Coherent and efficient light-matter interfaces between an atom and a single mode of the electromagnetic field are essential for quantum technologies. Traditionally, these systems employ optical cavities or waveguides to isolate a specific mode of light, but a more recent approach is to engineer antennas from ordered configurations of trapped ultracold atoms that exhibit controllable and directed scattering. In this work, we propose a method to engineer an antenna from the center-of-mass wavefunction of a single atom, which can produce directed emission and thereby exhibit strong coupling to a target mode of light in free space. We predict that the resulting single-atom cooperativity can be comparable to the current state of the art in optical cavity and waveguide QED experiments. Building on this approach, we show that a wavepacket antenna becomes a single-atom mirror in the linear response regime. We study the modified dipole-dipole interactions and band structure of chains of such emitters, which can exhibit sub- and superradiance at spacings much larger than the wavelength of the light. Extending our approach to multi-level atoms, we propose a method to achieve arbitrary spatial scattering from a single atom, including uni-directional spontaneous emission. Finally, we elucidate how our approach can enhance cooperative scattering in conventional arrays of tightly trapped atoms.
Coherent and efficient light-matter interfaces between an atom and a single mode of the electromagnetic field are essential for quantum technologies. Traditionally, these systems employ optical cavities or waveguides to isolate a specific mode of light, but a more recent approach is to engineer antennas from ordered configurations of trapped ultracold atoms that exhibit controllable and directed scattering. In this work, we propose a method to engineer an antenna from the center-of-mass wavefunction of a single atom, which can produce directed emission and thereby exhibit strong coupling to a target mode of light in free space. We predict that the resulting single-atom cooperativity can be comparable to the current state of the art in optical cavity and waveguide QED experiments. Building on this approach, we show that a wavepacket antenna becomes a single-atom mirror in the linear response regime. We study the modified dipole-dipole interactions and band structure of chains of such emitters, which can exhibit sub- and superradiance at spacings much larger than the wavelength of the light. Extending our approach to multi-level atoms, we propose a method to achieve arbitrary spatial scattering from a single atom, including uni-directional spontaneous emission. Finally, we elucidate how our approach can enhance cooperative scattering in conventional arrays of tightly trapped atoms.
The ordered atomic array emerges as a versatile atom-photon interface for exquisite control of light-matter interaction at the nanoscale. In particular, the one-dimensional atom-waveguide system can achieve strong coupling between a single atom and a photon, where two atomic mirrors coupled to waveguide act as a high-finesse cavity. In this work we show that under the strong-coupling regime, the mirror atoms arranged in the form of a Su-Schrieffer-Heeger chain are advantageous in decoherence suppression compared to a nontopological Bragg configuration, manifesting a significant increase in the lifetime of dressed states, substantial narrowing of the spectral linewidth, and order-of-magnitude enhancement of the cooperativity of light-matter interaction. Furthermore, subradiant dressed states with a decay rate smaller than the emission rate of a free-space atom are found in the dissipationless atomic cavity with a few mirror atoms, which cannot be achieved with a Bragg atomic mirror. A theory of the local density of states (LDOS) of the atomic cavity is presented and reveals that the decoherence suppression is directly related to the negative LDOS in a wide frequency range contributed by the bulk modes of the topological atomic cavity. This peculiar feature of the LDOS indicates the destructive quantum interference of photon scattering by the topological edge- and bulk-state channels. Our work demonstrates the great potential of topology in engineering quantum states and enhancing quantum coherence for future applications in quantum computing and quantum information processing.
Cavity quantum electrodynamics (cavity QED) enables the control of light-matter interactions at the single-photon level, rendering it a key component of many quantum technologies. Its practical realization, however, is complex since it involves placing individual quantum emitters close to mirror surfaces within a high-finesse cavity. In this work, we propose a cavity QED architecture fully based on atoms trapped in free space. In particular, we show that a pair of two-dimensional, ordered arrays of atoms can be described by conventional cavity QED parameters. Such an atom-array cavity exhibits the same cooperativity as a conventional counterpart with matching mirror specifications even though the cavity coupling strength and decay rate are modified by the narrow bandwidth of the atoms. We estimate that an array cavity composed of Rb 87 atoms in an optical lattice can reach a cooperativity of about 10. This value can be increased suppressing atomic motion with larger trap depths and may exceed 10 4 with an ideal placement of the atoms. To reduce the experimental complexity of our scheme, we propose a spatially dependent ac Stark shift as an alternative to curving the arrays, which may be of independent interest. In addition to presenting a promising platform for cavity QED, our work creates opportunities for exploring novel phenomena based on the intrinsic nonlinearity of atom arrays and the possibility to dynamically control them.
Recent experimental advances in preparing regular defect-free 2D arrays of atoms with optical traps have offered new opportunities to engineer strong collective couplings between light and atoms as quantum optical dipoles. Applications of such collective light-matter interactions include the realization of atom-thick mirrors, retrieval of quantum memories with high efficiency, or the implementation of topological quantum optics. I will present novel applications in the context of quantum networking. First, I will discuss the design of a chiral photonic quantum link, where distant single atoms interact by exchanging photons propagating in a unique direction in free space. This is achieved by coupling both single atoms, representing qubits implemented using a pair of Rydberg states, to bi-layer atomic arrays which act as quantum phased-array antennas. Exploiting the combination of a “Rydberg-dressing” laser and a control laser driving the atomic arrays, an effective Rydberg dipole-dipole interaction can be engineered between atoms and atomic arrays as quantum emitters, allowing to match the spatial modes of spontaneously emitted and absorbed photons to a Gaussian mode of interest. In this way, we realize a chiral quantum interface, i.e., where atoms couple to photonic modes with a unique direction of propagation. This setup provides a basic building block of a novel platform for quantum networks in free space, i.e., without requiring coupling atoms to modes of cavities or nanostructures, which I will illustrate with the deterministic coherent transfer of quantum states between single atoms with high fidelity. Second, I will discuss the collective radiation properties of two distant single-layer atomic arrays acting as quantum memories. This system can support a long-lived non-local superposition state of atomic excitations exhibiting strong subradiance. This “dark” mode consists of an atomic excitation which is delocalized between the two distant atomic arrays, in such a way that the overall radiation is strongly suppressed by quantum interference. I will describe the preparation of these states and their application as resource of non-local entanglement. In particular, by weakly driving the arrays, the state of the quantum memories, localized in each array, can be transferred to this “non-local” subradiant state, allowing again for a deterministic coherent quantum state transfer with high fidelity between the memories. Finally, I will discuss experimental realizations using cold atoms in optical trap arrays, and the effect of experimental imperfections in the arrays, such as finite defect probability, temperature, and depth of the optical traps.
We describe the design of an artificial `free space' 1D-atom for quantum optics, where we implement an effective two-level atom in a 3D optical environment with a chiral light-atom interface, i.e. absorption and spontaneous emission of light is essentially unidirectional. This is achieved by coupling the atom of interest in a laser-assisted process to a `few-atom' array of emitters with subwavelength spacing, which acts as a phased-array optical antenna. We develop a general quantum optical model based on Wigner-Weisskopf theory, and quantify the directionality of spontaneous emission in terms of a Purcell β-factor for a given Gaussian (paraxial) mode of the radiation field, predicting values rapidly approaching unity for `few-atom' antennas in bi- and multilayer configurations. Our setup has for neutral atoms a natural implementation with laser-assisted Rydberg interactions, and we present a study of directionality of emission from a string of trapped ions with superwavelength spacing.
Enhancing light-matter coupling at the level of single quanta is essential for numerous applications in quantum science. The cooperative optical response of subwavelength atomic arrays has been found to open new pathways for such strong light-matter couplings, while simultaneously offering access to multiple spatial modes of the light field. Efficient single-mode free-space coupling to such arrays has been reported, but the spatial control over the modes of outgoing light fields has remained elusive. Here, we demonstrate such spatial control over the optical response of an atomically thin mirror formed by a subwavelength array of atoms in free space using a single controlled ancilla atom excited to a Rydberg state. The switching behavior is controlled by the admixture of a small Rydberg fraction to the atomic mirror, and consequently strong dipolar Rydberg interactions with the ancilla. Driving Rabi oscillations on the ancilla atom, we demonstrate coherent control of the transmission and reflection of the array. These results represent a step towards the realization of quantum coherent metasurfaces, the demonstration of controlled atom-photon entanglement and deterministic engineering of quantum states of light.
Neutral-atom array and cavity quantum electrodynamics offer complementary strengths for quantum science: scalable, reconfigurable qubit architectures and strong coherent light-matter coupling. Combining them in a single platform requires an optical cavity with simultaneously high cooperativity, sufficient mode volume to accommodate atom array, and ample side optical access for atom trapping, imaging, cooling, and rearrangement, a combination that is challenging to achieve. Here we realize an atomic array integrated with a millimeter-scale Fabry--Pérot cavity whose optically-characterized single-atom cooperativity reaches ηcav=125±13. Atom-cavity transmission spectra of trapped atoms yield an effective spectroscopic cooperativity ηspec=106±3, providing an in-situ verification of strong coupling in the integrated platform. In this integrated system, we achieve a state-measurement fidelity of 99.925−18+15% for a single atom with a 4-μs readout time. We also demonstrate simultaneous coupling of up to 21 individually trapped atoms to the antinode of the cavity mode. The key technical advance is a two-step mirror-fabrication method combining precision mechanical shaping and carbon-dioxide laser polishing, which produces concave fused-silica mirrors with sub-millimeter radii of curvature and residual roughness below 2A˚. Our results establish a regime of cavity-integrated atomic array that simultaneously provides high cooperativity, large mode volume, and flexible manipulation of individual atoms, opening opportunities for cavity-assisted quantum state readout and long-range entanglement-engineering in atom-array platforms.