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arXiv:2606.28535

Dynamical decoupling of a quantum dot spin in a micropillar cavity for spin-multiphoton entanglement

H. Huet, P. R. Ramesh, R. Frantzeskakis, L. Couronné, P. Steindl, V. Guichard, M. Morassi, A. Lemaître, I. Sagnes, M. F. Doty, L. Lanco, D. A. Fioretto, S. C. Wein, P. Senellart, O. Krebs

quant-phSubmitted Jun 26, 2026• Announced Jun 30, 2026• 0 citations
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Abstract

Graph states of mutually entangled photons are key resources for quantum computation and communication and can be generated by leveraging the entanglement between a single resident spin and emitted photons from a charged semiconductor quantum dot (QD). This approach is intrinsically limited by the decoherence of the spin. We study how to mitigate this decoherence with dynamical decoupling of an electron spin in the weak transverse magnetic field regime using spin echo and Carr-Purcell-Meiboom-Gill (CPMG) techniques. Application of these techniques allows us to extend the coherence time of a spin by more than two orders of magnitude, extracting a $T_2^{CPMG}$ of $298\pm53$ ns. We further demonstrate that this technique is compatible with the generation of a spin-photon-photon entangled state at a high rate enabled by a micropillar cavity, with a 20% improvement in simulated state fidelity when using dynamical decoupling. These results pave the way for generating larger and more complex entangled states with QDs.

Related papers

Spin-Photon Entanglement and Quantum Optics with Single Quantum Dots.

John R. Schaibley

InAs quantum dots (QDs) can be used as optically coupled quantum storage devices for quantum information applications. The QD can be charged with a single electron, where the spin state (up or down) provides a long lived quantum bit (qubit). The QD's optically excited states are used to initialize, manipulate, and read out the electron spin state with laser pulses. However, most practical quantum information applications require many interacting qubits, forming a quantum network. Since QDs are based on semiconductor technology, and are compatible with standard nano-fabrication processing, there is promise that they can provide a solid state platform where a scalable quantum information architecture is realizable. We focus on scaling the QD system to multiple qubits using intermediate spin-photon entangled states. In this work, experimental and theoretical techniques are developed to study the QD-light matter interaction at the single photon level. Resonance fluorescence from a single QD is experimentally realized, and the single photon nature of the scattered radiation is verified through intensity correlation experiments. Transient fluorescence measurements on resonantly excited QDs are performed using time correlated single photon counting techniques to measure the excited state lifetime. High speed electro-optic modulators are used to time gate narrow bandwidth lasers, so that a QD can be driven under step-wise excitation, allowing for the direct observation of time-dependent optical Rabi oscillations. From these measurements, we are able to extract a decoherence rate which is consistent with the lifetime limit, indicating that pure dephasing is negligible in this system. These techniques are applied to the QD spin system to demonstrate a spin-photon entangled state, by performing correlation measurements on the spin and photon state in two bases. A lower bound on the entanglement fidelity of 0.59(4) is achieved, which exceeds the classical limit of 0.5 by more than two standard deviations. The entanglement fidelity is limited primarily by the finite timing resolution of available single photon detectors. Taking this into account, we achieve 84% of the apparatus limited fidelity. These spin-entangled photons can be used to mediate entanglement between distant QD spins, providing the basis of an optically coupled QD spin network.

•Jan 1, 2013•0 citations

Investigation of efficient spin-photon interfaces for the realisation of quantum networks

L. Huthmacher

Quantum networks lie at the heart of distributed quantum computing and secure quantum communication - research areas that have seen a strong increase of interest over the last decade. Their basic architecture consist of stationary nodes composed of quantum processors which are linked via photonic channels. The key requirement, and at the same time the most demanding challenge, is the efficient distribution of entanglement between distant nodes. The two ground states of single spins confined in self-assembled InGaAs quantum dots provide an effective two-level system for the implementation of quantum bits. Moreover, they offer strong transition dipole moments with outstanding photonic properties allowing for the realisation of close to ideal, high-bandwidth spin-photon interfaces. These properties are combined with the benefits of working in the solid state, such as scalability and integrability of devices, to form a promising candidate for the implementation of fast entanglement distribution. In this dissertation we provide the first implementation of a unit cell of a quantum network based on single electron spins in InGaAs. We use a probabilistic scheme based on spin-photon entanglement and the erasure of which path information to project the two distant spins into a maximally entangled Bell state. The successful generation of entanglement is verified through a reconstruction of the final two-spin state and we achieve an average fidelity of $61.6\pm2.3\%$ at a record-high generation rate of $5.8\,\mathrm{kHz}$. One of the main constraints to the achieved fidelity is the limited coherence of the electron spin. We show that it can be extended by three orders of magnitude through decoupling techniques and develop a new measurement technique, allowing us to investigate the origins of the decoherence which has previously been obscured by nuclear feedback processes. Our results evidence that further extension of coherence is ultimately limited by intrinsic mechanisms closely related to local strain due to the growth method of self-assembled quantum dots. After establishing the intrinsic limits to the electron coherence we investigate the coherence properties of the single hole spin as an alternative two-level system with the potential for higher coherence times. We show that the hole spin coherence is indeed superior to the one of the electron and realise the first successful dynamic decoupling scheme implemented in these systems. We find that the decoherence at low external magnetic fields is still governed by coupling to the nuclear spins whereas it is dominated by electrical noise for fields exceeding a few Tesla. This noise source is extrinsic to the quantum dots and a better understanding offers the potential for further improvement of the coherence time. The findings of this work present a complete study of the coherence of the charge carriers in self-assembled quantum dots and provide the knowledge needed to improve the implementation of a quantum-dot based quantum network. In particular, the combination of spin-spin entanglement and the hole coherence times enable further research towards multidimensional photonic cluster states.

•Apr 6, 2018•0 citations

Protocol for generating multiphoton entangled states from quantum dots in the presence of nuclear spin fluctuations

Emil V. Denning, Jake Iles-Smith, Dara P. S. McCutcheon +1 more

Multiphoton entangled states are a crucial resource for many applications in quantum information science. Semiconductor quantum dots offer a promising route to generate such states by mediating photon-photon correlations via a confined electron spin, but dephasing caused by the host nuclear spin environment typically limits coherence (and hence entanglement) between photons to the spin ${T}_{2}^{*}$ time of a few nanoseconds. We propose a protocol for the deterministic generation of multiphoton entangled states that is inherently robust against the dominating slow nuclear spin environment fluctuations, meaning that coherence and entanglement is instead limited only by the much longer spin ${T}_{2}$ time of microseconds. Unlike previous protocols, the present scheme allows for the generation of very low error probability polarization encoded three-photon GHZ states and larger entangled states, without the need for spin echo or nuclear spin calming techniques.

arXiv:1706.02486•Physical Review A•Dec 26, 2017•7 citations

Extending the Versatility and Coherence of Spin-Photon Entanglement Generation with Semiconductor Quantum Dots

Polluri Ramesh

Quantum computation using photons offers one possible route towards the long-standing goal of scalable, fault-tolerant quantum computing. Within this realm, measurement-based quantum computing offers a promising approach exploiting many of the advantages of photons. Implementing photonic measurement-based architectures relies upon the deterministic generation of graph states composed of many entangled photons. Semiconductor quantum dots (QDs) are sources of indistinguishable single photons and hosts of solid-state spins, marking them desirable platforms for controlled entanglement generation. Such a platform consisting of a single charged QD coupled to a photonic cavity has been proven for the generation of multipartite spin-photon graph states. This dissertation will present advancements in the versatility and coherence of such entanglement generation. First, background on quantum dots, single photon generation, spin control, and entanglement will be introduced. Then, sources of error and decoherence will be addressed using control of the hole g-factor and dynamical decoupling techniques. The aim of versatility is advanced through results on the generation of four-partite graph states with on-demand reconfigurability of the type of state produced. Finally, a different paradigm using quantum dot molecules will be introduced, and novel estimation of important physical parameters in this system is developed.

•Jan 5, 2026•0 citations

Ultrafast optical control of individual electron and hole spin qubits: entanglement between a single quantum dot electron spin and a downconverted 1560-nm single photon

Kristiaan De Greve, Peter L. McMahon, Leo Yu +14 more

Individual electron and hole quantum dot spin qubits can be coherently manipulated using picosecond modelocked laser pulses; an all-optical spin-echo was implemented that decouples slow environmental changes. While dephasing and decoherence mechanisms for electrons and holes are intrinsically different, similar qualitative results are obtained, except for dynamic nuclear polarization effects that affect the controllability of electrons. In addition, we demonstrate spin-photon entanglement in a charged InAs quantum dot, using an ultrafast downconversion technique that converts a single, spontaneously emitted photon at 900 nm into a 1560 nm photon with picosecond timing resolution. This ultrafast conversion technique allows quantum erasure of which-path frequency information in the spontaneous emission process.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Mar 29, 2013•1 citation

Extending the time of coherent optical response in ensemble of singly-charged InGaAs quantum dots

A. N. Kosarev, A. V. Trifonov, I. A. Yugova +10 more

The ability to extend the time scale of the coherent optical response from large ensembles of quantum emitters is highly appealing for applications in quantum information devices. In semiconductor nanostructures, spin degrees of freedom can be used as auxiliary, powerful tools to modify the coherent optical dynamics. Here, we apply this approach to negatively charged (In,Ga)As/GaAs self-assembled quantum dots which are considered as excellent quantum emitters with robust optical coherence and high bandwidth. We study 3-pulse spin-dependent photon echoes subject to moderate transverse magnetic fields up to 1 T. We demonstrate that the timescale of coherent optical response can be extended by at least an order of magnitude by the field. Without magnetic field, the photon echo decays with $T_ 2$ = 0.45 ns which is determined by the radiative lifetime of trions $T_1$ = 0.27 ns. In the presence of the transverse magnetic field, the decay of the photon echo signal is given by spin dephasing time of the ensemble of resident electrons $T_{2,e}$ ~ 4 ns. We demonstrate that the non-zero transverse g-factor of the heavy holes in the trion state plays a crucial role in the temporal evolution and magnetic field dependence of the long-lived photon echo signal.

arXiv:2201.09383•Jan 23, 2022•0 citations
Graph states of mutually entangled photons are key resources for quantum computation and communication and can be generated by leveraging the entanglement between a single resident spin and emitted photons from a charged semiconductor quantum dot (QD). This approach is intrinsically limited by the decoherence of the spin. We study how to mitigate this decoherence with dynamical decoupling of an electron spin in the weak transverse magnetic field regime using spin echo and Carr-Purcell-Meiboom-Gill (CPMG) techniques. Application of these techniques allows us to extend the coherence time of a spin by more than two orders of magnitude, extracting a T2CPMGT_2^{CPMG}T2CPMG​ of 298±53298\pm53298±53 ns. We further demonstrate that this technique is compatible with the generation of a spin-photon-photon entangled state at a high rate enabled by a micropillar cavity, with a 20% improvement in simulated state fidelity when using dynamical decoupling. These results pave the way for generating larger and more complex entangled states with QDs.
InAs quantum dots (QDs) can be used as optically coupled quantum storage devices for quantum information applications. The QD can be charged with a single electron, where the spin state (up or down) provides a long lived quantum bit (qubit). The QD's optically excited states are used to initialize, manipulate, and read out the electron spin state with laser pulses. However, most practical quantum information applications require many interacting qubits, forming a quantum network. Since QDs are based on semiconductor technology, and are compatible with standard nano-fabrication processing, there is promise that they can provide a solid state platform where a scalable quantum information architecture is realizable. We focus on scaling the QD system to multiple qubits using intermediate spin-photon entangled states. In this work, experimental and theoretical techniques are developed to study the QD-light matter interaction at the single photon level. Resonance fluorescence from a single QD is experimentally realized, and the single photon nature of the scattered radiation is verified through intensity correlation experiments. Transient fluorescence measurements on resonantly excited QDs are performed using time correlated single photon counting techniques to measure the excited state lifetime. High speed electro-optic modulators are used to time gate narrow bandwidth lasers, so that a QD can be driven under step-wise excitation, allowing for the direct observation of time-dependent optical Rabi oscillations. From these measurements, we are able to extract a decoherence rate which is consistent with the lifetime limit, indicating that pure dephasing is negligible in this system. These techniques are applied to the QD spin system to demonstrate a spin-photon entangled state, by performing correlation measurements on the spin and photon state in two bases. A lower bound on the entanglement fidelity of 0.59(4) is achieved, which exceeds the classical limit of 0.5 by more than two standard deviations. The entanglement fidelity is limited primarily by the finite timing resolution of available single photon detectors. Taking this into account, we achieve 84% of the apparatus limited fidelity. These spin-entangled photons can be used to mediate entanglement between distant QD spins, providing the basis of an optically coupled QD spin network.
Quantum networks lie at the heart of distributed quantum computing and secure quantum communication - research areas that have seen a strong increase of interest over the last decade. Their basic architecture consist of stationary nodes composed of quantum processors which are linked via photonic channels. The key requirement, and at the same time the most demanding challenge, is the efficient distribution of entanglement between distant nodes. The two ground states of single spins confined in self-assembled InGaAs quantum dots provide an effective two-level system for the implementation of quantum bits. Moreover, they offer strong transition dipole moments with outstanding photonic properties allowing for the realisation of close to ideal, high-bandwidth spin-photon interfaces. These properties are combined with the benefits of working in the solid state, such as scalability and integrability of devices, to form a promising candidate for the implementation of fast entanglement distribution. In this dissertation we provide the first implementation of a unit cell of a quantum network based on single electron spins in InGaAs. We use a probabilistic scheme based on spin-photon entanglement and the erasure of which path information to project the two distant spins into a maximally entangled Bell state. The successful generation of entanglement is verified through a reconstruction of the final two-spin state and we achieve an average fidelity of 61.6±2.3%61.6\pm2.3\%61.6±2.3% at a record-high generation rate of 5.8 kHz5.8\,\mathrm{kHz}5.8kHz. One of the main constraints to the achieved fidelity is the limited coherence of the electron spin. We show that it can be extended by three orders of magnitude through decoupling techniques and develop a new measurement technique, allowing us to investigate the origins of the decoherence which has previously been obscured by nuclear feedback processes. Our results evidence that further extension of coherence is ultimately limited by intrinsic mechanisms closely related to local strain due to the growth method of self-assembled quantum dots. After establishing the intrinsic limits to the electron coherence we investigate the coherence properties of the single hole spin as an alternative two-level system with the potential for higher coherence times. We show that the hole spin coherence is indeed superior to the one of the electron and realise the first successful dynamic decoupling scheme implemented in these systems. We find that the decoherence at low external magnetic fields is still governed by coupling to the nuclear spins whereas it is dominated by electrical noise for fields exceeding a few Tesla. This noise source is extrinsic to the quantum dots and a better understanding offers the potential for further improvement of the coherence time. The findings of this work present a complete study of the coherence of the charge carriers in self-assembled quantum dots and provide the knowledge needed to improve the implementation of a quantum-dot based quantum network. In particular, the combination of spin-spin entanglement and the hole coherence times enable further research towards multidimensional photonic cluster states.
Multiphoton entangled states are a crucial resource for many applications in quantum information science. Semiconductor quantum dots offer a promising route to generate such states by mediating photon-photon correlations via a confined electron spin, but dephasing caused by the host nuclear spin environment typically limits coherence (and hence entanglement) between photons to the spin T2∗{T}_{2}^{*}T2∗​ time of a few nanoseconds. We propose a protocol for the deterministic generation of multiphoton entangled states that is inherently robust against the dominating slow nuclear spin environment fluctuations, meaning that coherence and entanglement is instead limited only by the much longer spin T2{T}_{2}T2​ time of microseconds. Unlike previous protocols, the present scheme allows for the generation of very low error probability polarization encoded three-photon GHZ states and larger entangled states, without the need for spin echo or nuclear spin calming techniques.
Quantum computation using photons offers one possible route towards the long-standing goal of scalable, fault-tolerant quantum computing. Within this realm, measurement-based quantum computing offers a promising approach exploiting many of the advantages of photons. Implementing photonic measurement-based architectures relies upon the deterministic generation of graph states composed of many entangled photons. Semiconductor quantum dots (QDs) are sources of indistinguishable single photons and hosts of solid-state spins, marking them desirable platforms for controlled entanglement generation. Such a platform consisting of a single charged QD coupled to a photonic cavity has been proven for the generation of multipartite spin-photon graph states. This dissertation will present advancements in the versatility and coherence of such entanglement generation. First, background on quantum dots, single photon generation, spin control, and entanglement will be introduced. Then, sources of error and decoherence will be addressed using control of the hole g-factor and dynamical decoupling techniques. The aim of versatility is advanced through results on the generation of four-partite graph states with on-demand reconfigurability of the type of state produced. Finally, a different paradigm using quantum dot molecules will be introduced, and novel estimation of important physical parameters in this system is developed.
Individual electron and hole quantum dot spin qubits can be coherently manipulated using picosecond modelocked laser pulses; an all-optical spin-echo was implemented that decouples slow environmental changes. While dephasing and decoherence mechanisms for electrons and holes are intrinsically different, similar qualitative results are obtained, except for dynamic nuclear polarization effects that affect the controllability of electrons. In addition, we demonstrate spin-photon entanglement in a charged InAs quantum dot, using an ultrafast downconversion technique that converts a single, spontaneously emitted photon at 900 nm into a 1560 nm photon with picosecond timing resolution. This ultrafast conversion technique allows quantum erasure of which-path frequency information in the spontaneous emission process.
The ability to extend the time scale of the coherent optical response from large ensembles of quantum emitters is highly appealing for applications in quantum information devices. In semiconductor nanostructures, spin degrees of freedom can be used as auxiliary, powerful tools to modify the coherent optical dynamics. Here, we apply this approach to negatively charged (In,Ga)As/GaAs self-assembled quantum dots which are considered as excellent quantum emitters with robust optical coherence and high bandwidth. We study 3-pulse spin-dependent photon echoes subject to moderate transverse magnetic fields up to 1 T. We demonstrate that the timescale of coherent optical response can be extended by at least an order of magnitude by the field. Without magnetic field, the photon echo decays with T2T_ 2T2​ = 0.45 ns which is determined by the radiative lifetime of trions T1T_1T1​ = 0.27 ns. In the presence of the transverse magnetic field, the decay of the photon echo signal is given by spin dephasing time of the ensemble of resident electrons T2,eT_{2,e}T2,e​ ~ 4 ns. We demonstrate that the non-zero transverse g-factor of the heavy holes in the trion state plays a crucial role in the temporal evolution and magnetic field dependence of the long-lived photon echo signal.