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arXiv:2608.19528

Physics-Based versus Data-Driven Classification of Single-Photon Quantum Emitters from Sparse Autocorrelation Data

Nhat Minh Nguyen, Md Shakhawath Hossain, Duc Anh Ngo, Chaohao Chen, Xiaoxue Xu, Toan Trong Tran, Carlo Bradac

quant-phSubmitted Aug 20, 2026• Announced Aug 21, 2026• 0 citations
arXivHTMLPDF

Abstract

Identifying single photon emitters from large, inhomogeneous candidate populations is key to realizing many quantum applications. This requires measuring the emitters second order autocorrelation function, whose statistical reliability is fundamentally limited by acquisition time. Machine learning classifiers can accelerate identification from sparse data, but their performance relative to physics-based inference has not been systematically examined. Here, we introduce sequential Bayesian inference for single photon emitter classification and benchmark it against Levenberg-Marquardt fitting and a feedforward neural network. We use synthetic training and test data calibrated against real Hanbury Brown-Twiss measurements from hexagonal boron nitride emitters, enabling evaluation against an exactly known ground-truth emitter number under realistic noise and background conditions. All three approaches achieve high, near-perfect accuracy with sufficient integration time, but differ greatly in convergence rate and robustness under sparse photon statistics. The neural network is most robust at short integration times. The Bayesian classifier reaches near-perfect accuracy fastest, while retaining full physical interpretability. Levenberg-Marquardt fitting remains a valuable, fully interpretable method, achieving the highest recall despite being the slowest to converge. These results lead to several key conclusions. No single method dominates across all performance metrics. Relying on any one metric alone can give a misleading picture of classifier performance, particularly under sparse photon statistics. Physics-based and data-driven methods are complementary rather than competing approaches. Together, these findings provide practical guidance for selecting and combining classification strategies for scalable single-photon-source screening and other quantum-emitter characterization tasks.

Comments
Manuscript: 18 pages, 3 figures, 5 Tables. Supplementary Information: 7 pages, 1 figure

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Identifying single photon emitters from large, inhomogeneous candidate populations is key to realizing many quantum applications. This requires measuring the emitters second order autocorrelation function, whose statistical reliability is fundamentally limited by acquisition time. Machine learning classifiers can accelerate identification from sparse data, but their performance relative to physics-based inference has not been systematically examined. Here, we introduce sequential Bayesian inference for single photon emitter classification and benchmark it against Levenberg-Marquardt fitting and a feedforward neural network. We use synthetic training and test data calibrated against real Hanbury Brown-Twiss measurements from hexagonal boron nitride emitters, enabling evaluation against an exactly known ground-truth emitter number under realistic noise and background conditions. All three approaches achieve high, near-perfect accuracy with sufficient integration time, but differ greatly in convergence rate and robustness under sparse photon statistics. The neural network is most robust at short integration times. The Bayesian classifier reaches near-perfect accuracy fastest, while retaining full physical interpretability. Levenberg-Marquardt fitting remains a valuable, fully interpretable method, achieving the highest recall despite being the slowest to converge. These results lead to several key conclusions. No single method dominates across all performance metrics. Relying on any one metric alone can give a misleading picture of classifier performance, particularly under sparse photon statistics. Physics-based and data-driven methods are complementary rather than competing approaches. Together, these findings provide practical guidance for selecting and combining classification strategies for scalable single-photon-source screening and other quantum-emitter characterization tasks.
Identification of a suitable source of single photons via second-order autocorrelation function measurement within an array of thousand possible candidates is a routine, key step of any practical realization in quantum optics. Within this work, we have shown that machine learning algorithms enable high precision classification between “single” and “not single” quantum emitters based on sparse autocorrelation data measurement and require < 1 s acquisition time, while conventional methods demand > 1 min. Machine learning assisted classification, done on a sparse 1-s dataset, provides ~85% accuracy of “single”/“not single” emitter identification versus only 57% of the conventional Levenberg-Marquardt approach.
Abstract Deterministic nanoassembly may enable unique integrated on‐chip quantum photonic devices. Such integration requires a careful large‐scale selection of nanoscale building blocks such as solid‐state single‐photon emitters by means of optical characterization. Second‐order autocorrelation is a cornerstone measurement that is particularly time‐consuming to realize on a large scale. Supervised machine learning‐based classification of quantum emitters as “single” or “not‐single” is implemented based on their sparse autocorrelation data. The method yields a classification accuracy of 95% within an integration time of less than a second, realizing roughly a 100‐fold speedup compared to the conventional Levenberg–Marquardt fitting approach. It is anticipated that machine learning‐based classification will provide a unique route to enable rapid and scalable assembly of quantum nanophotonic devices.
Characterization of the photon statistics of an optical field is central to identifying light sources in various quantum-enabled technologies, from super-resolved quantum imaging to precise quantum sensing and spectroscopy. In practice, however, estimating photon-correlation functions with sufficient accuracy requires long acquisition times and computationally intensive statistical estimators, severely limiting real-time operation and the study of rapidly varying or weak sources. Here, we show that learned inference based on artificial neural networks enables rapid estimation of second-order coherence directly from photon-number-resolved measurements, outperforming the precision of conventional statistical methods with processing times three orders of magnitude shorter. Our approach is source-agnostic and remains accurate in few-photon illumination regimes where the statistics of coherent, partially coherent, thermal, and super-thermal light become nearly indistinguishable. We experimentally validate the method across more than 4000 distinct classical light sources, demonstrating equal or improved precision with drastically reduced data and computational requirements. These results establish machine-learning-enabled photon-statistics inference as a new operational route to rapid optical-coherence diagnostics, enabling real-time monitoring of classical light sources in regimes previously inaccessible to conventional estimators.
Quantum correlation measurements have emerged as a powerful tool for localizing multiple emitters with subwavelength separation. Multi-emitter localization consists of two distinct tasks: identifying the emitter count NNN and estimating their positions {xi}\left\{x^{i}\right\}{xi}. Existing fit-and-select frameworks fit the measured intensity and autocorrelation data using several models corresponding to different values of NNN and then select the best-supported model. This procedure lets errors from the multi-parameter optimization of emitter positions propagate into the choice of model, degrading performance under photon-limited and high-background conditions. We propose a method that directly infers the emitter count and positions from the multimodal data via learned inference. Learned inference improves both the emitter-counting accuracy and localization precision compared to the fit-and-select method. It achieves more than tenfold improvement in precision and requires up to five times fewer photons to achieve practically meaningful localization with the largest gains observed under low photon counts, strong background, narrowly spaced emitter configurations, and spatially truncated data. This photon-efficient quantum-assisted localization framework offers a promising route toward real-time biological imaging and single-particle tracking in densely labeled samples.
Abstract Identifying which candidate sites on a solid-state sample are single-photon emitters requires a Hanbury Brown–Twiss (HBT) measurement of the second-order correlation function g(2)(τ), which is slow because photon coincidences accumulate at a rate proportional to the square of the detected count rate. We examine how much of this time can be saved by deciding while the coincidences are still accumulating and by adapting the exposure of each site. A spiking neural network reads the coincidence record in short time slices and updates, after every slice, its estimate of the probability that the site hosts a single emitter; a reinforcement-learning controller decides, site by site, whether to expose longer, certify, or reject; and a graph that encodes the electronic level structure of each emitter class conditions one estimator on the class being measured. All components are trained on simulated data from a standard three-level photon-counting model, which we validate against the exact master-equation solution before use. In simulation, the event-driven estimator reaches 90% balanced accuracy with 6 times less acquisition time than a multistart least-squares fit, typically committing to a decision 312 ms into a 1 s exposure, and adaptive exposure screens simulated 48-site fields 1.7 times faster than fixed-dwell scanning at matched precision and recall. Applied without retraining to published experimental HBT data from an InGaAs/GaAs quantum dot, a network trained only on simulated pulsed-excitation histograms estimates g(2)(0) from 30 s records with half the error of peak-area analysis of the same records. The closed-loop results are obtained in simulation only. The code, data, and trained models are openly available.
With wide applications ranging from quantum communication and metrology to biomedicine, single photon sources in solid-state hosts have become a major area of study. Here, we focus on three applications: nanothermometry, optically detected magnetic resonance (ODMR), and second order autocorrelation. We present novel statistical and machine learning (ML) approaches to extract information from experimental and simulated data and benchmark these methods against traditional inference-based statistical approaches. We found that compared to traditional inference-based methods ML algorithms can: i) predict temperatures at the nanoscale with greater accuracy and with less calibration points than traditional fitting methods; ii) identify the resonance peaks in ODMR spectra with factors ~1.3x and ~4.7x better accuracy and resolution and achieved equal or better performance with ~5x less data; and iii) have the potential to parse second order autocorrelation data more efficiently. ML algorithms are thus powerful tools for quantum sensing techniques. Author Keywords: colour centers, machine learning, nanosensing, nanothermometry, optically detected magnetic resonance, second order autocorrelation