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arXiv:2604.27567

Experimental detection of entanglement in multimode Gaussian states from high-order intensity correlation moments

Ze-Shan He, Yukuan Zhao, Hao-Shu Tian, Kai Sun, Xiao-Ye Xu, Chuan-Feng Li, Guang-Can Guo

quant-phSubmitted Apr 30, 2026• Announced May 1, 2026• 0 citations
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Abstract

Quantum universal invariants of a Gaussian state's covariance matrix, which can be derived from intensity correlation moments, have been adopted to characterize the entanglement properties of Gaussian states via the positive partial transpose criterion, also known as the Peres-Horodecki separability criterion. Such intensity correlation moments enable the extraction of information about the covariance matrix without the need for a coherent local oscillator. Here, we experimentally detect the entanglement properties of multimode Gaussian states using high-order\,(up to sixth-order) intensity correlation moments. These multimode Gaussian states are prepared via spontaneous and cascaded parametric down-conversion pumped by a high-peak-energy pulsed laser. Their intensity correlation moments are measured using a pseudo-photon-number-resolving detector constructed through spatial multiplexing of 32 threshold superconducting nanowire single photon detectors. This method is successfully demonstrated for two-mode and three-mode Gaussian states and can be extended to $N$-mode Gaussian states with $N>3$.

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17 pages, 7 figures

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Quantum universal invariants of general N -beam Gaussian fields are investigated from the point of view of fields' intensity moments. A method that uniquely links these invariants, including the global and marginal fields' purities, to intensity moments is suggested. Determination of these invariants identifies the Gaussian states including their quantum correlations. In particular, the Peres-Horodecki separability criterion is reformulated in terms of quantum universal invariants, and consequently in terms of experimental intensity moments, offering a practical tool for determining the entanglement or separability of these states. The approach is experimentally demonstrated by determining the invariants of noisy symmetric three-beam Gaussian states using photon-number resolved measurements. Furthermore, their entanglement properties are analyzed and characterized.
Gaussian states are ubiquitous in quantum optics and information processing, and it is essential to have effective tools for their characterization. One such tool is a photon-number-resolving detector, and the simplest configuration involves counting the total number of photons in the state to be characterized. This motivates the following question: What properties of a multimode Gaussian state are determined by the signal from one detector that measures the total number of photons up to some bound? We find that if the Gaussian state occupies SSS modes and the probabilities of nnn photons for all $n\ensuremath{\le}8S$ are known, then we can determine the spectrum of the Gaussian covariance matrix and the magnitude of the displacements in each eigenspace of the covariance matrix. Nothing more can be learned, even if all photon-number probabilities are known. When the state is pure, the covariance matrix spectrum determines the squeezing parameters of the state.
Quantum correlations of symmetric three-beam Gaussian states are analyzed using their quantum universal invariants. These invariants, one-, two-, and three-beam purities, are expressed in terms of the beams’ intensity moments up to sixth order. The three-beam symmetric Gaussian states with varying amounts of the noise are experimentally generated using entangled photon pairs from down-conversion, their invariants are determined, and their quantum correlations are quantified. The coexistence of bipartite and tripartite entanglement and genuine tripartite entanglement is observed in these states that resemble the noisy GHZ/W states.
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Very recently, strongly non-Gaussian states have been observed via a direct three-mode spontaneous parametric down-conversion in a superconducting cavity [Phys. Rev. X 10, 011011 (2020)]. The created multiphoton non-Gaussian correlations are attractive and useful for various quantum information tasks. However, how to detect and classify multipartite non-Gaussian entanglement has not yet been completely understood. Here, we present an experimentally practical method to characterize continuous-variable multipartite non-Gaussian entanglement, by introducing a class of nonlinear squeezing parameters involving accessible higher-order moments of phase-space quadratures. As these parameters can depend on arbitrary operators, we consider their analytical optimization over a set of practical measurements, in order to detect different classes of multipartite non-Gaussian entanglement ranging from fully separable to fully inseparable. We demonstrate that the nonlinear squeezing parameters act as an excellent approximation to the quantum Fisher information within accessible third-order moments. The level of the nonlinear squeezing quantifies the metrological advantage provided by those entangled states. Moreover, by analyzing the above-mentioned experiment, we show that our method can be readily used to confirm fully inseparable tripartite non-Gaussian entangled states by performing a limited number of measurements without requiring full knowledge of the quantum state.