=mp\hbar$, while its variance is set by the residual transverse momentum spread of the beam prepared at the grating. For the Gaussian mixture, the transverse purity is $\mathcal P_{\perp,m}=[1+2(ΔL_{z,m}/\hbar)^2]^{-1}$. The observed annular profile is governed by a separate propagation-dependent blurring scale, so a beam can retain well-defined mean OAM while having low transverse purity or a partially filled vortex minimum. Within the radial phase-screen approximation, the Hartree self-field modifies the propagated profile while preserving the full-plane OAM moments and transverse purity.

Comments
14 pages 4 figures

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We analyze fork-grating generation of electron vortex beams beyond the ideal single-mode approximation. The incident beam is described as a paraxial Gaussian ensemble with finite transverse momentum spread and a first electromagnetic Hartree phase accumulated before the grating. Within Fresnel propagation we derive an analytical expression for each diffraction order and determine the corresponding orbital-angular-momentum statistics. The mean OAM of a selected order remains fixed by the topological rule, ⟨Lz⟩m=mpℏ\langle L_z\rangle_m=mp\hbar⟨Lz​⟩m​=mpℏ, while its variance is set by the residual transverse momentum spread of the beam prepared at the grating. For the Gaussian mixture, the transverse purity is P⊥,m=[1+2(ΔLz,m/ℏ)2]−1\mathcal P_{\perp,m}=[1+2(ΔL_{z,m}/\hbar)^2]^{-1}P⊥,m​=[1+2(ΔLz,m​/ℏ)2]−1. The observed annular profile is governed by a separate propagation-dependent blurring scale, so a beam can retain well-defined mean OAM while having low transverse purity or a partially filled vortex minimum. Within the radial phase-screen approximation, the Hartree self-field modifies the propagated profile while preserving the full-plane OAM moments and transverse purity.
The generation of relativistic vortex electron beams via photoemission requires ultraviolet laser beams with well-controlled orbital angular momentum (OAM) and compatibility with radio-frequency (RF) photoinjector drive-laser systems. High-OAM vortex beams at a wavelength of 266 nm are generated using three fabricated diffractive optical elements integrated into an operational photoinjector beamline: a reflective fork grating, a high-topological-charge spiral phase plate, and binary axicons. The spiral phase plate produces a high-purity Laguerre-Gaussian mode with an OAM of l = 64 and a conversion efficiency of 80%, whereas binary axicons generate low-divergence quasi-Bessel beams forming a superposition of multiple OAM states with a finite OAM bandwidth imposed by their binary phase structure. Fork gratings provide flexible access to lower OAM values and enable robust modal diagnostics. The generated beams are characterized using cylindrical-lens mode conversion and radial intensity analysis, demonstrating practical control of both the OAM content and spectral bandwidth of ultraviolet structured light for accelerator-based applications.
A novel encoding method based on the orbital angular momentum (OAM) mode and radial mode of composite vortex beams is proposed. The superposition of two vortex beams generates 32 different types of composite vortex beams: one of them is a Laguerre–Gaussian (LG) beam with a fixed OAM mode and radial mode, and the other is a LG beam containing four radial modes (p = 0, 1, 2, 3) and eight OAM modes with the same interval (l = ±3, ±5, ±7, ±9). A specially designed composite fork-shaped grating (CFG) is utilized to generate the intensity array pattern, and the received composite vortex beam is diffracted into a Gaussian beam with the relevant coordinates. Based on the coordinates and the number of bright rings in the intensity pattern, the OAM modes and radial modes of the two vortex beams composing the superposition state are determined, and finally the received composite vortex beam is decoded into the initially propagated information sequence. The correctness and effectiveness of the proposed encoding are confirmed through the comparative analysis of the correlation of the optical fields at both the transmitter and receiver in the two scenarios of interval and non-interval encoding. The proposed encoding method can significantly improve the efficiency of information transmission and its resistance to interference, holding great potential for future applications in free-space optical communication.
We formulate diffractive ring focusing of paraxial beams carrying orbital angular momentum (OAM) through a finite circular aperture as a variational optimization problem. For a fixed topological charge, we determine the real-valued radial pupil that maximizes the intensity at a prescribed ring radius and propagation distance under a normalization constraint on the input field. The resulting problem admits an exact analytical solution: the optimal pupil combines the familiar Fresnel phase structure with an OAM-dependent Bessel radial modulation, and the associated eigenvalue yields a rigorous upper bound on the achievable ring intensity. We further analyze the lens-assisted configuration and derive a simple bound that allows direct comparison between diffractive and refractive vortex focusing. The theory also provides a quantitative framework for evaluating the performance of practical mask designs, including binary Fresnel-Bessel zone plates and amplitude-weighted pupils. We have experimentally tested our predictions in the optical domain by implementing the corresponding vortex beam pupils and comparing their propagation and focusing performance with the optimal solution. Our results establish the vortex-beam analogue of optimal amplitude-only focusing and identify the fundamental limits governing diffractive concentration of structured waves
Understanding how optical orbital angular momentum (OAM) is transferred to matter requires treating recoil and translational motion alongside the internal electronic dynamics. We develop a center-of-mass-resolved theory of one-photon ionization of hydrogen by a monochromatic Laguerre--Gaussian beam and show that the Bessel-vortex photoelectron predicted in fixed-target models is a preparation-dependent limit. For a sharply defined atomic center-of-mass momentum, the recoil records the photon-cone azimuth, and tracing over it generally destroys the coherence required for a pure electron vortex. In the small-transverse-retardation regime, the optical OAM is transferred predominantly to the center-of-mass motion and hence, in the laboratory frame, to the proton. Finite-retardation corrections redistribute angular momentum between center-of-mass and relative motion, while an additional correlation contribution to the electron and proton angular momenta can be tuned through the spatial uncertainty of the atomic center of mass. These results reveal atomic recoil as a key element of OAM transfer in photoionization.
We show that the covariance matrix of any cylindrically symmetric coherent orbital angular momentum (OAM) eigenmode with quantum number ℓ\ellℓ takes a universal form depending only on ⟨r2⟩\langle r^2\rangle⟨r2⟩, ⟨kr2⟩\langle k_r^2\rangle⟨kr2​⟩, and ℓ\ellℓ, independently of the radial profile, and that this form is identical to the covariance matrix of a twisted Gaussian Schell-model (TGSM) beam.} More specifically, both matrices share the same pattern of zero and nonzero entries, with the off-diagonal blocks proportional to ℓ\ellℓ and the TGSM twist parameter uuu, respectively. This result holds for an arbitrary radial profile and provides direct term-by-term identification of parameters between the two sets of beams. We work out the correspondence in detail for three important families: Laguerre--Gaussian (LG), Bessel--Gaussian, and perfect vortex beams (PVBs), and derive the conditions under which each coherent OAM mode maps onto a physically realizable TGSM beam. {Because the covariance matrix governs second-moment evolution under arbitrary ABCD (symplectic) transformations, any two beams sharing the same covariance matrix are second-order indistinguishable at every propagation plane. In particular, the matched TGSM and coherent OAM beams share identical beam-width evolution, far-field divergence, and M2M^2M2 beam-quality factor.} In particular, the well-developed TGSM propagation toolbox applies directly to the second-order moment evolution of the three coherent families. We further show that within each beam family the covariance matrix uniquely determines the beam parameters, with exact uniqueness established for LG modes. Additional results include cross-family second-moment equivalence conditions and a proof that PVB modes form a complete orthonormal basis in the limit w→0w\to 0w→0.
Orbital angular momentum (OAM) beams with topological charge ℓ are commonly generated and detected by modulating an incoming field with an azimuthal phase profile of the form exp(iℓϕ) by a variety of approaches. This results in unwanted radial modes and reduced power in the desired OAM mode. Here, we show how to enhance the modal purity in the creation and detection of classical OAM beams and in the quantum detection of OAM photons. Classically, we combine holographic and metasurface control to produce high purity OAM modes and show how to detect them with high efficiency, extending the demonstration to the quantum realm with spatial light modulators. We demonstrate ultra-high purity OAM modes in orders as high as ℓ = 100 and a doubling of dimensionality in the quantum OAM spectrum from a spontaneous parametric downconversion source. Our work offers a simple route to increase the channel capacity in classical and quantum communication using OAM modes as a basis.