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arXiv:2603.07958

Enhanced Rydberg Blockade through RF-tuned Förster Resonance

Lukas Palm, Bowen Li, Yiming Cady Feng, Marius Jürgensen, Jon Simon

Published Mar 9, 2026• 1 citation
arXivHTMLPDF

Abstract

Enhancing interactions between Rydberg atoms is a key challenge in contemporary quantum technologies. Stronger interactions enable faster Rydberg gates in digital processors and larger entangled states in analog simulation. Achieving the same interaction strength at lower principal quantum number addresses current constraints in available Rabi frequency and field sensitivity in large scale tweezer or cavity QED experiments. Here, we demonstrate a new technique using AC Stark shifts from a microwave drive to tune into a Förster resonance, thereby modifying the interaction scaling with distance from $1/R^6$ to $1/R^3$. We validate enhanced Rydberg interactions (in strength and range) by probing cavity Rydberg polariton blockade at $n=44$ in $^{87}$Rb, improving from $g^{(2)}(0) = 1.0 (1)$ in the Van-der-Waals regime to $g^{(2)}(0) = 0.38 (1)$ in the dipolar regime on the Förster resonance. Importantly, our technique allows minimal shifts of the original Rydberg state, suppressing detuning errors in gate protocols while maintaining quadratic insensitivity to DC electric fields.

DOI
10.48550/arxiv.2603.07958

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Enhancing interactions between Rydberg atoms is a key challenge in contemporary quantum technologies. Stronger interactions enable faster Rydberg gates in digital processors and larger entangled states in analog simulation. Achieving the same interaction strength at lower principal quantum number addresses current constraints in available Rabi frequency and field sensitivity in large scale tweezer or cavity QED experiments. Here, we demonstrate a new technique using AC Stark shifts from a microwave drive to tune into a Förster resonance, thereby modifying the interaction scaling with distance from 1/R61/R^61/R6 to 1/R31/R^31/R3. We validate enhanced Rydberg interactions (in strength and range) by probing cavity Rydberg polariton blockade at n=44n=44n=44 in 87^{87}87Rb, improving from g(2)(0)=1.0(1)g^{(2)}(0) = 1.0 (1)g(2)(0)=1.0(1) in the Van-der-Waals regime to g(2)(0)=0.38(1)g^{(2)}(0) = 0.38 (1)g(2)(0)=0.38(1) in the dipolar regime on the Förster resonance. Importantly, our technique allows minimal shifts of the original Rydberg state, suppressing detuning errors in gate protocols while maintaining quadratic insensitivity to DC electric fields.
Achieving a substantial blockade radius is crucial for developing scalable and efficient quantum communication and computation. In this theoretical study, we present the enhancement of the Rydberg blockade radius by utilizing Förster resonance. This phenomenon occurs when the energy difference between two initial Rydberg states closely matches that between the corresponding final Rydberg states, giving rise to a resonant energy transfer process. We employ quantum defect theory to numerically calculate the 87 Rb– 87 Rb Rydberg atomic pair, enabling us to accurately estimate the van der Waals interaction. Our investigation reveals that when the principal quantum numbers of two Rydberg states differ only slightly, the Förster transition is rarely able to achieve a large blockade radius. However, in cases where the principal quantum numbers differ significantly, we substantially improve the Rydberg blockade radius. Most notably, we identify transition channels exhibiting an extensive blockade radius, surpassing 50 μ m. This significant increase in the blockade radius enables larger-scale quantum operations and advances quantum technologies, with broad implications for achieving long-range quantum entanglement and robust quantum processes.
Long-range interactions between cold Rydberg atoms, which are used in many important applications, can be enhanced using F\"orster resonances between collective many-body states controlled by an external electric field. Here we report on the first experimental observation of highly resolved radio-frequency-assisted F\"orster resonances in a few cold Rb Rydberg atoms. We also observed radio-frequency-induced F\"orster resonances which cannot be tuned by a dc electric field. They imply an efficient transition from van der Waals to resonant dipole-dipole interaction due to Floquet sidebands of Rydberg levels appearing in the rf field. This method can be applied to enhance the interactions of almost arbitrary Rydberg atoms with large principal quantum numbers.
We demonstrated a tuned dipole interaction between Rydberg atoms by employing a controllable electric field in a cold cesium ensemble. The | n P 3/2 ⟩ ( n = 38–40) Rydberg pairs are prepared with a three-photon scheme and detected via the state-selective field ionization technique. A weak DC electric field is used to tune the Rydberg pair interaction from the van der Waals interaction regime to the dipole–dipole interaction regime. The Förster resonant interaction and an adiabatic resonance energy transfer between the n P and n S Rydberg states are attained by precisely tuning the electric field. Rydberg excitation blockade with and without the electric field is investigated by changing the excitation pulse duration, which demonstrates that the dipole interaction–induced blockade effect is stronger than the van der Waals interaction–induced blockade effect. The precise control of the Rydberg interaction is of great significance to the coherent interaction in many-body systems and non-radiative collision processes.
Long-range interactions between cold Rydberg atoms are being investigated for neutral-atom quantum computing, quantum simulations, phase transitions in cold Rydberg gases and other applications. Fine tuning of the interaction strength can be implemented using Förster resonances between Rydberg atoms controlled by an electric field. The observation of the Stark-tuned Förster resonances between Rydberg atoms excited by narrowband cw laser radiation requires usage of a Stark-switching technique in order to excite the atoms first in a fixed electric field and then to induce the interactions in a varied electric field, which is scanned across the Förster resonance. The application of the radio-frequency field causes additional Förster resonances between collective states, whose line shape depends on the interaction strengths and time. Spatial averaging over the atom positions in a single interaction volume yields a cusped line shape of the Förster resonance. We present a detailed experimental and theoretical analysis of the line shape and time dynamics of the Stark-tuned Förster resonances Rb( nP 3/2 ) + Rb( nP 3/2 ) → Rb( nS 1/2 ) + Rb([ n + 1] S 1/2 ) for two Rb Rydberg atoms interacting in a time-varying electric field.
High-fidelity entangled Bell states are of great interest in quantum physics. Entanglement of ultracold neutral atoms in two spatially separated optical dipole traps is promising for implementation of quantum computing and quantum simulation and for investigation of Bell states of material objects. We propose a method to entangle two atoms via long-range Rydberg-Rydberg interaction. Alternative to previous approaches, based on Rydberg blockade, we consider radio-frequency-assisted Stark-tuned F\"orster resonances in Rb Rydberg atoms. To reduce the sensitivity of the fidelity of Bell states to the fluctuations of interatomic distance, we propose to use the double adiabatic passage across the radio-frequency-assisted Stark-tuned F\"orster resonances, which results in a deterministic phase shift of the collective two-atom state.
Advances in the coherent control of Rydberg atoms have led to an explosion in their use in a wide range of topics, including quantum computation, simulation, sensing, and networking. More specifically, Rydberg-coupled ensembles of atoms interfaced with a single mode of light have enabled studies of fundamental light-matter interactions at the single-photon level and have emerged as a promising platform to realize scalable quantum networking nodes. In the first part of this thesis, we utilize Rydberg blockade to generate large ensembles that host a single Rydberg excitation and use the collective state as a resource to efficiently generate single photons. We further investigate the shelving of the collective Rydberg excitations to the ground-state manifold, where we observe an order of magnitude increase in the coherence time of the excitation. In the latter half of the thesis, we use near-resonant microwave fields to generate microwave-dressed Rydberg states, where we utilize the degrees of freedom of the microwave field to tune the strength, form, and angular dependence of the dipole-dipole interactions. To this end, we develop a robust and highly tunable microwave polarization control system. We use a set of in-vacuum electrodes as microwave antennas. We measure the microwave polarizations produced by each source at the positions of the atoms using a Rydberg EIT-based polarimetry technique. By characterizing the three imperfect sources, we find the control settings necessary to produce \sigma_-, \pi, and \sigma_+ polarized microwaves with >99 % fidelity. We extend our purification techniques to frequencies away from Rydberg resonances by utilizing an auxiliary microwave field, generating two-photon microwave resonances. The high-fidelity microwave polarizations are used to resonantly admix opposite-parity Rydberg states, generating dressed states with dipole-dipole interactions that are longer range and stronger than the bare van der Waals interactions. To characterize the strength of the interactions, we measure the photon-number statistics of the light generated by the ensemble of atoms. By varying the cloud length relative to the blockade radii, we demonstrate a clear enhancement of the interaction strength due to microwave dressing. Our platform enables further engineering of interactions by exploiting the polarization and frequency degrees of freedom of the microwave fields, opening pathways for new quantum control strategies in many different experimental platforms.