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arXiv:2606.07458

Collective emission of subwavelengths atom-like emitter arrays in the presence of inhomogeneous broadening

Uri Israeli, Shahar Levi, Sagi Ben-Avi, Ada Kransnovsky, Daniel Silvian, Shlomo Winberg, Rivka Bekenstein

physics.opticsphysics.atom-phquant-phSubmitted Jun 5, 2026• Announced Jun 8, 2026• 0 citations
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Abstract

Quantum metasurfaces comprised of subwavelength atomic arrays emerged as a promising platform for enhanced atom-photon interaction. However, realizing such a system with solid-state emitters has been considered impractical due to strong inhomogeneous broadening, which was expected to suppress the photon-mediated interactions that underpin collective emission. Here we report the observation of collective emission from subwavelength arrays of silicon-vacancy centres in diamond -- solid-state emitters whose inhomogeneous broadening exceeds the natural linewidth by two orders of magnitude -- demonstrating that collective effects such as resonance shifts, modified decay rates and directional coherent emission survive this disorder. A crucial enabling element is the implantation of a high density of silicon ions at each array site. This creates so-called superatoms, local ensembles that probabilistically achieve frequency matching across the array and enhance the collective response. We support our observations with a theoretical analysis explaining the mechanisms that preserve the collective effects even in the presence of inhomogeneity. These observations have direct implications for the realization of subwavelength arrays in any solid-state system, paving the way for quantum-emitter metasurfaces that are naturally integrated into nanophotonic environments.

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Quantum metasurfaces comprised of subwavelength atomic arrays emerged as a promising platform for enhanced atom-photon interaction. However, realizing such a system with solid-state emitters has been considered impractical due to strong inhomogeneous broadening, which was expected to suppress the photon-mediated interactions that underpin collective emission. Here we report the observation of collective emission from subwavelength arrays of silicon-vacancy centres in diamond -- solid-state emitters whose inhomogeneous broadening exceeds the natural linewidth by two orders of magnitude -- demonstrating that collective effects such as resonance shifts, modified decay rates and directional coherent emission survive this disorder. A crucial enabling element is the implantation of a high density of silicon ions at each array site. This creates so-called superatoms, local ensembles that probabilistically achieve frequency matching across the array and enhance the collective response. We support our observations
with a theoretical analysis explaining the mechanisms that preserve the collective effects even in the presence of inhomogeneity. These observations have direct implications for the realization of subwavelength arrays in any solid-state system, paving the way for quantum-emitter metasurfaces that are naturally integrated into nanophotonic environments.
An efficient simulation framework is proposed to model collective emission in disordered ensembles of quantum emitters. Using a cumulant expansion approach, the computational complexity scales polynomially as opposed to exponentially with the number of emitters, enabling Monte Carlo sampling over a large number of realizations. The framework is applied to model negatively charged silicon-vacancy (SiV−^{-}−) centers inside diamond. Incorporating spatial disorder and inhomogeneous broadening, we obtain statistically averaged responses over hundreds of SiV−^{-}− clusters. These simulations reveal two signatures of collective behavior. First, dynamics of fully inverted clusters show that superradiant emission occurs only with sufficiently large emitter number and high quantum efficiency. Unlike ideal Dicke superradiance, the burst is substantially suppressed by strong near-field dipole-dipole interaction, consistent with existing theoretical predictions. Second, under continuous-wave excitation we compute photoluminescence-excitation spectra, which exhibit interaction-induced broadening in the distribution of resonance peaks. The corresponding density of states also displays a non-zero skewness. Overall, by incorporating realistic inhomogeneities in emitter clusters, our framework is able to predict statistics for disordered ensembles that can be compared to experiments directly. Our approach generalizes to other types of emitters, including atoms, molecules, and quantum dots, thus providing a practical tool for analyzing collective behavior in realistic quantum systems.
When quantum emitters couple indistinguishably to light, they can synchronize into a collective light matter system with radiative properties profoundly different from those of independent particles. To date, the resulting collective effects have largely been confined to point like or homogeneous ensembles. Here, we open access to a qualitatively new collective regime by realizing geometrically ordered, spatially extended atom arrays with subwavelength spacing. This establishes a fundamentally new platform in which collective emission is no longer confined to a single Dicke mode but instead emerges from an ordered network of photon mediated interactions. We find that 2D atom arrays undergo strong super and subradiant emission. Despite subwavelength spacing, we achieve site resolved imaging and directly observe the buildup of spatial correlations, demonstrating the transformation of cooperative decay into a strongly correlated many-body process. We observe extensive scaling of superradiance, uncover superradiant revivals, and reveal the ferromagnetic nature of superradiance and the antiferromagnetic nature of subradiance. Our results realize a novel programmable platform for exploring and utilizing dissipative many-body quantum physics, opening new possibilities for photon capture, storage, and atom photon entanglement.
Conventional approaches to light-matter interactions rely on engineering photonic density of states. More recently, tailoring the spatial geometry of atoms or emitters themselves has emerged as a powerful and complementary route to control collective radiative properties. Here we experimentally realize a geometry-engineered ensemble of rare-earth ions by fabricating a periodic array of subwavelength gold nanoholes on lithium niobate implanted with thulium ions, forming a semi-two-dimensional array of quantum emitters embedded in a high-index crystalline thin film. The hybrid structure can simultaneously support localized and lattice plasmon resonances from the metallic array and collective atomic resonances from the ion ensemble. Using time-resolved photoluminescence and temperature-dependent measurements, we observe enhanced radiative emission attributed to collective atomic effects mediated by the nanohole lattice, distinct from single-emitter Purcell enhancement. Our results demonstrate a new regime of light-matter interaction opening a pathway toward broadband and scalable, geometry-controlled quantum optical interfaces in solid-state platforms.
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