Spin squeezing serves as both a fundamental witness of quantum entanglement and a critical resource for quantum-enhanced metrology. While generating substantial spin squeezing in finite-range interacting systems remains challenging, such capability is important for advancing quantum technologies. In this work, we develop an optimal control strategy for achieving enhanced spin squeezing in a two-dimensional XX model with dipolar interactions. Leveraging rotor-spin-wave theory for periodic boundary conditions, we circumvent computational bottlenecks to explore control strategies at unprecedented scales. Remarkably, optimizing a single collective transverse field is sufficient to achieve substantial squeezing enhancement, exceeding the two-axis-twisting benchmark. The optimized control field achieves this breakthrough by dynamically suppressing inter-subspace mixing induced by the finite-range interactions, thereby confining the system evolution predominantly within the maximal spin subspace. We further extend rotor-spin-wave theory to open boundary conditions and incorporate dephasing noise, providing a scalable framework for realistic systems. Under these conditions, the optimized protocol remains effective, highlighting its robustness and suitability for experimental implementation.
Spin squeezing serves as both a fundamental witness of quantum entanglement and a critical resource for quantum-enhanced metrology. While generating substantial spin squeezing in finite-range interacting systems remains challenging, such capability is important for advancing quantum technologies. In this work, we develop an optimal control strategy for achieving enhanced spin squeezing in a two-dimensional XX model with dipolar interactions. Leveraging rotor-spin-wave theory for periodic boundary conditions, we circumvent computational bottlenecks to explore control strategies at unprecedented scales. Remarkably, optimizing a single collective transverse field is sufficient to achieve substantial squeezing enhancement, exceeding the two-axis-twisting benchmark. The optimized control field achieves this breakthrough by dynamically suppressing inter-subspace mixing induced by the finite-range interactions, thereby confining the system evolution predominantly within the maximal spin subspace. We further extend rotor-spin-wave theory to open boundary conditions and incorporate dephasing noise, providing a scalable framework for realistic systems. Under these conditions, the optimized protocol remains effective, highlighting its robustness and suitability for experimental implementation.
Spin squeezing is both a fundamental witness of quantum entanglement and a key resource for quantum-enhanced metrology. While all-to-all interactions provide a paradigmatic route to generate spin squeezing, many programmable quantum simulators naturally realize finite-range interactions that induce coupling between collective spin dynamics and finite-momentum spin-wave modes, thereby degrading the achievable squeezing. Here we develop an optimization-based global-control strategy for enhancing spin squeezing in a two-dimensional XX model with dipolar interactions. By combining rotor-spin-wave theory with an extension to open boundary conditions, we enable efficient optimization of control protocols for large finite-range interacting systems. We show that a single collective transverse field generates squeezing beyond the conventional two-axis-twisting benchmark across system sizes accessible to numerical benchmarking. The optimized dynamics exploits squeezing-axis reorientation while suppressing spin-wave excitations, thereby stabilizing strong squeezing over extended times. We further implement the optimized protocol in a two-dimensional Rydberg-atom array and experimentally observe enhanced, long-lived spin squeezing in good agreement with theory.
Scalable spin squeezing in two-dimensional arrays of dipolar large-S spins
Controlling the quantum many-body state of arrays of qudits, possessing a large local Hilbert space, opens the path to a broad range of possibilities for many-particle entanglement, interesting both for fundamental quantum science, as well as for potential metrological applications. In this work we theoretically show that the spin-spin interactions realized in two-dimensional Mott insulators of large-spin magnetic atoms (such as Cr, Er or Dy) lead to scalable spin squeezing along the non-equilibrium unitary evolution initialized in a coherent spin state. An experimentally relevant perturbation to the collective squeezing dynamics is offered by a quadratic Zeeman shift, which leads instead to squeezing of individual spins. Making use of a truncated cumulant expansion for the quantum fluctuations of the spin array, we show that, for sufficiently small quadratic shifts, the spin squeezing dynamics is akin to that produced by the paradigmatic one-axis-twisting (OAT) model -- as expected from an effective separation between collective spin and spin-wave variables. Spin squeezing with OAT-like scaling is shown to be protected by the robustness of long-range ferromagnetic order to quadratic shifts in the equilibrium phase diagram of the system, that we reconstruct via quantum Monte Carlo and mean-field theory.
Spin squeezing generated via inter-atom entanglement in multilevel atomic ensembles provides a powerful resource for quantum-enhanced metrology. Existing schemes that harness internal atomic degrees of freedom to boost squeezing typically encode the collective squeezing in complex superpositions of magnetic sublevels, which complicates state control and limits practical applications. Here, we propose a coherent control scheme that simultaneously enhances collective spin squeezing and maps the resulting atom-atom entanglement onto two well-defined magnetic sublevels suitable for subsequent metrology experiments. Our protocol sandwiches a quantum non-demolition measurement between two internal one-axis-twisting interactions arranged in an echo sequence. We show that this approach can optimally leverage internal states to boost the inter-atom entanglement and, at the same time, encode it in two magnetic sublevels, which is readily convertible into metrologically useful spin squeezing. Our results offer a straightforward and efficient strategy for generating highly entangled yet readily accessible quantum states in multilevel atomic systems.
Spin squeezed entanglement enables metrological precision beyond the classical limit. Understood through the lens of continuous symmetry breaking, dipolar spin systems exhibit the remarkable ability to generate spin squeezing via their intrinsic quench dynamics. To date, this understanding has primarily focused on lattice spin systems; in practice however, dipolar spin systems$\unicode{x2014}$ranging from ultracold molecules to nuclear spin ensembles and solid-state color centers$\unicode{x2014}$often exhibit significant amounts of positional disorder. Here, we develop a theory for scalable spin squeezing in a two-dimensional randomly diluted lattice of quantum dipoles, which naturally realize a dipolar XXZ model. Via extensive quantum Monte Carlo simulations, we map out the phase diagram for finite-temperature XY order, and by extension scalable spin squeezing, as a function of both disorder and Ising anisotropy. As the disorder increases, we find that scalable spin squeezing survives only near the Heisenberg point. We show that this behavior is due to the presence of rare tightly-coupled dimers, which effectively heat the system post-quench. In the case of strongly-interacting nitrogen-vacancy centers in diamond, we demonstrate that an experimentally feasible strategy to decouple the problematic dimers from the dynamics is sufficient to enable scalable spin squeezing.
Entanglement can improve the measurement precision of quantum sensors beyond the shot noise limit. Neutral atoms, the basis of some of the most precise and accurate optical clocks and interferometers, do not naturally exhibit the all-to-all interactions traditionally used to generate such entangled states. On the other hand, these systems exhibit exceedingly high degrees of experimental control over parameters such as temperature, spatial entropy, and itinerancy. In this work, we investigate spin squeezing in a highly coherent itinerant system of neutral atoms with magnetic dipole-dipole interactions. We achieve 7.1 dB of metrologically useful squeezing using finite-range spin-exchange interactions in an erbium quantum gas microscope, and we demonstrate that introducing atomic motion, realizing a dipolar t − J model, protects the spin sector coherence at low fillings, significantly improving the achievable spin squeezing in a 2D dipolar system. This work’s protocol can be implemented with most neutral atoms, opening the door to quantum-enhanced metrology in other itinerant dipolar systems, such as molecules or optical lattice clocks, and serves as a novel method for studying itinerant quantum magnetism with long-range interactions.
We theoretically show that the spin-spin interactions realized in two-dimensional Mott insulators of large-spin magnetic atoms (such as Cr, Er, or Dy) lead to scalable spin squeezing along the nonequilibrium unitary evolution initialized in a coherent spin state. An experimentally relevant perturbation to the collective squeezing dynamics is offered by a quadratic Zeeman shift, which leads instead to squeezing of individual spins. Making use of a truncated cumulant expansion for the quantum fluctuations of the spin array, we show that, for sufficiently small quadratic shifts, the spin squeezing dynamics is akin to that produced by the paradigmatic one-axis-twisting model-as expected from an effective separation between collective-spin and spin-wave variables. Scalable spin squeezing is shown to be protected by the robustness of long-range ferromagnetic order to quadratic shifts in the equilibrium phase diagram of the system that we reconstruct via quantum Monte Carlo and mean-field theory.