Domain walls are carriers of spin transport whose controlled manipulation underlies a wide range of spintronic and information-processing technologies. Here we demonstrate tunable domain-wall transport in a weakly interacting nondegenerate ultracold Bose gas. We initialize a three-domain pseudo-spin-1/2 texture and observe spontaneous propagation of long-lived domain walls driven by exchange-mediated spin currents. By varying the orientation of the spin domains, we control the balance of spin currents across the walls and thereby tune their trajectories, including reversals of the initial direction of motion. Measurements reveal a crossover from an exchange-stabilized regime, in which coherent spin-exchange collisions suppress wall motion, to a diffusion-dominated regime characterized by rapid transport at thermal velocities. Numerical solutions of a quantum Boltzmann equation reproduce the observed dynamics and identify transverse phase gradients as an important control parameter governing domain-wall propagation. These results establish coherence and phase engineering as tools for programming spin transport in ultracold gases and provide a route toward controllable domain-wall dynamics in atomtronic systems.
Domain walls are carriers of spin transport whose controlled manipulation underlies a wide range of spintronic and information-processing technologies. Here we demonstrate tunable domain-wall transport in a weakly interacting nondegenerate ultracold Bose gas. We initialize a three-domain pseudo-spin-1/2 texture and observe spontaneous propagation of long-lived domain walls driven by exchange-mediated spin currents. By varying the orientation of the spin domains, we control the balance of spin currents across the walls and thereby tune their trajectories, including reversals of the initial direction of motion. Measurements reveal a crossover from an exchange-stabilized regime, in which coherent spin-exchange collisions suppress wall motion, to a diffusion-dominated regime characterized by rapid transport at thermal velocities. Numerical solutions of a quantum Boltzmann equation reproduce the observed dynamics and identify transverse phase gradients as an important control parameter governing domain-wall propagation. These results establish coherence and phase engineering as tools for programming spin transport in ultracold gases and provide a route toward controllable domain-wall dynamics in atomtronic systems.
Ultra-cold trapped atoms, with their high degree of tunability, provide ideal model systems to study physical phenomena with applications in many different fields of research. This thesis describes studies on spin transport phenomenon in a trapped ultra-cold spin-polarized 87Rb gas at temperatures above quantum degeneracy. This work is focused on the less studied regime of cross-over between classical and quantum transport. Diffusion is a fundamental dissipative process that tends to relax any system towards a state of minimum inhomogeneity. In this work we study longitudinal spin diffusion as a special case of spin transport. The system studied here consists of two anti-parallel longitudinal spin domains separated by a helical domain-wall. We report that the diffusion process manifests a significant deviation from classical diffusion due to purely quantum mechanical modifications. The two-domain spin textures are prepared using optical and microwave pulse techniques, and the dynamics of the spin structure is studied as it relaxes towards the final equilibrium state. Generally, there is a wide range of parameter space that could be studied. In this work we focused our studies on the effects related to the degree of coherence in the domainwall as well as the effective magnetic field acting on the spins. By controllably tuning these experimental parameters, we studied in detail how the spatiotemporal behaviour of the diffusion dynamics is modified. Our results show that the longitudinal spin diffusion time scales depend sensitively on the domain-wall degree of coherence. External magnetic field gradients also alter the dynamics noticeably, manifesting a significant dependence on the sign of the applied field gradients.
We consider coherent states of weakly interacting bosons under the conditions of external resonant excitation, with a focus on a two-dimensional polariton fluid driven by a plane electromagnetic wave near the ground state. The coherent driving breaks the U(1) symmetry explicitly, which prevents the occurrence of quantum vortices in a uniform scalar condensate. Surprisingly, a spinor (two-component) system of the same kind admits topological excitations, such as domain walls of relative phase or confined half-vortex molecules, typical of a freely evolving spinor Bose system. Opposite-phase domains arise from the spontaneous breakdown of the spin symmetry (Z2). Domain walls form with time even when the initial state of the system is uniform or completely disordered; they fall into different topological types distinguished by the total phase variation in the transverse direction. One type of domain walls is similar to ``magnetic'' solitons in Bose-Einstein condensates and exhibits nonzero spin polarization whose sign depends on the direction of motion. Domain walls of the second type, by contrast, behave like monopoles with broken spatiotemporal symmetry and tend to move in certain preferred directions. The interaction of vortices and domain walls results in a long-range ordering of the system.
We study the stability of two-domain spin structures in an ultracold gas of magnetically trapped 87Rb atoms above quantum degeneracy. Adding a small effective magnetic field gradient stabilizes the domains via coherent collective spin rotation effects, despite negligibly perturbing the potential energy relative to the thermal energy. We demonstrate that domain stabilization is accomplished through decoupling the dynamics of longitudinal magnetization, which remains in time-independent domains, from transverse magnetization, which undergoes a purely transverse spin wave trapped within the domain wall. We explore the effect of temperature and density on the steady-state domains, and compare our results to a hydrodynamic solution to a quantum Boltzmann equation.
Diffusion plays a major role in describing how particles and heat move in any nonequilibrium system. The diffusion of quantum properties is not as well understood as the diffusion of classical properties, especially at low temperatures or high densities. Exploring the diffusion of the quantum property known as spin is beneficial for explaining quantum effects that arise at low temperatures or high densities, and this knowledge acquired could assist in the development of new ultra-low-power devices. This thesis examines spin diffusion at various temperatures and densities using the highly-tunable experimental platform of ultracold atoms. Around one million rubidium-87 atoms are cooled to nanokelvin temperatures to create an ultracold gas, where quantum interactions between atoms can significantly modify spin diffusion compared to classical diffusion. One-dimensional spin diffusion is observed for an initial two-domain spin profile. Remarkably, diffusion of this spin profile is slowed at temperatures above quantum degeneracy, where the ultracold gas is largely classical but with quantum collisions. We demonstrate that this slowing of spin diffusion is due to the presence of spin coherence between spin domains, and that the removal of coherence speeds up spin diffusion to classical timescales. Spin diffusion is further modified by applying a linear differential potential that can speed, slow, or stop spin diffusion of a two-domain spin profile. Differential potentials spatially alter the precession of spins, which then alters the spin-rotating quantum collisions that modify spin diffusion. For a linear differential potential with a specific sign and magnitude, stabilized spin domains in an ultracold gas are observed for 40 times longer than classical diffusion timescales. In addition to modifying spin diffusion with coherence and differential potentials, we demonstrate arbitrary control of one-dimensional spin diffusion using temporally varying differential potentials and three-domain spin profiles. These spin diffusion modifying techniques could be useful for manipulating spin in other nonequilibrium systems, and set the stage for simulating spin-based devices in ultracold atoms.
Spinful superfluids of ultracold atoms are ideal for investigating the intrinsic properties of spin current and texture because they are realized in an isolated, nondissipative system free from impurities, dislocations, and thermal fluctuations. This study theoretically reveals the impact of spin current on a magnetic domain wall in spinful superfluids. An exact wall solution is obtained in the ferromagnetic phase of a spin-1 Bose-Einstein condensate with easy-axis anisotropy at zero temperature. The bosonic-quasiparticle mechanics analytically show that the spin current along the wall becomes unstable if the velocity exceeds the critical spin-current velocities, leading to complicated situations because of the competition between transverse magnons and ripplons. Our direct numerical simulation reveals that this system has a mechanism to generate an eccentric fractional skyrmion, which has a fractional topological charge, but its texture is not similar to that of a meron. This mechanism is in contrast to the generation of conventional skyrmions in easy-axis magnets. The theoretical findings can be examined in the same situation as in a recent experiment on ultracold atoms. In terms of the universality of spontaneous symmetry breaking, unexplored similar phenomena are expected in different physical systems with the same broken symmetry.
The three experiments described in this thesis investigate fundamental properties of ultracold atoms. Using laser cooling and evaporative cooling, a dilute gas of sodium atoms is cooled to ~100 nK. Under these circumstances a Bose-Einstein condensate (BEC) forms, where millions of atoms collapse into the lowest energy state of the system and share a macroscopic wavefunction. The experiments are done in an ultrahigh vacuum and the atoms are manipulated remotely using laser beams, magnetic fields, and RF-fields. Using ultracold atoms allows unprecedented control over the internal and external degrees of freedom of the system, making it very suitable for precision measurements. Ultracold atoms also serve as a model system for more complicated or remote fields such as solid-state physics and cosmology. In the first experiment the refractive index of an ultracold bosonic gas is studied. The atomic clouds are analyzed for temperature and number of particles using nearly non-destructive phase-contrast imaging. After each pulse of probe light a small fraction of the atoms is lost, while the cloud is simultaneously slightly heated. This makes it possible to study the scattering rate as a function of temperature using only a single sample. It is observed that the scattering rate increases below the critical temperature for BEC by more than a factor of 3 compared to the classical value. This enhancement is in good agreement with the predictions by theoretical work that takes two-body correlation and the Lorentz-Lorenz correction into account. The method is also used to perform calorimetry on the Bose gas and directly measure the heat capacity of the BEC. The second chapter deals with magnetism in ultracold gases. When cooling an ultracold gas containing different spin components below the critical temperature for BEC, stable magnetic domains form. The appearance of these domains and the dynamics of the domain walls are studied. The spin mixture is prepared by performing an RF-sweep on ground state atoms in the presence of a magnetic field. Spin dynamics are induced by applying magnetic gradients. Spin drag, which is the transport coefficient responsible for damping spin currents, was measured in a two-component system. Furthermore a new method for spin resolved phase contrast imaging is presented, which is used to study time evolution in situ non-destructively. The last experiment focuses on spontaneous symmetry breaking. When passing a continuous phase transition, spontaneous symmetry breaking causes the development of domains with an independently chosen order parameter. The domains are separated by boundary defects. In this experiment the spontaneous creation of solitons was observed, which are boundary defects in the phase of the condensate, as well as magnetic domain walls, which are the boundary defects in the magnetization. Through the Kibble-Zurek mechanism it is possible to determine the critical exponents that characterize the phase transition. The critical exponents are predicted to be universal, i.e. do not depend on the microphysics of the system, so the results from our ultracold atoms lab can help answer universal questions for example from cosmology and from the early universe.