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arXiv:2608.19494

Stability and squeezing of the three-photon degenerate parametric down-conversion

Vinícius V. Seco, Alencar J. de Faria

quant-phcond-mat.otherphysics.opticsSubmitted Aug 19, 2026• Announced Aug 21, 2026• 0 citations
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Abstract

Nonlinear multiphoton conversion processes are theoretically and experimentally challenging systems in quantum optics and related areas. These phenomena bring remarkable quantum properties and can be of fundamental relevance in quantum information and computation applications. Based on recent experimental advances and the possible uses in generalized three-photon squeezing, we investigate degenerate three-photon parametric down-conversion generated inside a cavity fed by a classical pump. In addition, we consider that the process is stimulated by a coherent driving mode and subjected to dissipation by spontaneous emission of the cavity. A treatment using phase-space methods and stochastic differential equations is applied and the stability conditions of its steady states are found. We find that the system does not exhibit multistability, instead it has a limited parameter region leading to a single stable steady branch, alongside multiple unstable branches. Focusing on the stable steady states and linearizing the dynamics around them, we calculate the spectral densities of the quadrature variables. We identify and characterize the squeezing of three-photon down-conversion. Moreover, since the quasi-probability differential equations of the higher-order multiphoton processes have higher-order derivatives, hindering their mapping into stochastic differential equations, we make use of a positive Wigner function approach to calculate two-dimensional spectral densities associated with three-time correlation functions, with the goal of studying non-Gaussian properties of the system.

Comments
24 pages, 8 figures. To be submitted for publication

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Nonlinear multiphoton conversion processes are theoretically and experimentally challenging systems in quantum optics and related areas. These phenomena bring remarkable quantum properties and can be of fundamental relevance in quantum information and computation applications. Based on recent experimental advances and the possible uses in generalized three-photon squeezing, we investigate degenerate three-photon parametric down-conversion generated inside a cavity fed by a classical pump. In addition, we consider that the process is stimulated by a coherent driving mode and subjected to dissipation by spontaneous emission of the cavity. A treatment using phase-space methods and stochastic differential equations is applied and the stability conditions of its steady states are found. We find that the system does not exhibit multistability, instead it has a limited parameter region leading to a single stable steady branch, alongside multiple unstable branches. Focusing on the stable steady states and linearizing the dynamics around them, we calculate the spectral densities of the quadrature variables. We identify and characterize the squeezing of three-photon down-conversion. Moreover, since the quasi-probability differential equations of the higher-order multiphoton processes have higher-order derivatives, hindering their mapping into stochastic differential equations, we make use of a positive Wigner function approach to calculate two-dimensional spectral densities associated with three-time correlation functions, with the goal of studying non-Gaussian properties of the system.
The optical parametric oscillator is one of the most well-characterized devices in nonlinear optics, with many useful applications, especially as a frequency converter and as a wide-band amplifier. Novel discoveries made with these devices in the quantum domain include demonstrations of large amounts of both single-mode and two-mode squeezing, and, in the two-mode case, significant quantum intensity correlations between the two modes and quadrature correlations, which provided the first experimental demonstration of the original Einstein–Podolsky–Rosen (EPR) paradox. In this chapter, a systematic theory is developed of quantum fluctuations in the degenerate parametric oscillator. The quantum statistical effects produced by the degenerate parametric amplifier and oscillator have been intensely studied. As we have seen, the amount of transient squeezing produced in an ideal lossless parametric amplifier was calculated using asymptotic methods by Crouch and Braunstein. It was found to scale inversely with the square root of the initial pump photon number. When the system is put into a cavity, and driving and dissipation are introduced, we find that the steady state of a driven degenerate parametric oscillator bifurcates. There is a single steady state at low driving strengths, but, as the driving field increases, a threshold value is reached and the single state splits and forms two stable states. Below the threshold, a linearized analysis of squeezing in the quantum quadratures is possible; while above this threshold, or critical point, the tunneling time between the two states due to quantum fluctuations can be calculated.
We theoretically investigate the properties and temporal evolution of squeezed states generated using degenerate parametric down conversion in lossy cavities. We show that the Lindblad master equation, which governs the evolution of this system, has, as its solution, a squeezed thermal state with an effective temperature and squeezing parameter that depends on time. We derive analytical solutions for the time evolution of quadrature noise, thermal photon number, squeezing parameter, and total photon number under different pumping regimes. We also find the steady state limits of the quadrature noises and discuss the g(2) factor of the generated light inside the cavity in the steady state.
In this research, squeezing fragility due to thermal bath, in quantum squeezed state generation, is simulated. For this purpose, single mode dissipative cavity with non-zero second-order susceptibility is used. Cavity nonlinear medium is driving by laser pump with known frequency, and pairs of identical photons are created, with one-half frequency of driving pump. This process known as degenerate parametric down conversion. In the absence of any dissipation, simulation shows linear time dependent squeezing parameter, which is in agreement with theoretical results. In two photon loss of cavity in contact with cold reservoir, competition between gain and two photon loss, results in stable squeezing of initial vacuum, in steady state of system. At the end, has been shown that, non-zero thermal reservoir, omits the squeezing and leads the final cavity field to the thermal mixture of Fock states.
In quantum information processing, control of quantum entanglement is of central importance, particularly for applications in quantum computing. One established method for generating entanglement is squeezing, which exploits the uncertainty principle: fluctuations in one of a pair of conjugate variables are suppressed at the expense of enhanced fluctuations in the other. A representative approach for squeezing is the parametric amplifier. Depending on the parametric excitation amplitude, the system exhibits regimes of stability and instability of the trivial solution. Conventional studies of squeezing have focused on the stable regime, where the squeezing is maximized near the instability threshold. When the parametric excitation amplitude is increased further and the system enters the unstable regime, the system can reach a steady state due to cubic nonlinearity. However, the squeezing properties of this state have not been fully clarified. In this study, as a first step toward a quantum-mechanical treatment, we investigate squeezing in a classical parametric amplifier in the unstable regime. To enable analytical treatment, we approximate the white noise by a narrowband resonant cosine component and neglect stochasticity. The analysis shows that the steady-state amplitude depends on the phase difference between the noise and the parametric excitation, as in the stable regime, indicating a squeezing effect. Moreover, the conditions under which the steady-state amplitude is maximized and minimized with respect to this phase difference are derived. In addition, we analytically determine how the parametric excitation and noise modify the cubic-nonlinearity-induced bifurcation structure. Based on these findings, we propose a squeezing mechanism that exploits the properties of the unstable regime, unlike conventional approaches. Numerical simulations incorporating stochastic noise reveal the emergence of squeezing, although the effect is weaker than in the stable regime. These results suggest that the unstable regime may offer a possible route for utilizing previously unexplored characteristics.
Very recently, strongly non-Gaussian states have been observed via a direct three-mode spontaneous parametric down-conversion in a superconducting cavity [Phys. Rev. X 10, 011011 (2020)]. The created multiphoton non-Gaussian correlations are attractive and useful for various quantum information tasks. However, how to detect and classify multipartite non-Gaussian entanglement has not yet been completely understood. Here, we present an experimentally practical method to characterize continuous-variable multipartite non-Gaussian entanglement, by introducing a class of nonlinear squeezing parameters involving accessible higher-order moments of phase-space quadratures. As these parameters can depend on arbitrary operators, we consider their analytical optimization over a set of practical measurements, in order to detect different classes of multipartite non-Gaussian entanglement ranging from fully separable to fully inseparable. We demonstrate that the nonlinear squeezing parameters act as an excellent approximation to the quantum Fisher information within accessible third-order moments. The level of the nonlinear squeezing quantifies the metrological advantage provided by those entangled states. Moreover, by analyzing the above-mentioned experiment, we show that our method can be readily used to confirm fully inseparable tripartite non-Gaussian entangled states by performing a limited number of measurements without requiring full knowledge of the quantum state.
We investigate theoretically the properties of squeezed states generated using degenerate parametric down conversion in lossy cavities. We show that the Lindblad master equation, which governs the evolution of this system, has as its solution a squeezed thermal state with an effective temperature and squeezing parameter that depends on time. We derive analytical solutions for the time-evolution of quadrature noise, thermal photon number, squeezing parameter, and total photon number under different pumping regimes. We also find the steady state limits of the quadrature noises and discuss the $ g^{(2)} $ factor of the generated light inside the cavity in the steady state.