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arXiv:2609.18867

Liouvillian exceptional points in the emergence of quantum synchronization

Carlos Ortega Taberner, Rosalind E. Cotton, Paul R. Eastham

quant-phcond-mat.mes-hallphysics.opticsSubmitted Sep 16, 2026• Announced Sep 17, 2026
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Abstract

The coupling between self-sustained oscillators, such as lasers or polariton condensates, leads to different steady-states in different regimes. Weak coupling allows the oscillators to behave independently, with different frequencies and uncorrelated phases, while stronger coupling can produce synchronization. In classical or semiclassical theories transitions between these steady-states correspond to changes in the topology of the phase space attractors and occur at generalized exceptional points. We investigate the corresponding changes in a quantum theory of coupled lasers or condensates. We show how the different steady-state regimes of the classical limit give rise to distinct forms for the spectra and eigenmatrices of the slow modes of the Liouvillian. By following the spectral flow between the different regimes we show that the synchronization transition is controlled by cascades of exceptional points in these slow modes, protected by a generalized PT symmetry. Our results show how singularities of the quantum Liouvillian control the different dynamical regimes, and give rise to experimental signatures of the synchronization transition which remain well-defined in the few-particle regime dominated by quantum effects.

Comments
18 pages, 9 figures

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The coupling between self-sustained oscillators, such as lasers or polariton condensates, leads to different steady-states in different regimes. Weak coupling allows the oscillators to behave independently, with different frequencies and uncorrelated phases, while stronger coupling can produce synchronization. In classical or semiclassical theories transitions between these steady-states correspond to changes in the topology of the phase space attractors and occur at generalized exceptional points. We investigate the corresponding changes in a quantum theory of coupled lasers or condensates. We show how the different steady-state regimes of the classical limit give rise to distinct forms for the spectra and eigenmatrices of the slow modes of the Liouvillian. By following the spectral flow between the different regimes we show that the synchronization transition is controlled by cascades of exceptional points in these slow modes, protected by a generalized PT symmetry. Our results show how singularities of the quantum Liouvillian control the different dynamical regimes, and give rise to experimental signatures of the synchronization transition which remain well-defined in the few-particle regime dominated by quantum effects.
Usually, when investigating exceptional points (EPs) of an open Markovian bosonic system, one deals with spectral degeneracies of a non-Hermitian Hamiltonian (NHH), which can correctly describe the system dynamics only in the semiclassical regime. A recently proposed quantum Liouvillian framework [Minganti et al., Phys. Rev. A 100, 062131 (2019)] enables the complete determination of the dynamical properties of such systems and their EPs (referred to as Liouvillian EPs, or LEPs) in the quantum regime by taking into account the effects of quantum jumps, which are ignored in the NHH formalism. Moreover, the symmetry and eigenfrequency spectrum of the NHH become a part of much larger Liouvillian eigenspace. As such, the EPs of an NHH form a subspace of the LEPs. Here we show that once an NHH of a dissipative linear bosonic system exhibits an EP of a certain finite order nnn, it immediately implies that the corresponding LEP can become of any higher order $m\ensuremath{\ge}n$ defined in the infinite Hilbert space. These higher-order LEPs can be identified by the coherence and spectral functions at the steady state. The coherence functions can offer a convenient tool to probe extreme system sensitivity to external perturbations in the vicinity of higher-order LEPs. As an example, we study a linear bosonic system of a bimodal cavity with incoherent mode coupling to reveal its higher-order LEPs; particularly, of second and third order via first- and second-order coherence functions, respectively. Accordingly, these LEPs can be additionally revealed by squared and cubic Lorentzian spectral lineshapes in the power and intensity-fluctuation spectra. Moreover, we demonstrate that these EPs can also be associated with spontaneous parity-time (PT\mathcal{PT}PT) and anti-PT\mathcal{PT}PT-symmetry breaking in the system studied. These symmetries can be switched in the output fields (the so-called supermodes) of an additional linear coupler with a properly chosen coupling strength. Thus, we show that the initial loss-loss dynamics for the supermodes can be equivalent to the balanced gain-loss evolution.
In this paper we consider a spin chain locally coupled to dissipative environments with unbalanced gain and loss and explore the relation between the emergence of synchronization and exceptional points. For our model in the Liouvillian formalism the matrix of the Liouvillian superoperator is block diagonal and the different blocks correspond to the dynamics of different observables. We find that for ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\sigma}}}^{z}$ corresponding to the block having a single Liouvillian exceptional point (LEP), when the coupling strength between the nearest spins is beyond the LEP, the synchronization or antisynchronization will occur. For ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\sigma}}}^{x}$ and ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\sigma}}}^{y}$ corresponding to the block having two LEPs, when the coupling strength between the nearest spins is beyond both LEPs, the synchronization or antisynchronization will appear, and as time evolves the dynamical transition between synchronization and antisynchronization can occur. Moreover, we also find that the initial state of the system does not affect the emergence of synchronization or antisynchronization, but it determines whether the system is synchronized or antisynchronized and affects the time at which the dynamical transition between synchronization and antisynchronization occurs. Furthermore, by postselecting the quantum trajectories without quantum jump, the system can exhibit Hamiltonian exceptional points, and we find that quantum jumps play an important role in the synchronization of the system.
Non-Hermitian degeneracies of Lindblad generators (Liouvillian exceptional points) can induce non-exponential relaxation and higher-order poles in dynamical response functions. A collective spin coupled to a polarized Markovian bath exhibits an \emph{exceptional spectral phase} in which defective Liouvillian modes imprint super-Lorentzian features in frequency-resolved spectra. We compute the emission spectrum via the Liouvillian resolvent, identify symmetry-sector selection rules, and demonstrate that exceptional-point signatures are strongly state-dependent: they are suppressed in steady-state fluorescence yet become unambiguous for generic (infinite-temperature or random) initial states. Our results provide an experimentally accessible spectroscopic diagnostic of many-body Liouvillian exceptional phases and clarify when steady-state emission can (and cannot) reveal them.
Viewing a quantum thermal machine as a non-Hermitian quantum system, we characterize in full generality its analytical time-dependent dynamics by deriving the spectrum of its non-Hermitian Liouvillian for an arbitrary initial state.We show that the thermal machine features a number of Liouvillian exceptional points (EPs) for experimentally realistic parameters, in particular, a third-order exceptional point that leaves signatures both in short-and long-time regimes.Remarkably, we demonstrate that this EP corresponds to a regime of critical decay for the quantum thermal machine towards its steady state, bearing a striking resemblance with a critically damped harmonic oscillator.These results open up exciting possibilities for the precise dynamical control of quantum thermal machines exploiting exceptional points from non-Hermitian physics and are amenable to state-of-the-art solid-state platforms such as semiconducting and superconducting devices.
Exceptional points in non-Hermitian quantum systems give rise to novel genuine quantum phenomena. Recent explorations of exceptional-point-induced quantum phase transitions have extended from discrete-variable to continuous-variable-encoded quantum systems. However, quantum phase transitions driven by Liouvillian exceptional points (LEPs) in continuous-variable platforms remain largely unexplored. Here, we construct and investigate a Liouvillian exceptional structure based on a driven-dissipative Kerr-cat qubit. Through numerical simulations, we reveal a quantum phase transition occurring at the LEP characterized by a sudden change in dynamical behavior from underdamped oscillations to overdamped relaxations as visualized via Wigner functions and Bloch sphere trajectories. Notably the negativity of the Wigner function serves as a direct signature of genuine quantum coherence unattainable in conventional single-qubit non-Hermitian systems. Furthermore, we introduce the phase difference between the off-diagonal elements of the Liouvillian eigenmatrices as a novel parameter to quantify the transition. Our results establish the Kerr-cat qubit as a novel continuous-variable setting for exploring dissipative quantum criticality and intrinsic non-Hermitian physics.
Abstract Hamiltonian exceptional points (HEPs) are spectral degeneracies of non-Hermitian Hamiltonians describing classical and semiclassical open systems with losses and/or gain. However, this definition overlooks the occurrence of quantum jumps in the evolution of open quantum systems. These quantum effects are properly accounted for by considering quantum Liouvillians and their exceptional points (LEPs). Specifically, an LEP corresponds to the coalescence of two or more eigenvalues and the corresponding eigenmatrices of a given Liouvillian at critical values of external parameters (Minganti et al 2019 Phys. Rev. A 100 062131). Here, we explicitly describe how standard quantum process tomography, which reveals the dynamics of a quantum system, can be readily applied to detect and characterize quantum LEPs of quantum non-Hermitian systems. We conducted experiments on an IBM quantum processor to implement a prototype model with one-, two-, and three qubits simulating the decay of a single qubit through competing channels, resulting in LEPs but not HEPs. Subsequently, we performed tomographic reconstruction of the corresponding experimental Liouvillian and its LEPs using both single- and two-qubit operations. This example underscores the efficacy of process tomography in tuning and observing LEPs even in the absence of HEPs.