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arXiv:2608.30276

Efficient biphoton generation by a waveguide-coupled single atom

Mao-Hua Wang, Xiao-Jun Zhang, M. Artoni, G. C. La Rocca, Jin-Hui Wu

quant-phSubmitted Aug 31, 2026• Announced Sep 1, 2026• 0 citations
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Abstract

A single atom undergoing spontaneous four-wave mixing near a chiral waveguide can efficiently channel an emitted Stokes-anti-Stokes photon pair into two tightly confined waveguide modes, yielding thus enhanced biphoton generation without requiring loss suppression or stringent phase matching. We develop a perturbative treatment, valid for a four-level atomic system under experimentally realistic conditions, to explain physical origins and clarify relevant constraints of such an enhancement determined by the interplay of atomic decay rates toward guided and unguided modes. Besides achieving optimal generation rates equivalent to a cold atomic ensemble hundreds of micrometers long in free space, our biphoton source naturally fulfills key requirements for next-generation on-chip quantum light sources, namely low-loss operation, robustness, compactness, and scalability.

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European Quantum Electronics Conference (EQEC)•Jun 21, 2015•0 citations
A single atom undergoing spontaneous four-wave mixing near a chiral waveguide can efficiently channel an emitted Stokes-anti-Stokes photon pair into two tightly confined waveguide modes, yielding thus enhanced biphoton generation without requiring loss suppression or stringent phase matching. We develop a perturbative treatment, valid for a four-level atomic system under experimentally realistic conditions, to explain physical origins and clarify relevant constraints of such an enhancement determined by the interplay of atomic decay rates toward guided and unguided modes. Besides achieving optimal generation rates equivalent to a cold atomic ensemble hundreds of micrometers long in free space, our biphoton source naturally fulfills key requirements for next-generation on-chip quantum light sources, namely low-loss operation, robustness, compactness, and scalability.
In this paper we study the generation of photon pairs through the process of spontaneous four wave mixing (SFWM) in a χ (3) cavity. Our key interest is the generation of photon pairs in a guided-wave configuration—fiber or waveguide—where at least one of the photons in a given pair is matched in frequency and bandwidth to a particular atomic transition, as required for the implementation of photon–atom interfaces. We present expressions, along with plots, for the two-photon joint intensity both in the spectral and temporal domains. We also present expressions for the absolute brightness, along with numerical simulations, and show that the presence of the cavity can result in a flux enhancement relative to an equivalent source without a cavity.
The pairing ratio, a crucial metric assessing a biphoton source's ability to generate correlated photon pairs, remains underexplored despite theoretical predictions. This study presents experimental findings on the pairing ratio, utilizing a double- Λ spontaneous four-wave mixing biphoton source in cold atoms. At an optical depth (OD) of 20, we achieved an ultrahigh biphoton generation rate of up to 1.3 × 10 7 per second, with a successful pairing ratio of 61%. Increasing the OD to 120 significantly improved the pairing ratio to 89%, while maintaining a consistent biphoton generation rate. This achievement, marked by high generation rates and robust biphoton pairing, holds great promise for advancing efficiency in quantum communication and information processing. Additionally, in a scenario with a lower biphoton generation rate of 5.0 × 10 4 per second, we attained an impressive signal-to-background ratio of 241 for the biphoton wavepacket, surpassing the Cauchy-Schwarz criterion by approximately 1.5 × 10 4 times. Published by the American Physical Society 2024
Third-order nonlinear processes require phase matching between the interacting fields to achieve high efficiencies. Typically in guided-wave χ(3)χ^{(3)}χ(3) platforms this is achieved by engineering the dispersion of the modes through the transverse profile of the device. However, this limits the flexibility of the phase matching that can be achieved. Instead, we analyze four-wave mixing in a pair of asymmetric waveguides and show that phasematching may be achieved in any χ(3)χ^{(3)}χ(3) waveguide by coupling of a nondegenerate pump from an adjacent waveguide. We demonstrate the additional flexibility that this approach yields in the case of photon-pair generation by spontaneous FWM, where the supermode dispersion may be modified to produce pure heralded single photons -- a critical capability required for example by silicon platforms for chip-scale quantum photonics.
We theoretically investigate the coherent manipulation of biphoton generation via spontaneous four-wave mixing in a cavity-QED system with a single atom. The atom is driven by pumping, coupling, and driving fields, and the generation of the Stokes and anti-Stokes photons are enhanced by two cavities. By solving the master equation in the steady state, we analyze the spectral brightness, as well as the degree of the auto-correlation and cross-correlation. Our results show that when the pumping and driving fields are in two-photon resonance, the dark state established between the ground and Rydberg states. efficiently enhances the controllability of the driving field over the biphoton generation and the quantum statistics. In contrast, under large two-photon detuning, the control capability of the driving field is significantly reduced. The coupling field, which directly relates to the electromagnetically induced transparency, modifies the linewidth of the biphoton, while the atom-cavity coupling strength only changes the brightness without affecting the linewidth.
Heralded single photon sources, based on probabilistic non-linear interactions, currently serve as the de-facto standard for performing multi-photon quantum interference experiments. Already, interesting phenomena may be explored with a handful of such sources [1], whilst in the future, large arrays of identical sources could be multiplexed with a switching network to achieve a truly scalable, near-deterministic emission [2]. However, fabricating such a large number of indistinguishable, pure, heralded single photon sources, operating with low-loss, remains an open challenge. Spontaneous four-wave mixing (SFWM) in a silica waveguide is a promising route to building such a source. The low-loss and excellent mode-matching to optical fibre of silica waveguides allows high preparation efficiency. Guided-wave photonics also allows the precise control of the optical modes needed to engineer emission of photons into a single pair of Schmidt modes: allowing heralded photons of high purity without narrowband filtering [3].