Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2609.06894

Pulse-by-pulse programmable synthesis of ultrafast optical waveforms

Shilong Liu, Gabriel Demontigny, Émile Dessureault, Stéphane Virally, Denis V. Seletskiy

physics.opticsnlin.PSquant-phSubmitted Sep 7, 2026• Announced Sep 8, 2026
arXivHTMLPDF

Abstract

Programmable control of individual pulses in a high-repetition-rate (typically MHz) ultrafast pulse train is a long-standing goal for optical arbitrary waveform synthesis. Here, we report a programmable pulse-by-pulse shaper that enables deterministic spectral-temporal control of ultrafast pulses at a repetition rate of $\sim$ 20~MHz. By synchronizing an FPGA-driven electro-optic modulation on the stretched waveform in a temporal 4$f$ shaping system, the regime writes pulse-index-dependent spectral phase profiles onto individual pulses. We demonstrate three levels of programmable ability: zero-order phase coding that maps pulse-by-pulse phase sequences into double-slit-like spectral-temporal interference; first-order phase programming that produces arbitrary temporal trajectories with deterministic delay; and fractional-order phase engineering that generates programmable temporal breathing. By launching the shaped pulse train into a nonlinear fiber stage, the programmed temporal breathing is converted into one spectral breathing. We further construct a phase-level-dependent regime map of nonlinear spectral breathing, revealing transitions from weak single-envelope breathing to multi-peak spectral splitting and strongly breathing merged-spectrum dynamics, in agreement with numerical simulations. This pulse-by-pulse spectral-temporal synthesis platform establishes pulse index as a programmable degree of freedom for ultrafast pulse shaping and provides a route toward real-time and pulse resolved optical arbitary waveform synthesis.

Comments
Comments and suggestions are welcome

Related papers

Quantum pulse shaping by direct temporal phase modulation

Laura Jayne Wright

Creating and controlling well-defined single-photon states is important for many quantum enhanced technologies. Information can be encoded in any degree of freedom associated with a single-photon field excitation, for example in the polarization or transverse spatial mode structure. The ability to encode multiple qubits in these states is desirable for high data transmission rates and increased information processing capacity. The spectral-temporal domain offers a large Hilbert space for encoding information, well suited to integrated optical architectures owing to the low cross-talk between channels. Indeed, time-frequency encoding is an integral component of existing information technologies infrastructure. Thus, complete, coherent control of the spectral-temporal mode structure of light is essential to advancing optical quantum technologies. Arbitrary control of single-photon states has been demonstrated in the polarization and spatial-momentum degrees of freedom however, is yet to be established in the spectral-temporal domain. Recently it was shown that spectral-temporal pulse shaping is experimentally feasible using nonlinear optical methods. However, such techniques can introduce noise photons, are challenging to implement deterministically and require specially prepared auxiliary pump pulses. Furthermore, they are typically only possible at relatively low repetition rates to avoid damage of nonlinear optical materials. Here, we demonstrate deterministic pulse shaping of single-photon wave packets by introducing a time-varying phase. Applying linear or quadratic phase to the wave packet introduces a spectral shift or spectral broadening, respectively. Achieving significant spectral manipulation requires temporal-phase modulation on the order of π. The phase must also vary on the same time scale as the optical pulses, approximately 1 ps in duration here. This relatively rapid phase variation is achieved using a fast electro-optic phase modulator. The modulator is driven by a time-varying voltage that is synchronized with a pulse train of single-photon wave packets for accurate temporal phase control. In this thesis, we experimentally demonstrate control of the spectral-temporal state of single-photon wave packets using this method. Heralded single-photon wave packets are generated by spontaneous parametric down conversion pumped by a frequency-doubled Titanium-Sapphire laser oscillator with 80 MHz repetition rate. To achieve significant modulation of single-photon pulses a 10 V peak-to-peak radio-frequency signal of 40 GHz drives the phase modulator, which requires approximately 3.6 V to achieve a π phase shift. The signal is synchronized with the oscillator pulse train using custom designed electronics. Details of these electronics are presented, resulting in a robust phase and amplitude controllable 40 GHz voltage source, phase locked to the single-photon pulse train. To demonstrate the utility of this pulse-shaping method we experimentally show spectral shearing of almost 1 nm for single-photon wave packets with 830 nm central wavelength and 1 nm bandwidth. Measurement of the second-order intensity correlation before and after the wave-packet manipulation remains constant within uncertainty of the measurement, showing that the quantum nature of the single-photon source is not deteriorated by the modulator. Preservation of the wave-packet coherence is verified by two-photon interference between spectrally sheared and non-modulated single-photons.

•Jan 1, 2015•1 citation

Electro-optic bandwidth manipulation of quantum light (Conference Presentation)

Michał Karpiński, Michał Jachura, Laura J. Wright +1 more

Spectral-temporal manipulation of optical pulses has enabled numerous developments within a broad range of research topics, ranging from fundamental science to practical applications. Within quantum optics spectral-temporal degree of freedom of light offers a promising platform for integrated photonic quantum information processing. An important challenge in experimentally realizing spectral-temporal manipulation of quantum states of light is the need for highly efficient manipulation tools. In this context the intrinsically deterministic electro-optic methods show great promise for quantum applications. We experimentally demonstrate application of electro-optic platform for spectral-temporal manipulation of ultrashort pulsed quantum light. Using techniques analogous to serrodyne frequency shifting we show active spectral translation of few-picosecond single photon pulses by up to 0.5 THz. By employing an approach based on an electro-optic time lens we demonstrate up to 6-fold spectral compression of heralded single photon pulses with efficiency that enables us to significantly increase single photon flux through a narrow bandpass filter. We realize the required temporal phase manipulation by driving a lithium niobate waveguided electrooptic modulator with 33 dBm sinusoidal RF field at the frequency of either 10 GHz or 40 GHz. We use a phase lock loop to temporally lock the RF field to the 80 MHz repetition rate of approximately 1 ps long optical pulses. Heralded single photon wavepackets are generated by means of spontaneous parametric down-conversion in potassium dihydrogen phosphate (KDP) crystal, which enables preparation of spectrally pure single photon wavepackets without the need for spectral filtering. Spectral shifting is achieved by locking single-photon pulses to the linear slope of sinusoidal 40 GHz RF phase modulation. We verify the spectral shift by performing spectrally resolved heralded single photon counting, using frequency-to-time conversion by means of a highly dispersive chirped fiber Bragg grating. We verify the non-classicality of spectrally shifted single photons by measuring high-visibility Hong-Ou-Mandel interference using a reference single photon pulse. Spectral compression is based on the time lens principle, which requires locking optical pulses to approximately quadratic region of sinusoidal phase modulation. We utilize both 10 GHz and 40 GHz RF driving frequencies. Bandwidth compression is achieved by chirping the single photon pulse using an appropriate length of single-mode fibre and subsequently subjecting it to the action of the time lens. We verify spectral compression directly using the aforementioned spectrally-resolved heralded single photon counting method. We achieve 3-fold spectral compression of 2 nm bandwidth single photon pulses using 40 GHZ modulation frequency, and 6-fold spectral compression of 0.9 nm bandwidth single photon pulses using 10 GHz modulation frequency. Overall transmission of our set-up exceeding 30% enables practical usability of our spectral compression method which we demonstrate experimentally by showing an increased photon flux through a narrowband filter. Our results present an important contribution towards implementing quantum information processing in the spectral-temporal degree of freedom of a photon. In the context of quantum networks they present an enabling tool towards efficient photonic interfacing of different quantum information processing platforms.

•Aug 3, 2016•0 citations

Sub-GHz resolution line-by-line pulse shaper for driving superconducting circuits

Dahyeon Lee, Takuma Nakamura, Andrew J. Metcalf +4 more

We demonstrate a sub-GHz resolution, fully programmable Fourier-domain pulse shaper capable of generating arbitrary optical pulse patterns for superconducting circuit platforms. This high resolution allows line-by-line pulse shaping of a 1 GHz-spaced comb, and the pulse shaper can accommodate an optical bandwidth as large as 1 THz, which represents the highest resolution programmable line-by-line pulse shaping to our knowledge. Linear optical sampling with a dual-comb system confirms independent control of 1 GHz-spaced optical lines, and the low phase noise of the pulse shaper is characterized. We apply the pulse shaper as an optical drive for an array of Josephson junctions operating at a temperature of 4 K, where cryogenic photodetection of pulse doublets with user-defined separation characterizes the Josephson junction response. Furthermore, we demonstrate a pulse-density modulation pattern of 4 ps duration optical pulses that can serve as the high bandwidth drive of a quantum-based Josephson arbitrary waveform synthesizer. By leveraging the exquisite control, large bandwidth, and low noise of photonics, this represents an important advance toward the realization of high power and high spectral purity AC voltage standards at gigahertz frequencies without requiring 100 GHz bandwidth driving electronics.

APL Photonics•Aug 1, 2023•11 citations

Programmable optical waveform reshaping on a picosecond timescale

Paritosh Manurkar, Nitin Jain, Prem Kumar +1 more

We experimentally demonstrate the temporal reshaping of optical waveforms in the telecom wavelength band using the principle of quantum frequency conversion. The reshaped optical pulses do not undergo any wavelength translation. The interaction takes place in a nonlinear chi((2)) waveguide using an appropriately designed pump pulse programmed via an optical waveform generator. We show the reshaping of a single-peak pulse into a double-peak pulse and vice versa. We also show that exponentially decaying pulses can be reshaped into a near Gaussian shape, and vice versa, which is a useful functionality for quantum communications. (C) 2017 Optical Society of America

•Jan 1, 2017•6 citations

Quantum arbitrary waveform generator

Kan Takase, Akito Kawasaki, Byung Kyu Jeong +13 more

Controlling the temporal waveform of light is the key to a versatile light source in classical and quantum electronics. Although pulse shaping of classical light is mature and has been used in various fields, more advanced applications would be realized by a light source that generates arbitrary quantum light with arbitrary temporal waveforms. We call such a device a quantum arbitrary waveform generator (Q-AWG). The Q-AWG must be able to handle various quantum states of light, which are fragile. Thus, the Q-AWG requires a radically different methodology from classical pulse shaping. Here, we invent an architecture of Q-AWGs that can operate semi-deterministically at a repetition rate over gigahertz in principle. We demonstrate its core technology via generating highly nonclassical states with temporal waveforms that have never been realized before. This result would lead to powerful quantum technologies based on Q-AWGs such as practical optical quantum computing.

arXiv:2205.13097•Science Advances•Oct 28, 2022•20 citations

Ultrafast manipulation of single photons using dispersion and sum-frequency generation

John M. Donohue

Single photons provide a natural platform for quantum communication and quantum networking, as they can be entangled in many degrees of freedom and maintain coherence over long-distance links. However, while their minimal interactions with the environment isolate them from detrimental noise, it can make them difficult to measure and manipulate. In particular, manipulation on the ultrafast timescale is necessary to fully exploit the energy-time (or spectral) photonic degree of freedom. Full control over the spectral properties of single photons is key to many quantum technologies and opens the door to natural high-dimensional quantum encodings. \n \nIn this thesis, we theoretically and experimentally examine the use of nonlinear optical processes mediated by strong laser pulses as a method to control the spectral properties of ultrafast single photons. By mixing single-photon pulses with strong escort pulses that have been shaped through dispersion in a nonlinear crystal, the shape of the escort is imprinted on the photon, resulting in a custom-tailored upconverted pulse. We theoretically examine this process for quadratic spectral phases and show that it has the potential to be simultaneously effective and efficient for the customization of single-photon spectral waveforms, and can be performed in an entanglement-conserving manner. \n \nWe then experimentally demonstrate the range of this technique through three applications. First, we show that sum-frequency generation with shaped pulses can be used to coherently measure time-bin encoded photons with bin separations on the order of picoseconds, well below the timing resolution of our detectors. Secondly, we show that this technique can be adapted to convert a train of pulses to a frequency comb, which can be read out in a straightforward manner using diffraction-based spectrometry. We also show here that this process can be performed in a polarization-maintaining fashion, and demonstrate that entanglement with a partner photon is conserved with high fidelity. Finally, we show that this process can be viewed as a time lens, which modulates a temporal waveform in an analogous fashion to a lens focusing a beam of light. We apply the time lens to a photon from an energy-time entangled pair, and show negative magnification of the joint spectrum through a reversal of the spectral correlations. Such processes could find application in quantum state engineering and high-speed single-photon measurement.

•Dec 1, 2016•0 citations
Programmable control of individual pulses in a high-repetition-rate (typically MHz) ultrafast pulse train is a long-standing goal for optical arbitrary waveform synthesis. Here, we report a programmable pulse-by-pulse shaper that enables deterministic spectral-temporal control of ultrafast pulses at a repetition rate of ∼\sim∼ 20~MHz. By synchronizing an FPGA-driven electro-optic modulation on the stretched waveform in a temporal 4fff shaping system, the regime writes pulse-index-dependent spectral phase profiles onto individual pulses. We demonstrate three levels of programmable ability: zero-order phase coding that maps pulse-by-pulse phase sequences into double-slit-like spectral-temporal interference; first-order phase programming that produces arbitrary temporal trajectories with deterministic delay; and fractional-order phase engineering that generates programmable temporal breathing. By launching the shaped pulse train into a nonlinear fiber stage, the programmed temporal breathing is converted into one spectral breathing. We further construct a phase-level-dependent regime map of nonlinear spectral breathing, revealing transitions from weak single-envelope breathing to multi-peak spectral splitting and strongly breathing merged-spectrum dynamics, in agreement with numerical simulations. This pulse-by-pulse spectral-temporal synthesis platform establishes pulse index as a programmable degree of freedom for ultrafast pulse shaping and provides a route toward real-time and pulse resolved optical arbitary waveform synthesis.
Creating and controlling well-defined single-photon states is important for many quantum enhanced technologies. Information can be encoded in any degree of freedom associated with a single-photon field excitation, for example in the polarization or transverse spatial mode structure. The ability to encode multiple qubits in these states is desirable for high data transmission rates and increased information processing capacity. The spectral-temporal domain offers a large Hilbert space for encoding information, well suited to integrated optical architectures owing to the low cross-talk between channels. Indeed, time-frequency encoding is an integral component of existing information technologies infrastructure. Thus, complete, coherent control of the spectral-temporal mode structure of light is essential to advancing optical quantum technologies. Arbitrary control of single-photon states has been demonstrated in the polarization and spatial-momentum degrees of freedom however, is yet to be established in the spectral-temporal domain. Recently it was shown that spectral-temporal pulse shaping is experimentally feasible using nonlinear optical methods. However, such techniques can introduce noise photons, are challenging to implement deterministically and require specially prepared auxiliary pump pulses. Furthermore, they are typically only possible at relatively low repetition rates to avoid damage of nonlinear optical materials. Here, we demonstrate deterministic pulse shaping of single-photon wave packets by introducing a time-varying phase. Applying linear or quadratic phase to the wave packet introduces a spectral shift or spectral broadening, respectively. Achieving significant spectral manipulation requires temporal-phase modulation on the order of π. The phase must also vary on the same time scale as the optical pulses, approximately 1 ps in duration here. This relatively rapid phase variation is achieved using a fast electro-optic phase modulator. The modulator is driven by a time-varying voltage that is synchronized with a pulse train of single-photon wave packets for accurate temporal phase control. In this thesis, we experimentally demonstrate control of the spectral-temporal state of single-photon wave packets using this method. Heralded single-photon wave packets are generated by spontaneous parametric down conversion pumped by a frequency-doubled Titanium-Sapphire laser oscillator with 80 MHz repetition rate. To achieve significant modulation of single-photon pulses a 10 V peak-to-peak radio-frequency signal of 40 GHz drives the phase modulator, which requires approximately 3.6 V to achieve a π phase shift. The signal is synchronized with the oscillator pulse train using custom designed electronics. Details of these electronics are presented, resulting in a robust phase and amplitude controllable 40 GHz voltage source, phase locked to the single-photon pulse train. To demonstrate the utility of this pulse-shaping method we experimentally show spectral shearing of almost 1 nm for single-photon wave packets with 830 nm central wavelength and 1 nm bandwidth. Measurement of the second-order intensity correlation before and after the wave-packet manipulation remains constant within uncertainty of the measurement, showing that the quantum nature of the single-photon source is not deteriorated by the modulator. Preservation of the wave-packet coherence is verified by two-photon interference between spectrally sheared and non-modulated single-photons.
Spectral-temporal manipulation of optical pulses has enabled numerous developments within a broad range of research topics, ranging from fundamental science to practical applications. Within quantum optics spectral-temporal degree of freedom of light offers a promising platform for integrated photonic quantum information processing. An important challenge in experimentally realizing spectral-temporal manipulation of quantum states of light is the need for highly efficient manipulation tools. In this context the intrinsically deterministic electro-optic methods show great promise for quantum applications. We experimentally demonstrate application of electro-optic platform for spectral-temporal manipulation of ultrashort pulsed quantum light. Using techniques analogous to serrodyne frequency shifting we show active spectral translation of few-picosecond single photon pulses by up to 0.5 THz. By employing an approach based on an electro-optic time lens we demonstrate up to 6-fold spectral compression of heralded single photon pulses with efficiency that enables us to significantly increase single photon flux through a narrow bandpass filter. We realize the required temporal phase manipulation by driving a lithium niobate waveguided electrooptic modulator with 33 dBm sinusoidal RF field at the frequency of either 10 GHz or 40 GHz. We use a phase lock loop to temporally lock the RF field to the 80 MHz repetition rate of approximately 1 ps long optical pulses. Heralded single photon wavepackets are generated by means of spontaneous parametric down-conversion in potassium dihydrogen phosphate (KDP) crystal, which enables preparation of spectrally pure single photon wavepackets without the need for spectral filtering. Spectral shifting is achieved by locking single-photon pulses to the linear slope of sinusoidal 40 GHz RF phase modulation. We verify the spectral shift by performing spectrally resolved heralded single photon counting, using frequency-to-time conversion by means of a highly dispersive chirped fiber Bragg grating. We verify the non-classicality of spectrally shifted single photons by measuring high-visibility Hong-Ou-Mandel interference using a reference single photon pulse. Spectral compression is based on the time lens principle, which requires locking optical pulses to approximately quadratic region of sinusoidal phase modulation. We utilize both 10 GHz and 40 GHz RF driving frequencies. Bandwidth compression is achieved by chirping the single photon pulse using an appropriate length of single-mode fibre and subsequently subjecting it to the action of the time lens. We verify spectral compression directly using the aforementioned spectrally-resolved heralded single photon counting method. We achieve 3-fold spectral compression of 2 nm bandwidth single photon pulses using 40 GHZ modulation frequency, and 6-fold spectral compression of 0.9 nm bandwidth single photon pulses using 10 GHz modulation frequency. Overall transmission of our set-up exceeding 30% enables practical usability of our spectral compression method which we demonstrate experimentally by showing an increased photon flux through a narrowband filter. Our results present an important contribution towards implementing quantum information processing in the spectral-temporal degree of freedom of a photon. In the context of quantum networks they present an enabling tool towards efficient photonic interfacing of different quantum information processing platforms.
We demonstrate a sub-GHz resolution, fully programmable Fourier-domain pulse shaper capable of generating arbitrary optical pulse patterns for superconducting circuit platforms. This high resolution allows line-by-line pulse shaping of a 1 GHz-spaced comb, and the pulse shaper can accommodate an optical bandwidth as large as 1 THz, which represents the highest resolution programmable line-by-line pulse shaping to our knowledge. Linear optical sampling with a dual-comb system confirms independent control of 1 GHz-spaced optical lines, and the low phase noise of the pulse shaper is characterized. We apply the pulse shaper as an optical drive for an array of Josephson junctions operating at a temperature of 4 K, where cryogenic photodetection of pulse doublets with user-defined separation characterizes the Josephson junction response. Furthermore, we demonstrate a pulse-density modulation pattern of 4 ps duration optical pulses that can serve as the high bandwidth drive of a quantum-based Josephson arbitrary waveform synthesizer. By leveraging the exquisite control, large bandwidth, and low noise of photonics, this represents an important advance toward the realization of high power and high spectral purity AC voltage standards at gigahertz frequencies without requiring 100 GHz bandwidth driving electronics.
We experimentally demonstrate the temporal reshaping of optical waveforms in the telecom wavelength band using the principle of quantum frequency conversion. The reshaped optical pulses do not undergo any wavelength translation. The interaction takes place in a nonlinear chi((2)) waveguide using an appropriately designed pump pulse programmed via an optical waveform generator. We show the reshaping of a single-peak pulse into a double-peak pulse and vice versa. We also show that exponentially decaying pulses can be reshaped into a near Gaussian shape, and vice versa, which is a useful functionality for quantum communications. (C) 2017 Optical Society of America
Controlling the temporal waveform of light is the key to a versatile light source in classical and quantum electronics. Although pulse shaping of classical light is mature and has been used in various fields, more advanced applications would be realized by a light source that generates arbitrary quantum light with arbitrary temporal waveforms. We call such a device a quantum arbitrary waveform generator (Q-AWG). The Q-AWG must be able to handle various quantum states of light, which are fragile. Thus, the Q-AWG requires a radically different methodology from classical pulse shaping. Here, we invent an architecture of Q-AWGs that can operate semi-deterministically at a repetition rate over gigahertz in principle. We demonstrate its core technology via generating highly nonclassical states with temporal waveforms that have never been realized before. This result would lead to powerful quantum technologies based on Q-AWGs such as practical optical quantum computing.
Single photons provide a natural platform for quantum communication and quantum networking, as they can be entangled in many degrees of freedom and maintain coherence over long-distance links. However, while their minimal interactions with the environment isolate them from detrimental noise, it can make them difficult to measure and manipulate. In particular, manipulation on the ultrafast timescale is necessary to fully exploit the energy-time (or spectral) photonic degree of freedom. Full control over the spectral properties of single photons is key to many quantum technologies and opens the door to natural high-dimensional quantum encodings. \n \nIn this thesis, we theoretically and experimentally examine the use of nonlinear optical processes mediated by strong laser pulses as a method to control the spectral properties of ultrafast single photons. By mixing single-photon pulses with strong escort pulses that have been shaped through dispersion in a nonlinear crystal, the shape of the escort is imprinted on the photon, resulting in a custom-tailored upconverted pulse. We theoretically examine this process for quadratic spectral phases and show that it has the potential to be simultaneously effective and efficient for the customization of single-photon spectral waveforms, and can be performed in an entanglement-conserving manner. \n \nWe then experimentally demonstrate the range of this technique through three applications. First, we show that sum-frequency generation with shaped pulses can be used to coherently measure time-bin encoded photons with bin separations on the order of picoseconds, well below the timing resolution of our detectors. Secondly, we show that this technique can be adapted to convert a train of pulses to a frequency comb, which can be read out in a straightforward manner using diffraction-based spectrometry. We also show here that this process can be performed in a polarization-maintaining fashion, and demonstrate that entanglement with a partner photon is conserved with high fidelity. Finally, we show that this process can be viewed as a time lens, which modulates a temporal waveform in an analogous fashion to a lens focusing a beam of light. We apply the time lens to a photon from an energy-time entangled pair, and show negative magnification of the joint spectrum through a reversal of the spectral correlations. Such processes could find application in quantum state engineering and high-speed single-photon measurement.