Mechanical resonators ultrastrongly coupled to quantum two-level systems provide a promising route towards mechanical qubits by introducing significant anharmonicity to the mechanical modes, particularly in the slow-oscillator regime. Although the resulting hybrid system is well described by the quantum Rabi model, a consistent treatment of dissipation remains challenging across the broad parameter space routinely probed in current nanotube electromechanical devices. Here, we investigate dissipation in the open quantum Rabi model using a Born-Markov framework based on the slowly varying bath spectrum approximation, yielding a Lindblad master equation applicable far beyond conventional descriptions while recovering them in their respective limits. Using this framework, we analyze experimentally accessible observables across this parameter space. As the secular approximation breaks down, phonon blockade progressively washes out. Our approach remains valid in this regime, enabling a quantitative description of the continuous evolution of phonon blockade with coupling strength and dissipation. At finite temperature, we find a suppression of the temperature-induced increase of coherence decay rate for weak anharmonicity. Under driving, our approach remains applicable to substantially stronger perturbations than conventional dressed-state master equations and shows that an apparently classical observable can coexist with Wigner negativity. We further capture the weakly anharmonic regime arising from finite detuning in the double-quantum dot. These results establish a unified description of dissipation from weakly anharmonic operating regimes to the strongly anharmonic mechanical-qubit regime and provide experimentally relevant predictions for ultrastrong electromechanical systems.
Mechanical resonators ultrastrongly coupled to quantum two-level systems provide a promising route towards mechanical qubits by introducing significant anharmonicity to the mechanical modes, particularly in the slow-oscillator regime. Although the resulting hybrid system is well described by the quantum Rabi model, a consistent treatment of dissipation remains challenging across the broad parameter space routinely probed in current nanotube electromechanical devices. Here, we investigate dissipation in the open quantum Rabi model using a Born-Markov framework based on the slowly varying bath spectrum approximation, yielding a Lindblad master equation applicable far beyond conventional descriptions while recovering them in their respective limits. Using this framework, we analyze experimentally accessible observables across this parameter space. As the secular approximation breaks down, phonon blockade progressively washes out. Our approach remains valid in this regime, enabling a quantitative description of the continuous evolution of phonon blockade with coupling strength and dissipation. At finite temperature, we find a suppression of the temperature-induced increase of coherence decay rate for weak anharmonicity. Under driving, our approach remains applicable to substantially stronger perturbations than conventional dressed-state master equations and shows that an apparently classical observable can coexist with Wigner negativity. We further capture the weakly anharmonic regime arising from finite detuning in the double-quantum dot. These results establish a unified description of dissipation from weakly anharmonic operating regimes to the strongly anharmonic mechanical-qubit regime and provide experimentally relevant predictions for ultrastrong electromechanical systems.
The interaction among the components of a hybrid quantum system is often neglected when considering the coupling of these components to an environment. However, if the interaction strength is large, this approximation leads to unphysical predictions, as has been shown for cavity-QED and optomechanical systems in the ultrastrong-coupling regime. To deal with these cases, master equations with dissipators retaining the interaction between these components have been derived for the quantum Rabi model and for the standard optomechanical Hamiltonian. In this article, we go beyond these previous derivations and present a general master equation approach for arbitrary hybrid quantum systems interacting with thermal reservoirs. Specifically, our approach can be applied to describe the dynamics of open hybrid systems with harmonic, quasiharmonic, and anharmonic transitions. We apply our approach to study the influence of temperature on multiphoton vacuum Rabi oscillations in circuit QED. We also analyze the influence of temperature on the conversion of mechanical energy into photon pairs in an optomechanical system, which has been recently described at zero temperature. We compare our results with previous approaches, finding that these sometimes overestimate decoherence rates and underestimate excited-state populations.
Abstract The standard weak-coupling approximations associated to open quantum systems have been extensively used in the description of a two-level quantum system, qubit, subjected to relatively weak dissipation compared with the qubit frequency. However, recent progress in the experimental implementations of controlled quantum systems with increased levels of on-demand engineered dissipation has motivated precision studies in parameter regimes that question the validity of the approximations, especially in the presence of time-dependent drive fields. In this paper, we address the precision of weak-coupling approximations by studying a driven qubit through the numerically exact and non-perturbative method known as the stochastic Liouville–von Neumann equation with dissipation. By considering weak drive fields and a cold Ohmic environment with a high cutoff frequency, we use the Markovian Lindblad master equation as a point of comparison for the SLED method and study the influence of the bath-induced energy shift on the qubit dynamics. We also propose a metric that may be used in experiments to map the regime of validity of the Lindblad equation in predicting the steady state of the driven qubit. In addition, we study signatures of the well-known Mollow triplet and observe its meltdown owing to dissipation in an experimentally feasible parameter regime of circuit electrodynamics. Besides shedding light on the practical limitations of the Lindblad equation, we expect our results to inspire future experimental research on engineered open quantum systems, the accurate modeling of which may benefit from non-perturbative methods.
Recent progress in the experimental implementations of controlled quantum systems and especially of tunable dissipation for them provides an ideal starting point for precision studies of open quantum systems and their models. However, typically the standard weak-coupling approximations are very accurate in describing the dynamics of the simplest and most easily experimentally approachable system, the qubit, since it is challenging to engineer dissipation that is strong relative to the qubit frequency while preserving a high level of control. In this paper, we propose to overcome such challenges by studying a driven qubit, for which the weak-coupling approaches may fail at dissipation rates comparable to the Rabi frequency of the drive which is typically much lower than the qubit frequency. Consequently, we observe such failure of the temporally local Lindblad master equation, the induced dynamics of which are compared with a numerically exact method. To this end, we propose a metric that may be used in experiments to verify our predictions. In addition, we study the well-known Mollow triplet and observe its meltdown owing to dissipation in an experimentally feasible parameter regime. Thus we expect our results to inspire future experimental research on open quantum systems and expand the understanding on this intriguing field of physics.
The model of a two-level system (TLS) coupled to a harmonic oscillator has found a widespread application in physics and chemistry. In this thesis we focus on the field of circuit quantum electrodynamics where the TLS stands for a quantum bit (qubit), which is the basic building unit of a potential quantum computer, and the oscillator represents a transmission-line resonator, which can be used, e.g., to store information contained on the qubit or for communication between several qubits. Furthermore, the oscillator can model a superconducting quantum interference device (SQUID) determining the state of the qubit. In first experimental realizations the coupling between the qubit and the oscillator was small compared to characteristic frequencies of the two devices. In such a situation the Jaynes-Cummings model provides a realistic and completely analytical description of the energy spectrum and the dynamics of the setup. However, it relies on a rotating-wave approximation (RWA) which neglects counter-rotating terms in the full qubit-oscillator Hamiltonian. These counter-rotating terms become important under increase of the coupling strength, as it has been achieved in recent experiments. We present two analytical approaches to take these additional contributions into account: The first one treats the qubit-oscillator Hamiltonian perturbatively in the coupling strength and predicts a frequency shift in its energy spectrum, the Bloch-Siegert shift. The second one considers the qubit's tunneling splitting as small parameter and thus treats the problem to all orders in the coupling allowing to enter the ultrastrong coupling regime, where the coupling strength becomes comparable to the qubit's and/or oscillator's frequency. For both cases we give a thorough analysis of the qubit's dynamics. In order to perform operations the qubit is usually probed by an external driving force. We model this situation by coupling the TLS to a classical oscillator and examine the resulting time dependent Hamiltonian using a combination of Floquet theory and Van Vleck perturbation theory. Thus, we provide an analysis of the qubit's energy spectrum and dynamics which is nonperturbative in the driving amplitude. We investigate effects like coherent destruction of tunneling and driving-inducing tunneling oscillations. By coupling the driven TLS to a quantized oscillator we give for the first time an analytical treatment of the qubit-oscillator system being simultaneously exposed to both ultrastrong coupling and extreme driving. We observe interesting phenomena in the dynamics like the suppression of specific frequencies under a variation of the coupling strength. To mimic environmental influences on the qubit we apply the Caldeira-Leggett master equation approach to the driven TLS and to the qubit-oscillator system and provide for both cases analytical expressions for the relaxation and dephasing rates.
Strong periodic driving of cavity-quantum electrodynamics (QED) in the ultrastrong-coupling regime creates nonequilibrium states whose dissipation is governed by Floquet quasienergies rather than undriven dressed resonances. However, modeling such a regime is a significant theoretical challenge, including a number of subtle problems such as the need to ensure gauge invariance for truncated matter-cavity systems with time-dependent driving. To fill this theoretical gap, we introduce a nonsecular Floquet generalized master equation framework for strongly driven open cavity-QED systems, formulated in the dressed basis of the quantum Rabi model and applicable to structured reservoirs without rotating-wave approximations. Our theory can thus model Floquet-driven dynamics in open ultrastrong-coupling cavity-QED, and demonstrates a wide range of quantum state control. Using strong optical pumping and parametric mechanical modulation, we compute long-time populations, fluorescence spectra, and the Floquet-Liouville eigenspectra, resolving observable resonances into hybridized quasienergy channels and decay rates. By systematically comparing with conventional time-independent dressed-basis generalized master equations, we show that static approaches only reproduce steady-state populations in restricted excitation regimes, and fail for frequency-resolved observables and break down under appropriate Floquet engineering, surprisingly, even for spectrally flat baths. Structured environments, such as Lorentzian-Ohmic reservoirs, further amplify these discrepancies through sideband-selective decay. Our results demonstrate that dissipation in driven ultrastrong cavity-QED is intrinsically quasienergy resolved and we establish Floquet-dissipative theory as an accurate and powerful framework for predicting spectra, controlling decay pathways, and engineering nonequilibrium quantum states and reservoirs.
We consider the quantum Rabi model as an open system that is subject to dissipation, dephasing, and sinusoidal qubit driving. One can change to an interaction picture where the qubit-driving term disappears at the expense of changing the free energy of the qubit which becomes time dependent. If the driving frequency is large with respect to the rest of the parameters with the exception of the driving strength, then one can obtain an effective Hamiltonian that accurately describes the dynamics of the system. The driving has two effects: the qubit-transition frequency is changed and the qubit has reduced dephasing. The driving strength can be chosen so that the qubit-transition frequency is reduced, made equal to zero, or even made negative so that the excited and ground states of the qubit are interchanged. Therefore, sinusoidal qubit driving offers another method to control the qubit-transition frequency and to reduce qubit dephasing. Adjusting the driving strength allows one to consider a qubit with degenerate energy levels. Not taking dissipation into account, the evolution operator of the qubit-harmonic oscillator system is given by a linear combination of the orthogonal projectors onto the eigenstates of ${\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\sigma}}}_{x}$ followed by the evolution operator of a forced harmonic oscillator, the harmonic oscillator can be prepared in such a way that it is always found in a Schr\"odinger cat state, and the transition probability of the qubit can exhibit a collapse-revival behavior. In addition, the Born-Markov-secular master equation is deduced and the effects of dissipation are presented. In particular, smaller ultrastrong-coupling values are preferable over larger ultrastrong-coupling values and deep strong-coupling values in order to have long-lived, easily distinguishable Schr\"odinger cat states because the decoherence rate is inversely proportional to the square of the coupling. Finally, the qubit-harmonic oscillator system can be prepared in highly entangled states that are stable under dissipation.