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arXiv:2609.01157

A continuous-mode quantum-optical representation of finite strong-field laser pulses in free space

Szabolcs Hack, Attila Czirják, Péter Földi

quant-phSubmitted Sep 1, 2026• Announced Sep 2, 2026• 0 citations
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Abstract

We formulate an energy-consistent quantum-optical representation of finite paraxial laser pulses in free space. The formulation is based on a continuous-mode description and provides a step toward a unified treatment of coherent and nonclassical strong-field drivers. Starting from plane-wave quantization, we construct a transverse vector-mode reduction in which the selected mode can reproduce an arbitrary normalized spatial--polarization profile. For a coherent pulse, the measured pulse energy and full laboratory analytic signal determine the frequency-dependent coherent-state displacement $(α(ω))$, without introducing a physical quantization volume. For nonclassical pulses, the same first-order field data and total energy do not uniquely specify the quantum state. Additional correlation information or model assumptions are required. We incorporate this information through normal and anomalous covariance kernels and discuss $g^{(2)}$-based diagnostics of squeezed pulses. We also derive a phase-sensitive convergence criterion for numerical frequency-bin discretizations. An exactly solvable continuum-mode free-electron application shows that the coherent displacement reproduces the semiclassical mean trajectory, whereas the field covariances determine the electron wave packet width. The framework offers a convenient, energy-consistent interface between measured free-space pulses and quantum-optical calculations.

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We formulate an energy-consistent quantum-optical representation of finite paraxial laser pulses in free space. The formulation is based on a continuous-mode description and provides a step toward a unified treatment of coherent and nonclassical strong-field drivers. Starting from plane-wave quantization, we construct a transverse vector-mode reduction in which the selected mode can reproduce an arbitrary normalized spatial--polarization profile. For a coherent pulse, the measured pulse energy and full laboratory analytic signal determine the frequency-dependent coherent-state displacement (α(ω))(α(ω))(α(ω)), without introducing a physical quantization volume. For nonclassical pulses, the same first-order field data and total energy do not uniquely specify the quantum state. Additional correlation information or model assumptions are required. We incorporate this information through normal and anomalous covariance kernels and discuss g(2)g^{(2)}g(2)-based diagnostics of squeezed pulses. We also derive a phase-sensitive convergence criterion for numerical frequency-bin discretizations. An exactly solvable continuum-mode free-electron application shows that the coherent displacement reproduces the semiclassical mean trajectory, whereas the field covariances determine the electron wave packet width. The framework offers a convenient, energy-consistent interface between measured free-space pulses and quantum-optical calculations.
We formulate the quantum theory of optical wave propagation without recourse to cavity quantization. This approach avoids the introduction of a box-related mode spacing and enables us to use a continuum frequency space description. We introduce a complete orthonormal set of operators that can describe states of finite energy. The set is countable and the operators have all the usual properties of the single-mode frequency operators. With use of these operators a generalization of the single-mode normal-ordering theorem is proved. We discuss the inclusion of material dispersion and pulse propagation in an optical fiber. Finally, we consider the process of photodetection in free space, concluding with a discussion of homodyne detection with both local oscillator and signal fields pulsed.
Space-time description of pulsed laser radiation by means of coherent states is presented. The corresponding displacement operator contains space dependent annihilation and creation operators, not the "standard" operators corresponding to mode decomposition of the electromagnetic field. This allowed for a direct description of space and time dependence of the electromagnetic field of the pulse. The main characteristics of the pulse is its profile in the wave-vector space. It determines space-time structure of expectation values of the electromagnetic field carried by the pulse, and the distribution of photon modes as well. Determination of the latter required transition from the space-time, or field description to the photon mode approach. Expectation values of the electric field of a Gaussian pulse propagating in the z-direction and linearly polarized in the x-direction are presented graphically in the form of contour plots in the x-z plane. Apart of the dominant x-component electric field has a small longitudinal component in the z-direction. The dominant component of the magnetic field in the y-direction is acompannied by small components in z- and x-directions. The plane wave limit of the pulse can be implemented by shrinking transverse width of the profile to zero (transverse spatial extension goes to infinity), while keeping the photon density constant. One can then retrieve standard plane wave form of the pulse also in the dipole approximation.
We develop a theoretical framework for high-harmonic generation (HHG) driven by quantum states of light based on a temporal-mode expansion of the electromagnetic field. This approach extends previous single plane-wave mode treatments to realistic pulse configurations and arbitrary multi-mode states of light, resolving conceptual inconsistencies arising from non-normalizable infinite plane waves and establishing consistency between analytical and numerical methods. We derive a correction factor that quantifies deviations from the diagonal approximation (in which the yield becomes a statistical average over classical-field simulations) both for the response of a single atom and in the many-atom regime. Our results confirms that the HHG spectrum for atoms driven by any quantum state of light in free space is accurately described by averaging semi-classical calculations over the Husimi distribution, with no observable genuine quantum effects in the spectrum. We also demonstrate that in the many-atom regime, the mean-field coherent-state approximation underlying this treatment does not preserve probabilities, although unitarity is restored by in the diagonal approximation. The absence of genuine quantum effects in the HHG yield is attributed to the large photon numbers (∼1011\sim 10^{11}∼1011) required to reach HHG intensities in free space, which render quantum fluctuations negligible. We discuss nanophotonic environments with ultrasmall mode volumes as potential platforms where few-photon strong-field processes could exhibit genuine quantum signatures.
Understanding quantum system dynamics driven by nonclassical light pulses is challenging, particularly for general light states with large photon numbers. Here we introduce an efficient framework that makes this task tractable. By introducing a pulse-shaped P-representation, the exact quantum evolution is decomposed into a mixture of many independent quasi-classical branches, each governed by a standard master equation with a classical pulse which can be solved efficiently. As an illustration, for a two-level system interacting with an exponential pulse, we first find out the exact analytical solutions to the Bloch equations in each quasi-classical branch, and then by taking proper P-function average over all branches, the full system dynamics driven by nonclassical light pulses is analytically obtained. For the one-photon and two-photon cases, our method well reproduces the previous exact results either analytically or numerically. Crucially, our approach scales efficiently to more complex light states (Fock, thermal, squeezed vacuum states) with large photon numbers (N∼100N\sim 100N∼100). We further provide a clear physical interpretation how the system dynamics is influenced through the high-order optical coherence of the nonclassical pulses. This work provides a unified and computationally efficient route and a useful starting point to explore more complex quantum dynamics driven by nonclassical light in quantum optics and quantum information processing.
Abstract Bright squeezed vacuum (BSV) has emerged as a macroscopic nonclassical light source capable of driving strong-field processes. Yet its broad, long-tailed photon-number distribution bears little resemblance to the narrow poissonian distribution of a coherent field, obscuring how the corresponding strong-field responses are connected. We show that field-quadrature space supplies the missing continuous description: coherent, squeezed coherent, and BSV states are Gaussian wave packets distinguished only by their centers and widths. This representation provides a unified framework for tracing the coherent-to-BSV transition at fixed mean photon number and for analyzing both ionization yields and photoelectron spectra. Crucially, BSV is a symmetry-protected endpoint in quadrature space. Near the BSV limit, we identify a simple scaling law of the ionization response associated with a residual coherent component. We show that this scaling arises from parity-induced stationarity with respect to the Gaussian center, together with the accompanying width variation near the BSV limit. The result provides a symmetry-based criterion for approaching the BSV regime and a potential probe of a mode-matched coherent displacement through the strong-field response itself.
We investigate the dynamics of a charged particle interacting with a multimode quantized electromagnetic field and obtain an analytic solution for the full electron--field system. This framework enables the calculation of position expectation values and uncertainties for arbitrary wave packets and field states, allowing us to identify quantum corrections to the corresponding classical motion. While the corrections to the position expectation value are weak and largely insensitive to the quantum state of the field, the wave packet broadening exhibits a pronounced dependence on the field state. In particular, the quantum uncertainty of the radiation is directly imprinted onto the spatial uncertainty of the particle. We illustrate these effects for Gaussian wave packets interacting with coherent, Fock, and squeezed states, including bright squeezed vacuum. The interaction with a finite-duration laser pulse is also analyzed as a multimode example. Our results provide a transparent analytic route toward understanding how quantum fluctuations of light influence electron dynamics in strong-field settings.