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arXiv:2605.21925 · Physical Review Research

Nonclassical Cutoff Fluctuations in Squeezed-Light-Driven High-Harmonic Generation

Tsendsuren Khurelbaatar, R. T. Sang, Igor Litvinyuk

quant-phSubmitted May 21, 2026• Announced May 22, 2026• 0 citations
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Abstract

Strong-field high-harmonic generation (HHG) is conventionally described semiclassically, with the driving laser treated as a classical field. This approximation becomes insufficient in nanoscale interaction geometries, where extreme spatial confinement raises the vacuum-field amplitude to the ~10^-2 level relative to the driving-field amplitude. When the quantum fluctuations of the driving field are redistributed between conjugate quadratures by squeezing, they can be directly imprinted onto macroscopic HHG observables. To model this interaction, we employ a Wigner phase-space approach that maps the quantum-optical driver onto a stochastic ensemble of time-dependent Schrodinger equation realizations. Although each realization remains classically simulable, the sub-vacuum quadrature covariance structure of squeezed states cannot be reproduced by any field admitting a non-negative Glauber-Sudarshan P-representation. Within this single-mode Gaussian framework, we show that amplitude squeezing suppresses the shot-to-shot variance of the HHG cutoff below the standard quantum limit (SQL). To leading order in the vacuum-to-driver ratio, the normalized cutoff variance decays exponentially with the squeezing parameter, independent of the absolute vacuum-field amplitude and therefore robust against uncertainties in the effective nanoscale mode volume. A subleading phase-noise contribution from the anti-squeezed quadrature produces a variance minimum near r_opt ~ 1.6, providing a concrete experimental target. These results establish the HHG cutoff variance ratio as a nonlinear, self-calibrating Heisenberg witness in which sub-SQL scaling directly reflects the redistribution of quantum uncertainty in the driving field.

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Strong-field high-harmonic generation (HHG) is conventionally described semiclassically, with the driving laser treated as a classical field. This approximation becomes insufficient in nanoscale interaction geometries, where extreme spatial confinement raises the vacuum-field amplitude to the ~10^-2 level relative to the driving-field amplitude. When the quantum fluctuations of the driving field are redistributed between conjugate quadratures by squeezing, they can be directly imprinted onto macroscopic HHG observables. To model this interaction, we employ a Wigner phase-space approach that maps the quantum-optical driver onto a stochastic ensemble of time-dependent Schrodinger equation realizations. Although each realization remains classically simulable, the sub-vacuum quadrature covariance structure of squeezed states cannot be reproduced by any field admitting a non-negative Glauber-Sudarshan P-representation. Within this single-mode Gaussian framework, we show that amplitude squeezing suppresses the shot-to-shot variance of the HHG cutoff below the standard quantum limit (SQL). To leading order in the vacuum-to-driver ratio, the normalized cutoff variance decays exponentially with the squeezing parameter, independent of the absolute vacuum-field amplitude and therefore robust against uncertainties in the effective nanoscale mode volume. A subleading phase-noise contribution from the anti-squeezed quadrature produces a variance minimum near r_opt ~ 1.6, providing a concrete experimental target. These results establish the HHG cutoff variance ratio as a nonlinear, self-calibrating Heisenberg witness in which sub-SQL scaling directly reflects the redistribution of quantum uncertainty in the driving field.
In recent years, strong-field processes such as high-order harmonic generation (HHG) and above-threshold ionization driven by nonclassical states of light have become an increasingly popular field of study. The theoretical modeling of these processes often applies an approximate phase-space expansion of the nonclassical driving field in terms of coherent states, which has been shown to accurately predict the harmonic spectrum. However, its accuracy for the computation of quantum optical observables like the degree of squeezing and photon statistics has not been thoroughly considered. In this work, we introduce this approximative phase-space description and discuss its accuracy, and we find that it mischaracterizes the quantum optical properties of the driving laser by making it an incoherent mixture of classical states. We further show that this error in the driving field description maps onto the light emitted from HHG, as neither sub-Poissonian photon statistics nor quadrature squeezing below vacuum fluctuations can be captured by the approximative phase-space description. Lastly, to benchmark the approximative phase-space description, we consider the quantum HHG from a one-band model, which yields an exact analytical solution. Using the approximative phase-space representation with this specific model, we find a small quantitative error in the quadrature variance of the emitted field that scales with pulse duration and emitter density. Our results show that using this approximative phase-space description can mischaracterize quantum optical observables. Attributing physical meaning to such results should therefore be accompanied by a quantitative analysis of the error.
High-harmonic generation (HHG) is a prototypical strong-field process in which intense light drives matter to emit radiation at integer multiples of the driving frequency. Extending HHG into the quantum-optical regime offers new opportunities to probe and control strongly nonlinear light-matter interactions using nonclassical states of light. Yet describing this regime requires a fully quantum treatment of the correlated electron-photon dynamics, which becomes computationally challenging for broadband, strongly squeezed fields. Here we solve the quantum-electrodynamical dynamics of a two-level system driven by bright squeezed vacuum in a converged multimode Hilbert space. Both the driving field and emitted harmonics are fully quantized, with the light-matter interaction treated nonperturbatively. This enables direct access to the multimode quantum state and its higher-order correlations beyond semiclassical sampling or perturbative descriptions. We show that squeezed-vacuum driving produces harmonic emission with qualitatively distinct second- and third-order photon correlations compared with coherent excitation. Moreover, back-action from the driven emitter strongly reshapes the incident squeezed field, generating pronounced Wigner-function negativities that evolve on attosecond timescales. Our results establish a fully quantum framework for broadband strong-field dynamics with squeezed light and provide a route to predicting and interpreting quantum-HHG experiments and their extension to more complex emitters.
High harmonic generation (HHG) is a highly nonlinear optical process in which radiation from a strong driving field is up-converted into its high-order harmonics. In atomic systems, this nonlinearity manifests itself through the intensity scaling of the emitted harmonics with the driving field strength. Despite the highly nonlinear nature of HHG, when the driving field is prepared in a classical Gaussian state and atomic depletion remains negligible, the quantum statistical properties of the generated harmonics retains classical Gaussian quantum statistics. Driving HHG with bright squeezed vacuum (BSV) light challenges this paradigm, as its enhanced field fluctuations can modify the statistical properties of the generated harmonics. In this work, we investigate the conditions under which BSV-driven HHG gives rise to non-classical Gaussian states, and identify the regimes where this Gaussian description breaks down. For bichromatic driving by a strong coherent field at frequency ωωω and a perturbative BSV field at 2ω2ω2ω, the even-harmonic response is approximately linear in the BSV quadrature, leading to non-classical multimode Gaussian entanglement in the harmonic field. We show that this state can be described as a distributed collective squeezed mode over the even-harmonic manifold, and characterize its covariance matrix, entanglement structure, and quantum teleportation fidelity as an operational benchmark. Our results highlight the potential of non-classically driven HHG as a platform for engineering Gaussian and non-Gaussian states of light in the extreme ultraviolet regime.
We analyse the quadrature variance of high harmonic photons, using a simplified quantum optical model associated with high-harmonic generation (HHG) in the case of an elementary quantum source, modelled with a two-level atom. Assuming classical excitation, we find weak, oscillating (anti-)squeezing in the scattered radiation, with the variance-spectrum following similar evolution to the photon-number spectrum. Investigating the phase-relations, we conclude that the squeezed states of each mode are {most of the time{ close to being amplitude-squeezed, and squeezed states appear periodically within each attosecond pulse. We have also defined an approximate single noise-ellipse based on the collective field, and its analysis shows that it is anti-squeezed.
Quantum-optical descriptions of strong-field processes have attracted significant attention in recent years. Typically, the theoretical modeling has been conducted in the Schrödinger picture, where results are only obtainable under certain approximations, while, in contrast, the Heisenberg picture has remained relatively unexplored. In this work, we develop an accurately controlled perturbative expansion of the time-evolution operator in the Heisenberg picture and derive beyond-semiclassical corrections to the emitter dynamics due to the coupling to the quantized electromagnetic field, capturing effects of the quantum fluctuations present in the latter. We focus on high-order harmonic generation (HHG), where the approach is accurate in parameter regimes of current interest and it gives closed-form expressions for key observables. This formulation not only simplifies numerical calculations compared to the Schrödinger-picture approach but also provides a clear correspondence between nonclassical features of the emitted light and the underlying induced dynamics of the generating medium including quantum fluctuations. Moreover, the Heisenberg framework naturally yields scaling relations with the number of independent emitters, enabling us to assess whether nonclassical behavior should persist under typical experimental conditions involving large emitter ensembles. Interestingly, we find that the degree of squeezing increases with the number of emitters, whereas the photon statistics approaches a classical Poissonian distribution in the many-emitter limit. We also find that the beyond-semiclassical emitter dynamics significantly enhances the degree of squeezing of the emitted light. Our work advances the theoretical understanding of quantum-optical HHG and introduces an accessible and well-controlled framework to describe realistic experiments.
Recently, the intersection of quantum optics and attosecond physics has attracted growing interest. Here, we study the quantum optical signatures of high-harmonic generation (HHG) from solid-state material driven by squeezed coherent states. We find that squeezed coherent states can either enhance or suppress the HHG yields compared to that driven by coherent light, depending on the photon bunching or antibunching characteristics of driving light. The analysis on semiclassical trajectories indicates that the amplitude fluctuation alters the recombination energy, while the phase fluctuation affects the birth and recombination time of electron-hole pairs. By calculating the Husimi Q distributions of HHG, we demonstrate that the squeezing of the two conjugate quadratures of driving light asymmetrically influence the squeezing phase of harmonics. Surprisingly, we find that even under coherent driving, the harmonics still exhibit squeezing due to the highly nonlinear response of solid-state HHG, which was overlooked previously. Numerical calculations of the Mandel parameter are performed to characterize the photon statistics of emitted HHG arising from different microscopic mechanisms. The results indicate that intraband radiation can exhibit a super-Poissonian distribution, while interband emission exhibits sub-Poissonian distribution under coherent driving.