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arXiv:2609.07082

Broad-angle photon-pair generation from flatband quasi-BIC resonant 3R-MoS$_{2}$ metasurfaces

Tingting Liu, Huifu Qiu, Xintong Shi, Jumin Qiu, Shuyuan Xiao

Published Sep 7, 2026• 0 citations
arXivHTMLPDF

Abstract

Spontaneous parametric down-conversion (SPDC) in ultrathin optical resonant metasurfaces offers a promising platform for integrated quantum light sources. However, conventional resonances suffer from steep momentum dispersion, limiting photon-pair generation to narrow excitation and emission angles. Here, we demonstrate a flatband-resonant 3R-MoS$_{2}$ metasurface for high-efficiency, broad-angle SPDC photon-pair generation. By implementing a supercell symmetry-breaking strategy via Brillouin zone folding, we achieve a flatband quasi-bound states in the continuum (quasi-BICs) resonance in the near-infrared regime that maintains a robust quality factor across a wide range of incident angle. Exploiting the strong local electric field enhancement of resonance and the large second-order susceptibility of 3R-MoS$_{2}$, the metasurface boosts the degenerate SPDC pair-generation rate with orders of magnitude enhancement over an unpatterned film of identical thickness. Crucially, the near-zero band dispersion extends the effective emission angle to $\pm 5^{\circ}$ with negligible spectral drift $\sim 0.1$ nm and high directional tolerance. Under pulsed excitation with a finite spectral bandwidth, the photon pair yield remains high, demonstrating strong spectral locking to the quasi-BIC resonance against pump detunings. This work establishes a versatile strategy for momentum-independent quantum light sources, opening new avenues for scan-free quantum ghost imaging and spatial-frequency quantum processing.

DOI
10.48550/arxiv.2609.07082

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Spontaneous parametric down-conversion (SPDC) in ultrathin optical resonant metasurfaces offers a promising platform for integrated quantum light sources. However, conventional resonances suffer from steep momentum dispersion, limiting photon-pair generation to narrow excitation and emission angles. Here, we demonstrate a flatband-resonant 3R-MoS2_{2}2​ metasurface for high-efficiency, broad-angle SPDC photon-pair generation. By implementing a supercell symmetry-breaking strategy via Brillouin zone folding, we achieve a flatband quasi-bound states in the continuum (quasi-BICs) resonance in the near-infrared regime that maintains a robust quality factor across a wide range of incident angle. Exploiting the strong local electric field enhancement of resonance and the large second-order susceptibility of 3R-MoS2_{2}2​, the metasurface boosts the degenerate SPDC pair-generation rate with orders of magnitude enhancement over an unpatterned film of identical thickness. Crucially, the near-zero band dispersion extends the effective emission angle to ±5∘\pm 5^{\circ}±5∘ with negligible spectral drift ∼0.1\sim 0.1∼0.1 nm and high directional tolerance. Under pulsed excitation with a finite spectral bandwidth, the photon pair yield remains high, demonstrating strong spectral locking to the quasi-BIC resonance against pump detunings. This work establishes a versatile strategy for momentum-independent quantum light sources, opening new avenues for scan-free quantum ghost imaging and spatial-frequency quantum processing.
Abstract We reveal that strongly enhanced generation of photon pairs with narrow frequency spectra and sharp angular correlations can be realised through spontaneous parametric down-conversion in metasurfaces. This is facilitated by creating meta-gratings through nano-structuring of nonlinear films of sub-wavelength thickness to support the extended bound state in the continuum resonances, associated with ultra-high Q-factors, at the biphoton wavelengths across a wide range of emission angles. Such spectral features of photons can be beneficial for various applications, including quantum imaging. Our modelling demonstrates a pronounced enhancement, compared to unpatterned films, of the total photon-pair generation rate normalized to the pump power reaching 1.75 kHz mW−1, which is robust with respect to the angular bandwidth of the pump, supporting the feasibility of future experimental realisations.
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Here we demonstrate the efficient photon-pair generation via spontaneous parametric down conversion from a semiconductor metasurface supporting dual quasibound states in the continuum (quasi-BICs). In a simple metasurface composed of AlGaAs elliptical nanocyclinders, the two high-QQQ quasi-BIC resonances that coincide with the generated signal and idler frequencies significantly boost the local electric field. This leads to a substantial enhancement in the reverse classical nonlinear process of sum-frequency generation and subsequently the remarkably high generation rate of photon pairs under the quantum-classical correspondence principle. Within a narrowband wavelength regime around the quasi-BIC resonances, the rate of pair production is enhanced up to $\ensuremath{\sim}{10}^{4}$ Hz, two orders of magnitude larger than that in the Mie resonant AlGaAs nanoantennas. Moreover, the photon pair emission is mainly concentrated in the normal direction with respect to the metasurface, and shows a tunable rate with the QQQ factor by engineering the rotation angle of nanocylinders. The presented work enables nanoscale sources of high-quality entangled photons which will find applications in advanced quantum imaging and communications.
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spontaneous parametric down conversion from a metasurface supporting a quasi-bound state in the continuum (BIC) leading to remarkable emission directivities. The pair generation rate is enhanced 67 times compared to the case of an unpatterned film of the same thickness and material. At the wavelength of the quasi-BIC resonance, photons are mostly emitted backwards, while their partners, spectrally detuned by only 8 nm, are emitted forwards. This behavior demonstrates fine spectral splitting of entangled photons and their bi-directional emission, never before observed in nanoscale sources. We expect this work to be a starting point for the efficient demultiplexing of photons in nanoscale quantum optics.
All-dielectric optical metasurfaces are a workhorse in nano-optics due to both their ability to manipulate light in different degrees of freedom and their excellent performance at light frequency conversion. Here, we demonstrate first-time generation of photon pairs via spontaneous parametric-down conversion in lithium niobate quantum optical metasurfaces with electric and magnetic Mie-like resonances at various wavelengths. By engineering the quantum optical metasurface, we tailor the photon-pair spectrum in a controlled way. Within a narrow bandwidth around the resonance, the rate of pair production is enhanced up to two orders of magnitude compared to an unpatterned film of the same thickness and material. These results enable flat-optics sources of entangled photons -- a new promising platform for quantum optics experiments.