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arXiv:2608.25534

A universal loss-limited optimum for fixed multi-pass quantum sensing per absorbed photon

Christoph F. Wildfeuer

quant-phSubmitted Aug 26, 2026• Announced Aug 27, 2026• 0 citations
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Abstract

Multi-pass schemes send a photon through a sample several times to learn more about it. When the sample rather than the light is scarce, the natural figure of merit is the information gained per photon the object absorbs. We show that one constant fixes the loss-limited optimum of every fixed scheme in which a single photon passes repeatedly through the sample and is detected once at the end. Three properties suffice: information that grows as the square of the pass number, a fixed survival probability per pass, and no dose from a photon already lost. They force a single trade-off function $h(x)=x^2/(e^x-1)$, where $x$ is the number of passes times the loss per pass. Its maximum, 0.648, sits at $x_{\mathrm{opt}}=1.594$. The loss-limited ceiling of interaction-free interrogation and the multi-pass phase optimum of Yu et al. are two instances. Phase sensing of a weakly absorbing object is a third, optimal at $m_{\mathrm{opt}}=x_{\mathrm{opt}}/(ε+α)$ passes; the absorption $α$ and the parasitic loss $ε$ enter the optimum only through their sum, but the damage counts only $α$. N00N states and their loss-robust generalisations do worse per absorbed photon, and optimising over photon number and pass number together returns a single recycled photon. Two further problems are priced in the same measure. Absorption estimation gains nothing, for any scheme. Detecting a faint companion below the Rayleigh limit costs the companion a dose that does not depend on its faintness, while under direct imaging the dose grows without bound. For a fragile sample the gentlest measurement is also the simplest one: a single photon, recycled.

Comments
8 pages, 2 figures, one table

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Multi-pass schemes send a photon through a sample several times to learn more about it. When the sample rather than the light is scarce, the natural figure of merit is the information gained per photon the object absorbs. We show that one constant fixes the loss-limited optimum of every fixed scheme in which a single photon passes repeatedly through the sample and is detected once at the end. Three properties suffice: information that grows as the square of the pass number, a fixed survival probability per pass, and no dose from a photon already lost. They force a single trade-off function h(x)=x2/(ex−1)h(x)=x^2/(e^x-1)h(x)=x2/(ex−1), where xxx is the number of passes times the loss per pass. Its maximum, 0.648, sits at xopt=1.594x_{\mathrm{opt}}=1.594xopt​=1.594. The loss-limited ceiling of interaction-free interrogation and the multi-pass phase optimum of Yu et al. are two instances. Phase sensing of a weakly absorbing object is a third, optimal at mopt=xopt/(ε+α)m_{\mathrm{opt}}=x_{\mathrm{opt}}/(ε+α)mopt​=xopt​/(ε+α) passes; the absorption ααα and the parasitic loss εεε enter the optimum only through their sum, but the damage counts only ααα. N00N states and their loss-robust generalisations do worse per absorbed photon, and optimising over photon number and pass number together returns a single recycled photon. Two further problems are priced in the same measure. Absorption estimation gains nothing, for any scheme. Detecting a faint companion below the Rayleigh limit costs the companion a dose that does not depend on its faintness, while under direct imaging the dose grows without bound. For a fragile sample the gentlest measurement is also the simplest one: a single photon, recycled.
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Quantum sensing with undetected photons is a technique where photons of one wavelength probe a sample, but information is extracted by measuring photons of another wavelength that never interacts with the sample. This has seen significant experimental advances in applications such as spectroscopy, microscopy, and bio-sensing. However, a detailed theoretical analysis using the tools of quantum metrology is currently lacking. Thus it is unclear how far away current schemes are from fundamental limits, and what the optimal measurement strategies are. We apply a multiparameter quantum estimation framework to quantify the error when estimating the unknown transmission and phase shift of a sample. The optimal measurement scheme is shown to require only a single controllable phase shift, easily implementable in existing setups. We also study how to use multipass interactions to maximise information gain. In general the optimum number of passes scales inversely with the log of the transmission of the sample. This work clarifies the metrological power of quantum sensing with undetected photons, and provides guidance for the design of experiments requiring high sensitivity.
Interferometry with quantum light is known to provide enhanced precision for estimating a single phase. However, depending on the parameters involved, the quantum limit for the simultaneous estimation of multiple parameters may not attainable, leading to trade-offs in the attainable precisions. Here we study the simultaneous estimation of two parameters related to optical interferometry: phase and loss, using a fixed number of photons. We derive a trade-off in the estimation of these two parameters which shows that, in contrast to single-parameter estimation, it is impossible to design a strategy saturating the quantum Cramer-Rao bound for loss and phase estimation in a single setup simultaneously. We design optimal quantum states with a fixed number of photons achieving the best possible simultaneous precisions. Our results reveal general features about concurrently estimating Hamiltonian and dissipative parameters, and has implications for sophisticated sensing scenarios such as quantum imaging.
Optical interferometry is a cornerstone technique for precise phase measurements across various fields. In many applications, for example, biological imaging, it often necessitates stringent limits on light intensity to prevent adverse effects on light-sensitive samples, a condition known as dose-limited regimes. Maximizing the precision per dose is therefore crucial. In quantum metrology, quantum correlations enable high precision in phase estimation while adhering to dose constraints. Nevertheless, photon loss, including absorption by a sample, substantially diminishes the benefits of quantum enhancement in interferometry. In this work, we experimentally investigate a dose-efficient approach to quantum phase estimation using sequential strategies in the presence of loss. Performance of sequential strategies with and without control is evaluated through quantum Fisher information (QFI) per dose. Experimental results show that both sequential strategies exceed the classical limit and outperform the parallel strategy using unbalanced N00N states. Notably, the control-enhanced sequential strategy attains superior QFI per dose, approaching the quantum limit. These results highlight the promise of sequential strategy for imaging and sensing in resource-constrained scenarios, marking a significant step toward practical and efficient quantum metrology in lossy environments.
Abstract Two-photon absorption (TPA) is a nonlinear optical process with wide-ranging applications from spectroscopy to super-resolution imaging. Despite this, the precise measurement and characterisation of TPA parameters are challenging due to their inherently weak nature. We study the potential of single-mode quantum light to enhance TPA parameter estimation through the quantum Fisher information (QFI). Discrete variable quantum states (defined to be a finite superposition of Fock states) are optimised to maximise the QFI for given absorption, revealing a quantum advantage compared to both the coherent state (classical) benchmark and the single-mode squeezed vacuum state. For fixed average energy n ¯ ∈ 2 N , the Fock state is shown to be optimal for large TPA parameters, while a superposition of vacuum and a particular Fock state is optimal for small absorption for all n ¯ . This differs from single-photon absorption where the Fock state is always optimal. Notably, photon counting is demonstrated to offer optimal or nearly optimal performance compared to the QFI bound for all levels of TPA parameters for the optimised quantum probes, and their quantum advantage is shown to be robust to single-photon loss. Our findings provide insight into known limiting behaviours of Gaussian probes and their different FI scalings under photon counting ( ∝ n ¯ 2 for squeezed vacuum states versus n ¯ 3 for coherent states). The squeezed state outperforms coherent states for small TPA parameters but underperforms in the intermediate regime, becoming comparable in the large absorption limit. This can be explained through fundamental differences between behaviours of even and odd number Fock states: the former’s QFI diverges in both large and small absorption limits, while the latter diverges only in the small absorption limit, dominating at intermediate scales.
Interferometry with quantum light is known to provide enhanced precision for estimating a single phase. However, depending on the parameters involved, the quantum limit for the simultaneous estimation of multiple parameters may not be attainable, leading to tradeoffs in the attainable precisions. Here we study the simultaneous estimation of two parameters related to optical interferometry: phase and loss, using a fixed number of photons. We derive a tradeoff in the estimation of these two parameters which shows that, in contrast to single-parameter estimation, it is impossible to design a strategy saturating the quantum Cram\'er-Rao bound for loss and phase estimation in a single setup simultaneously. We design optimal quantum states with a fixed number of photons achieving the best possible simultaneous precisions. Our results reveal general features about concurrently estimating Hamiltonian and dissipative parameters and have implications for sophisticated sensing scenarios such as quantum imaging.