Direct, real-space imaging of spin-wave propagation and wavefronts in magnetic materials is crucial for advancing both fundamental understanding of spin dynamics and the development of functional devices. This, however, remains a significant challenge, especially in materials with complex magnetic characteristics at the nanoscale. Here, we employ scanning nitrogen-vacancy center spectroscopy to achieve visualization of spin waves in two archetypical magnetic films: yttrium-iron-garnet and lanthanum strontium manganese oxide. We reveal a wavelength-dependent spin-wave filtering effect near point-like magnetic scatterers and a modified spin wavefront in antiferromagnetically coupled stripe domains. The spin-wave characteristics are explained using micromagnetic simulations and analytical calculations. These findings point to possible fine control of spin-wave propagation near complex magnetic structures and extend the scope of spin-wave imaging based on nitrogen-vacancy centers beyond uniform magnets.
Direct, real-space imaging of spin-wave propagation and wavefronts in magnetic materials is crucial for advancing both fundamental understanding of spin dynamics and the development of functional devices. This, however, remains a significant challenge, especially in materials with complex magnetic characteristics at the nanoscale. Here, we employ scanning nitrogen-vacancy center spectroscopy to achieve visualization of spin waves in two archetypical magnetic films: yttrium-iron-garnet and lanthanum strontium manganese oxide. We reveal a wavelength-dependent spin-wave filtering effect near point-like magnetic scatterers and a modified spin wavefront in antiferromagnetically coupled stripe domains. The spin-wave characteristics are explained using micromagnetic simulations and analytical calculations. These findings point to possible fine control of spin-wave propagation near complex magnetic structures and extend the scope of spin-wave imaging based on nitrogen-vacancy centers beyond uniform magnets.
Spin waves carry their propagation direction in the handedness of their circularly polarized stray field, a property inaccessible to scalar magnetometers. In the Damon-Eshbach surface wave of an in-plane magnetized film, the dipolar field above the film rotates with a handedness fixed by the direction of travel. The nitrogen-vacancy (NV) centre in diamond is an intrinsic polarization analyser: a right-handed field about the NV axis drives one spin transition, and a left-handed field drives the other, in both the ground and the excited state. Here, we exploit the two excited-state transitions, which lie inside the spin-wave band of yttrium iron garnet (YIG), as a pair of chirality channels and image Damon-Eshbach waves in both directions. Because reflection from an etched boundary reverses the handedness, the incident and reflected waves appear as two lines in one spectrum and are imaged separately. In the ground state, the same rule applies, and the selected field drives Rabi oscillations, a route to chirality-selective control of the NV spin by magnons. Reading the two channels gives the direction of a spin wave at one point, without a phase reference. This advances chirality-resolved quantum sensing and provides insight into chiral spin-wave dynamics.
Magnetic field fluctuations on nanometer length scales manifest in a diverse range of phenomena -- electron and spin dynamics in materials and devices, quantum many-body systems, and molecular chemistry. Measuring these phenomena requires sensors with a challenging combination of broad spectral bandwidth, high sensitivity, and nanoscale spatial resolution. Nitrogen-vacancy (NV) centers, atom-like quantum sensors in diamond, possess the requisite sensitivity and nanoscale sensing volume, but are typically limited in bandwidth by the practical speed of the applied quantum control sequence. Here, we overcome this limitation by exposing the NV qubit to a microwave dressing field during a dynamical decoupling sequence, which both amplifies and frequency-mixes target signals at arbitrary frequencies into the detection band of the dynamical decoupling protocol. We demonstrate this approach by using NV centers to detect both coherent and noisy nanoscale spin wave dynamics in a magnetic yttrium-iron-garnet (YIG) thin film over a broad frequency range. Our technique generalizes to other qubit platforms, providing a versatile framework for nanoscale spectroscopy across diverse physical and chemical systems.
This work combines theory and experiment to examine the mechanisms underlying the harmonic generation of magnons. We develop a nonlinear spin-wave framework that is directly analogous to harmonic generation in nonlinear optics, and combine it with scanning nitrogen-vacancy (NV) center magnetometry to image and quantify magnonic harmonic generation in a Ni81Fe19/Pt microstripe. Within this framework, the harmonic response arises from nonlinear magnetization dynamics localized at strongly inhomogeneous textures, such as the sample edges and domain walls, that act as anharmonic confining potentials. Scanning probe imaging confirms that the harmonic response is correspondingly nonuniform and concentrated near the sample edges. We measure an expected nonlinear power-law scaling, a systematic shift toward larger wavevector excitations at higher harmonic order, and a spin-selective response indicative of an increasingly chiral harmonic stray field. These results provide a microscopic understanding of magnonic harmonic generation and highlight its potential for engineering nonlinear functionality in magnonic systems.
Quantum sensors harness the high sensitivity of quantum systems to external perturbations to accurately measure various physical quantities. Among the quantum systems employed for sensing purposes, the nitrogen-vacancy (NV) defect in diamond has garnered considerable attention as a magnetometer. A single NV center can be integrated in a scanning probe microscope to build a highly sensitive imaging tool which is particularly adapted to the investigation of antiferromagnets. Two approaches are possible, either the measurement of small static stray fields or the detection of magnetic noise.For canted antiferromagnetic textures, like the cycloidal state in multiferroic bismuth ferrite, the NV center can probe the stray field produced by the uncompensated moments, revealing the presence of topological defects in the magnetic order at the surface of bulk single crystals [1].Alternatively, thermally activated spin waves confined in domain walls generate a magnetic noise to which the NV center is also sensitive. This property allows the localization of the domain walls, which was demonstrated in synthetic antiferromagnets [2].Besides the NV centers, new sensors are emerging as magnetic field probes like the boron vacancies in h-BN, which offer the possibilty to integrate a sensing layer inside a van der Waals heterostructure [3].[1] Finco et al., Physical Review Letters, 128, 187201 (2022)[2] Finco et al., Nature Communications 12, 767 (2021)[3] Kumar et al., Physical Review Applied, 18, L061002 (2022)
The nitrogen-vacancy (NV) defect center in diamond has demonstrated great capability for nanoscale magnetic sensing and imaging for both static and periodically modulated target fields. However, it remains a challenge to detect and image randomly fluctuating magnetic fields. Recent theoretical and numerical works have outlined detection schemes that exploit changes in decoherence of the detector spin as a sensitive measure for fluctuating fields. Here we experimentally monitor the decoherence of a scanning NV center in order to image the fluctuating magnetic fields from paramagnetic impurities on an underlying diamond surface. We detect a signal corresponding to roughly 800 μB in 2 s of integration time, without any control on the target spins, and obtain magnetic-field spectral information using dynamical decoupling techniques. The extracted spatial and temporal properties of the surface paramagnetic impurities provide insight to prolonging the coherence of near-surface qubits for quantum information and metrology applications.
Individual, scannable nitrogen vacancy (NV) centers in single crystal diamond nanostructures enable nanoscale, quantitative imaging of magnetic stray fields. Nevertheless, important parameters like distance between the NV center and the sample and the orientation of the NV high symmetry axis are often not known precisely and enter data evaluation as free fitting parameters. We here use scanning NV imaging on micro-patterned, perpendicularly magnetized stripes and discs. From these measurements, we directly infer NV - sample distance d_NV and the NV's azimuthal orientation without the need for an external vector magnet control. We determine d_NV = 31.5 nm, while we infer the azimuthal orientation with a precision of 3°. We additionally employ commercially available silicon needles to image the apex topography of our diamond nanostructures to detect surface contamination. Simultaneously, monitoring NV fluorescence as a function of the needle's position allows us to estimate the lateral placement of the NV inside the diamond nanostructure.