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arXiv:2609.28694

Mediating gates between polar molecules using microwave-dressed Rydberg atoms

Bas Gerritsen, Sean R. Muleady, Arghavan Safavi-Naini, Alexey V. Gorshkov, Jeremy T. Young

quant-phSubmitted Sep 23, 2026• Announced Sep 25, 2026• 0 citations
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Abstract

We propose a scheme for mediating many simultaneous, fast entangling gates between pairs of polar molecules using Rydberg atoms. By using microwave drives, the dipolar interactions between Rydberg atoms are nullified. Using the freedom left in the microwave dressing parameters, the Rydberg van der Waals interactions are minimized and the Rydberg-molecule interaction is tuned into resonance, allowing for the mediation of a modified iSWAP gate between molecules. In the example of mediating gates between $\rm{{}^{23}Na {}^{133}Cs}$ molecules with $\rm {}^{133}Cs$ atoms, the gate is more than two orders of magnitude faster than an equivalent direct molecule-molecule gate. We model the decay of the dressed Rydberg states and the motion of the atom and molecules and obtain a leading-order estimate of the resulting gate infidelities. Finally, we show that by detecting the state of the Rydberg atom after a gate, a subset of gate errors can be converted into erasure errors and mitigated by post-selection or quantum error-correction.

Comments
6+3 pages, 4+1 figures

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We propose a scheme for mediating many simultaneous, fast entangling gates between pairs of polar molecules using Rydberg atoms. By using microwave drives, the dipolar interactions between Rydberg atoms are nullified. Using the freedom left in the microwave dressing parameters, the Rydberg van der Waals interactions are minimized and the Rydberg-molecule interaction is tuned into resonance, allowing for the mediation of a modified iSWAP gate between molecules. In the example of mediating gates between 23Na133Cs\rm{{}^{23}Na {}^{133}Cs}23Na133Cs molecules with 133Cs\rm {}^{133}Cs133Cs atoms, the gate is more than two orders of magnitude faster than an equivalent direct molecule-molecule gate. We model the decay of the dressed Rydberg states and the motion of the atom and molecules and obtain a leading-order estimate of the resulting gate infidelities. Finally, we show that by detecting the state of the Rydberg atom after a gate, a subset of gate errors can be converted into erasure errors and mitigated by post-selection or quantum error-correction.
The advent of digital neutral-atom quantum computers relies on the development of fast and robust protocols for high-fidelity quantum operations. In this work, we introduce a novel scheme for entangling gates using four atomic levels per atom: a ground-state qubit and two Rydberg states. A laser field couples the qubit to one of the two Rydberg states, while a microwave field drives transitions between the two Rydberg states, enabling a resonant dipole-dipole interaction between different atoms. We show that controlled- Z gates can be realized in this scheme without requiring optical phase modulation and relying solely on a microwave field with time-dependent phase and amplitude. We demonstrate that such gates are faster and less sensitive to Rydberg decay than state-of-the-art Rydberg gates based on van der Waals interactions. Moreover, we systematically stabilize our protocol against interatomic distance fluctuations and analyze its performance in realistic setups with rubidium or cesium atoms. Our results open up new avenues to the use of microwave-driven dipolar interactions for quantum computation with neutral atoms.
We study the possibility to use interaction between a polar molecule in the ground electronic and vibrational state and a Rydberg atom to construct two-qubit gates between molecular qubits and to coherently control molecular states. A polar molecule within the electron orbit in a Rydberg atom can either shift the Rydberg state, or form a Rydberg molecule. Both the atomic shift and the Rydberg molecule states depend on the initial internal state of the polar molecule, resulting in molecular state dependent van der Waals or dipole-dipole interaction between Rydberg atoms. Rydberg atoms mediated interaction between polar molecules can be enhanced up to 10(3) times. We describe how the coupling between a polar molecule and a Rydberg atom can be applied to coherently control molecular states, and specifically, to individually address molecules in an optical lattice, and to non-destructively readout molecular qubits.
Tweezer arrays of polar molecules present new opportunities for quantum science and quantum information. However, a major challenge, especially in bialkali molecule platforms, is the fact that current measurement schemes for the internal states are destructive. In this work, we present a method to use Rydberg atoms to nondestructively measure the internal state of a molecular qubit. We achieve this via microwave dressing of both molecules and Rydberg atoms, allowing us to tune the interactions so that there are minimal Rydberg-Rydberg interactions and many measurements can take place simultaneously. We consider two experimentally-motivated examples of detecting 23^{23}23Na133^{133}133Cs and 87^{87}87Rb133^{133}133Cs with 133^{133}133Cs atoms. Finally, we discuss several strategies for mitigating various sources of crosstalk.
We demonstrate finite range binding potentials between pairs of Rydberg atoms interacting with each other via attractive and repulsive van der Waals potentials and driven by a microwave field. We show that, using destructive quantum interference to cancel single-atom Rydberg excitation, the Rydberg-dimer states can be selectively and coherently populated from the two-atom ground state. This can be used to realize a two-qubit interaction gate which is not susceptible to mechanical forces between the atoms and is therefore immune to motional decoherence.
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We investigate the interaction between Rydberg atoms, whose electronic states are dressed by multiple microwave fields. Numerical calculations are used for an exact description of the microwave induced interactions, and employed to benchmark a perturbative treatment that yields simple insights into the involved mechanisms. Based on this theory, we demonstrate that microwave dressing provides a powerful approach to control dipolar as well as van der Waals interactions and even permits us to turn them off entirely. In addition, the proposed scheme also opens up possibilities for engineering dominant three-body interactions.