The rapid development of photonic quantum information processing necessitates precise and programmable control over optical frequency, a capability critical not only for achieving photon indistinguishability but also for exploiting a virtually unbounded frequency dimension. However, efficient and scalable processing of frequency-encoded photon states remains challenging, primarily due to the limited nonlinear optical interaction in most photonic materials. Here, by harnessing the high-performance thin-film lithium niobate electro-optic (EO) platform, we demonstrate an integrated quantum photonic frequency processor that enables coherent and programmable control of photon frequency with high precision. We establish a scalable architecture for frequency-encoded quantum information processing. Using a fully integrated photonic chip, we realize a universal set of frequency-encoded quantum logic gates, including arbitrary single-qubit rotation gates and the two-qubit controlled-phase gate. Furthermore, we demonstrate its application in high fidelity characterization of frequency-bin entangled states. Our work reveals the unprecedented potential of utilizing the frequency degree of freedom in integrated quantum photonic systems.
The rapid development of photonic quantum information processing necessitates precise and programmable control over optical frequency, a capability critical not only for achieving photon indistinguishability but also for exploiting a virtually unbounded frequency dimension. However, efficient and scalable processing of frequency-encoded photon states remains challenging, primarily due to the limited nonlinear optical interaction in most photonic materials. Here, by harnessing the high-performance thin-film lithium niobate electro-optic (EO) platform, we demonstrate an integrated quantum photonic frequency processor that enables coherent and programmable control of photon frequency with high precision. We establish a scalable architecture for frequency-encoded quantum information processing. Using a fully integrated photonic chip, we realize a universal set of frequency-encoded quantum logic gates, including arbitrary single-qubit rotation gates and the two-qubit controlled-phase gate. Furthermore, we demonstrate its application in high fidelity characterization of frequency-bin entangled states. Our work reveals the unprecedented potential of utilizing the frequency degree of freedom in integrated quantum photonic systems.
Integrated thin-film lithium niobate (TFLN) photonics has emerged as a powerful platform for quantum information science, offering its outstanding nonlinear, electro-optic (EO), and integration capabilities. In this review, we present the latest advances in TFLN-based integrated photonics tailored to quantum technologies. We first explore state-of-the-art quantum light sources realized in both straight waveguide and resonator configuration, including high-brightness photon pair generations, squeezed light, and versatile entanglement schemes. Next, we detail progress in integrated photonic processors, with a focus on programmable interferometric networks, ultrafast EO modulators, and essential passive components for photonic qubit processing. We then address critical challenges in optical interfacing and detection technologies, discussing recent innovations in low-loss fiber-to-chip and grating coupler designs, as well as the integration of on-chip single photon detectors. This review provides a forward-looking perspective on scalable quantum photonic systems that could underpin future advances in quantum communication, computing, and sensing.
Integrated quantum photonics requires material platforms that can combine photon generation, spectral control, and electro-optic reconfiguration with low loss and operational stability. Thin-film lithium niobate (TFLN) is a promising platform for this purpose because its second-order nonlinearity and Pockels effect support nonlinear optical processes and active phase control within compact photonic circuits. This dissertation develops TFLN integrated photonic devices and, through collaborative experiments, demonstrates methods toward a frequency-bin quantum information processing platform in which quantum states are represented by discrete optical frequency modes. The work focuses on the design and validation of chip-scale building blocks for frequency-bin operation, including spectral selection, electro-optic tuning, and programmable phase control. Device design, process development, packaging, and experimental characterization led to functional TFLN hardware with resonator-based frequency selectivity, electrically controlled channel tuning, and stable optical and electrical access. Measurements demonstrate stable and programmable frequency-bin control: drift-compensated bias control mitigates electro-optic relaxation and stabilizes multiple frequency channels, while dual-comb spectroscopy verifies repeatable spectral phase programming and waveform reconstruction. These results establish a foundation for future integration of a complete frequency-bin quantum photonic system on TFLN. To support artificial-intelligence-assisted design of photonic and electromagnetic systems, this dissertation further develops a data-driven framework for electromagnetic wave modeling. The EM-OmniVerse dataset and foundation-model framework organize simulated field dynamics together with material, source, geometry, and language information. Across seven out-of-distribution transfer domains, the jointly trained foundation model gives the lowest prediction error in five cases and the second-lowest in two. A representative autoregressive test also shows improved long-horizon stability relative to a single-domain baseline. These results connect experimental photonic-platform development with scalable computational tools for electromagnetic design.
Within the last decade, thin-film lithium niobate (TFLN) has emerged as a leading integrated photonics platform with immediate applications in classical communications. Concurrently, TFLN components tailored to the requirements of photonic quantum information processing have also garnered considerable interest. Chief among these is the quasi-phase matched (QPM) nonlinear frequency mixer—implemented via periodic domain inversion in ferroelectric lithium niobate—which can be used to generate photon pairs, squeezed states of light, and to perform single photon frequency conversion. Here, we demonstrate progress towards realizing a spectrally separable photon pair source in lithium niobate via waveguide dispersion engineering—a technique uniquely enabled by sub-wavelength optical mode confinement in the thin-film platform. Subsequently, we design optimize a scalable fabrication process to produce QPM TFLN devices for applications that require strict adherence to a specified operating wavelength, such as quantum frequency conversion in a quantum communications network. Finally, we explore how high-performance electro-optic devices can be combined with these nonlinear optical devices to realize a multi-functional platform in which quantum states of light can be generated and manipulated within a single, compact photonic integrated circuit.
Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of heralded single-photon pulses using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (±641 GHz or ±5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.
Scalable photonic quantum computing architectures pose stringent requirements on photonic processing devices. The need for low-loss high-speed reconfigurable circuits and near-deterministic resource state generators are some of the most challenging requirements. Here we develop an integrated photonic platform based on thin-film lithium niobate and interface it with deterministic solid-state single-photon sources based on quantum dots in nanophotonic waveguides. The generated photons are processed with low-loss circuits programmable at speeds of several GHz. We realize a variety of key photonic quantum information processing functionalities with the high-speed circuits, including on-chip quantum interference, photon demultiplexing, and reprogrammability of a four-mode universal photonic circuit. These results show a promising path forward for scalable photonic quantum technologies by merging integrated photonics with solid-state deterministic photon sources in a heterogeneous approach to scaling up.
Abstract Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of nonclassical light using an integrated thin-film lithium niobate (TFLN) phase modulator. We achieve record-high electro-optic frequency shearing of telecom single photons over terahertz range (± 641 GHz or ± 5.2 nm), enabling high visibility quantum interference between frequency-nondegenerate photon pairs. We further operate the modulator as a time lens and demonstrate over eighteen-fold (6.55 nm to 0.35 nm) bandwidth compression of single photons. Our results showcase the viability and promise of on-chip quantum spectral control for scalable photonic quantum information processing.