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arXiv:2607.23064

Size characterization of neutral rare-gas clusters based on time-resolved polarization anisotropy measurements

Arne Morlok, Grzegorz Kowzan, Y. G. Li, Ulrich Bangert, Frank Stienkemeier, Lukas Bruder

Published Jul 25, 2026• 0 citations
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Abstract

The size determination of neutral clusters is experimentally challenging. In particular, weakly-bound rare-gas clusters tend to fragment upon ionization, resulting in systematic errors in cluster size studies. In contrast, characterization of the temporal polarization anisotropy dephasing provides a soft detection scheme for cluster size estimation, which avoids fragmentation of the clusters. Here, we present a systematic experimental study of argon and neon clusters in the size range of 50 to 10.000 atoms using this technique. In order to extract the mean cluster sizes from the data, we present an efficient analytical model of the polarization anisotropy dephasing of an ensemble of doped clusters. The approach shows remarkable sensitivity to small changes in the mean cluster size of just a few tens of atoms and allows us to refine the widely used Hagena scaling law for the estimation of rare-gas cluster sizes.

DOI
10.48550/arxiv.2607.23064

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The size determination of neutral clusters is experimentally challenging. In particular, weakly-bound rare-gas clusters tend to fragment upon ionization, resulting in systematic errors in cluster size studies. In contrast, characterization of the temporal polarization anisotropy dephasing provides a soft detection scheme for cluster size estimation, which avoids fragmentation of the clusters. Here, we present a systematic experimental study of argon and neon clusters in the size range of 50 to 10.000 atoms using this technique. In order to extract the mean cluster sizes from the data, we present an efficient analytical model of the polarization anisotropy dephasing of an ensemble of doped clusters. The approach shows remarkable sensitivity to small changes in the mean cluster size of just a few tens of atoms and allows us to refine the widely used Hagena scaling law for the estimation of rare-gas cluster sizes.
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In this paper, quantum fluctuations of a carbonyl sulfide molecule in helium-4 clusters are studied as a function of cluster size N in a small-to-large size regime (2 ≤ N ≤ 64). The molecular rotation of the dopant shows nonmonotonic size dependence in the range of 10≤N≤20, reflecting the density distribution of the helium atoms around the molecule. The size dependence on the rotational constant shows a plateau for N≥20, which is larger than the experimental nanodroplet value. Superfluid response of the doped cluster is found to show remarkable anisotropy especially for N ≤20. The superfluid fraction regarding the axis perpendicular to the molecular axis shows a steep increase at N = 10, giving the significant enhancement of the rotational fluctuation of the molecule. On the other hand, the superfluid fraction regarding the axis parallel to the molecular axis reaches 0.9 at N=5, arising from the bosonic exchange cycles of the helium atoms around the molecular axis. The anisotropy in the superfluid response is found to be the direct consequence of the configurations of the bosonic exchange cycles. © 2007 American Institute of Physics.
The dephasing time of spin-polarized atoms in an atomic vapor cell plays an important role in determining the stability of vapor-cell clocks as well as the sensitivity of optically-pumped magnetometers. The presence of a buffer gas can extend the lifetime of these atoms. Many vapor cell systems operate at a fixed (often elevated) temperature. For ambient temperature operation with no temperature control, it is necessary to characterize the temperature dependence as well. We present a spin-polarization lifetime study of Cesium vapor cells with different buffer gas pressures, and find good agreement with expectations based on the combined effects of wall collisions, spin exchange, and spin destruction. For our (7.5 mm diameter) vapor cells, the lifetime can be increased by two orders of magnitude by introducing Ne buffer gas up to 100 Torr. Additionally, the dependence of the lifetime on temperature is measured (25 - 47 oC) and simulated for the first time to our knowledge with reasonable agreement.
This paper investigates the possibility of suppressing the ionization rate in a magnetostatic trap of metastable neon atoms by spin-polarizing the atoms. Suppression of the ionization is critical for the possibility of reaching Bose-Einstein condensation with such atoms. We estimate the relevant long-range interactions for the system, consisting of electric quadrupole-quadrupole and dipole-induced dipole terms, and develop short-range potentials based on the Na2{\mathrm{Na}}_{2}Na2​ singlet and triplet potentials. The autoionization widths of the system are also calculated. With these ingredients we calculate the ionization rate for spin-polarized and for spin-isotropic samples, caused by anisotropy of the long-range interactions. We find that spin polarization may allow for four orders of magnitude suppression of the ionization rate for Ne. The results depend sensitively on a precise knowledge of the interaction potentials, however, pointing out the need for experimental input. The same model gives a suppression ratio close to unity for metastable xenon in accordance with experimental results, due to a much increased anisotropy in this case.