Accessing which-path information in the absorption and emission of light by a quantum dot in a Ramsey sequence
I. Maillette de Buy Wenniger, M. Maffei, S. C. Wein, S. P. Prasad, H. Lam, D. Fioretto, A. Lemaître, I. Sagnes, C. Antón-Solanas, P. Senellart, A. Auffèves
quant-phSubmitted Mar 13, 2026• Announced Mar 16, 2026• 0 citations
We quantify which-path information in the absorption and emission of light by a quantum dot along a Ramsey-like sequence. The quantum dot is excited by two successive classical $π/2$-pulses with tunable relative phase, yielding the spontaneous release of coherent superpositions of zero- and one-photon Fock states into two successive time bins. Along the sequence, the first time bin extracts information on the quantum dot energy state, behaving as a which-path detector for the Ramsey interferometer. The which-path information increases over time, and is accessed through the reduction of contrast of the Ramsey fringes. After the second pulse, the information still present in the first time bin controls the emission of coherent light into the second time bin, which is measurable through the reduction of the contrast of self-homodyne interference fringes in a Mach-Zehnder interferometer. Both measurements are in remarkable agreement with theoretical predictions. Our results quantitatively illustrate how which-path information and more generally quantum correlations impact light-matter energy exchanges in the quantum realm.
We quantify which-path information in the absorption and emission of light by a quantum dot along a Ramsey-like sequence. The quantum dot is excited by two successive classical π/2-pulses with tunable relative phase, yielding the spontaneous release of coherent superpositions of zero- and one-photon Fock states into two successive time bins. Along the sequence, the first time bin extracts information on the quantum dot energy state, behaving as a which-path detector for the Ramsey interferometer. The which-path information increases over time, and is accessed through the reduction of contrast of the Ramsey fringes. After the second pulse, the information still present in the first time bin controls the emission of coherent light into the second time bin, which is measurable through the reduction of the contrast of self-homodyne interference fringes in a Mach-Zehnder interferometer. Both measurements are in remarkable agreement with theoretical predictions. Our results quantitatively illustrate how which-path information and more generally quantum correlations impact light-matter energy exchanges in the quantum realm.
A well controlled, triggered source of entangled photons is desirable for many applications in quantum information processing. The two-photon cascade from a biexciton state, two electrons and holes, confined in a quantum dot can be such a source of polarisation-entangled photons provided the two decay paths from the biexciton carry no “which-path” information. In recent years many techniques have been employed to make the two optical decay paths from the biexciton state indistinguishable. A number of these techniques will be discussed and entangled-photon emission from a single quantum dot with a high fidelity in the expected Bell-state from the cascade will be demonstrated. This source of entangled photons allows optical interferometry beyond the limits imposed by the photon wavelength. Interference fringes of the entangled biphoton state reveals a periodicity half of that obtained with the single photon, and much less than that of the pump laser. High fringe visibility indicates that biphoton interference is less sensitive to decoherence than interference of two sequential single photons. The effect of the exciton fine-structure splitting on our entangled photon source will be shown. Surprisingly the entanglement is found to persist despite relatively large separations between the intermediate energy levels of up to 4µeV. Measurements demonstrate that entanglement of the photon pair is robust to the dephasing of the intermediate exciton state responsible for the first order coherence time of either single photon. We distinguish between the first-order coherence time, and a parameter defined as the cross-coherence time, this is illustrated in the figure.
We have scattered photons from an interfering path of a multiple beam Ramsey interference experiment realized with a cesium atomic beam. It is demonstrated that in multiple beam interference the decoherence from photon scattering cannot only lead to a decrease but, under certain conditions, also to an increase of the Michelson fringe contrast. In all cases, the atomic quantum state loses information with photon scattering, as "which-path" information is carried away by the photon field. We outline an approach to quantify this which-path information from observed fringe signals, which allows for an appropriate measure of decoherence in multiple path interference.
Self-assembled semiconductor quantum dots have attracted considerable interest recently, ranging from fundamental studies of quantum optics to advanced applications in the field of quantum information science. With their atom-like properties, quantum dot based nanophotonic devices may also substantially contribute to the development of quantum computers. This work presents experimental progress towards the understanding of light-matter interactions that occur beyond well-understood monochromatic resonant light scattering processes in semiconductor quantum dots. First, we report measurements of resonance fluorescence under bichromatic laser excitation. With the inclusion of a second laser, both first-order and second-order correlation functions are substantially altered. Under these conditions, the scattered light exhibits a rich spectrum containing many spectral features that lead to a range of nonlinear multiphoton dynamics. These observations are discussed and compared with a theoretical model. Second, we investigated the light scattered by a quantum dot in the presence of spectral filtering. By scanning the tunable filters placed in front of each detector of a Hanbury-Brown and Twiss setup and recording coincidence measurements, a \\two-photon spectrum" has been experimentally reconstructed for the first time. The two-photon spectrum contains a wealth of information about the cascaded emission involved in the scattering process, such as transitions occurring via virtual intermediate states. Our measurements also reveal that the scattered frequency-filtered light from a quantum dot violates the Cauchy-Schwarz inequality. Finally, Franson-interferometry has been performed using spectrally filtered light from quantum dot resonance fluorescence. Visibilities exceeding the classical limit were demonstrated by using a pair of folded Mach-Zehnder interferometers, paving the way for producing single time-energy entangled photon pairs that could violate Bell's inequalities.
Summary form only given. A realization of time-bin entanglement obtained from quantum dots would join the strength of long distance transmission that characterizes this type of entanglement with the single photon state purity of the quantum dot emission. Compared with polarization entanglement from quantum dots this scheme does not require elimination of the fine structure splitting responsible for partial distinguishability of the quantum dot cascades [1].Here, we present our results on coherent and resonant excitation of quantum dots, creation of photon pairs, scattering free emission and measurement of the high purity of the emitted photons [2, 3]. In addition, we will show our measurements of the generated time-bin entanglement. To excite a single quantum dot we performed two-photon resonant excitation of the biexciton state. Here, we exploited the biexciton binding energy in order to use the laser light which was not resonant to any photon emitted from the quantum dot (Fig. 1a). Our measurements were performed on a single self-assembled InAs/GaAs quantum dot. We confirmed the resonant nature of the excitation by observing Rabi oscillations (Fig. 1b). Additionally, we performed Ramsey interference measurement and determined the coherence time of the ground-biexciton state superposition. These measurements show that we can coherently transfer the phase of the excitation laser onto the quantum dot system, a necessary requirement to obtain time-bin entanglement.To test the statistics of the emitted state we measured the auto-correlation of the emitted photons (Fig. 3c). Here, the auto-correlation parameter at zero delay was measured to be 0.012(1) without and 0.0073(8) with background subtraction. In addition, we performed a measurement to characterize the state emitted from a quantum dot using a witness-based criterion described in [4]. With this measurement we experimentally confirmed that the resonantly excited quantum dot emits a non-Gaussian state of light (Fig. 1d). This measurement is the first of this nature ever performed on a semiconductor single photon emitter.
Abstract The relation between interference visibility and path distinguishability is a core pillar of quantum complementarity and decoherence theory. In standard quantum mechanics, all coherence decay in interferometric systems is attributed exclusively to path information leakage, which establishes a one-to-one relation between environmental distinguishability and fringe visibility. However, a fundamental question remains experimentally untested: whether discrete quantized energy exchange between light and matter can degrade quantum coherence independently of path distinguishability. In this work, we propose a high-precision cavity-QED experiment based on a Mach–Zehnder interferometer to decouple interaction modality from path information. A single trapped Rb atom inside an optical cavity is placed in one interferometer arm, enabling fully switchable light–matter interaction regimes: resonant discrete energy exchange and far-detuned continuous dispersive interaction. To eliminate systematic artifacts, we employ environmental state tomography to rigorously equalize the path distinguishability in both operational regimes. Furthermore, we systematically compensate all linear dynamical differences between resonant and dispersive cavity responses, including group delay, spectral distortion, and temporal mode mismatch. With all standard decoherence and dynamical contributions precisely calibrated, standard quantum mechanics predicts identical interference visibility for resonant and dispersive interactions. In contrast, a physically motivated alternative conjecture suggests that discrete energy exchange can induce intrinsic coherence suppression even at fixed path distinguishability. The two scenarios yield experimentally distinguishable visibility differences. Our scheme utilizes mature single-atom cavity quantum optics techniques without low-temperature superconducting devices, providing a robust and accessible platform to resolve this long-standing open question in quantum interferometry. The complete optical layout, timing sequence, tomography calibration, statistical criteria, and error suppression strategies are presented. This experiment offers a decisive experimental benchmark for the fundamental relationship between light–matter interaction type and quantum coherence.
Which-path information of a quantum particle in interferometers is the key to infer the past of the quantum particle. It has led to many extensive discussions, including discussions of quantum complementarity and the path-visibility relation. The basics of these discussions are the description, detection, and control of which-path information. In this paper, we focus on the investigation of multidimensional which-path information in a nested Mach-Zehnder interferometer. A general expression of which-path information is given and can be partially extracted by different detection methods. Further analysis shows that the which-path information can be controlled by the phase differences and beam-splitting ratios between the arms of the nested Mach-Zehnder interferometer. Moreover, an alternative which-path information elimination phenomenon has been predicted and demonstrated experimentally. Our work can help us to understand the physics of quantum particles, with potential applications for quantum information processing and quantum metrology.