Local Hilbert spaces with large dimension are of key interest for quantum information with applications in quantum computing and memories, quantum simulations and metrology. Thanks to its weak coupling to external perturbations, the large ground-state nuclear spin manifold of fermionic alkaline-earth atoms is an exciting resource to explore for quantum information. Simultaneous single atom and state-resolved detection however remains an outstanding challenge limiting the development of novel quantum computing and simulation schemes beyond qubits. Here, we report on a new imaging technique enabling the simultaneous detection of up to four quantum states encoded in the nuclear spin manifold of a single fermionic strontium atom within 100 microseconds, with state-resolved detection fidelities ranging from 0.936 to 0.997. This technique is further used to track the highly coherent nuclear spin dynamics after a quench highlighting the potential of this system for quantum information. These results offer fascinating perspectives for quantum science with multi-electron atoms ranging from qudit-based quantum computing to quantum simulations of the SU(N) Fermi-Hubbard model.
Local Hilbert spaces with large dimension are of key interest for quantum information with applications in quantum computing and memories, quantum simulations and metrology. Thanks to its weak coupling to external perturbations, the large ground-state nuclear spin manifold of fermionic alkaline-earth atoms is an exciting resource to explore for quantum information. Simultaneous single atom and state-resolved detection however remains an outstanding challenge limiting the development of novel quantum computing and simulation schemes beyond qubits. Here, we report on a new imaging technique enabling the simultaneous detection of up to four quantum states encoded in the nuclear spin manifold of a single fermionic strontium atom within 100 microseconds, with state-resolved detection fidelities ranging from 0.936 to 0.997. This technique is further used to track the highly coherent nuclear spin dynamics after a quench highlighting the potential of this system for quantum information. These results offer fascinating perspectives for quantum science with multi-electron atoms ranging from qudit-based quantum computing to quantum simulations of the SU(N) Fermi-Hubbard model.
Spin-resolved microscopy of 87Sr SU(N) Fermi-Hubbard systems
Quantum-gas microscopes provide direct access to the phases of the Hubbard model, bringing microscopic insight into the complex competition between interactions, SU(2) magnetism, and doping. Alkaline-earth(-like) fermions extend this spin-1/2 paradigm by realizing higher symmetries and giving access to SU(N) Hubbard models, with rich phase diagrams to be unveiled. Despite its fundamental interest, a microscopic exploration of SU(N) quantum systems has remained elusive. Here we report the realization of a quantum-gas microscope for fermionic 87Sr. Our imaging scheme, based on cooling and fluorescence on the narrow intercombination line at 689 nm, enables spin-resolved single-atom detection. By implementing a spin-selective optical pumping protocol, we determine the occupation of each of the 10 spin states in a single experimental realization, a crucial capability for probing site-resolved magnetic correlations. We benchmark our method by observing single-particle Larmor precession across the full spin-9/2 ground-state manifold and use numerical simulations of SU(N) Fermi-Hubbard chains, incorporating the measured detection fidelities, to demonstrate its capability to resolve many-body spin correlations. Our results establish 87Sr quantum-gas microscopy as a powerful approach to study exotic magnetism in the SU(N) Fermi-Hubbard model, and provide a new detection tool for studies in quantum simulation, computation, and metrology.
We demonstrate coherent manipulation of the nuclear degrees of freedom of ultracold ground-state strontium-87 atoms, thus providing a toolkit for fully exploiting the corresponding large Hilbert space as a quantum resource and for quantum simulation experiments with s u ( N ) -symmetric matter. By controlling the resonance conditions of Raman transitions with a tensor light shift, we can perform rotations within a restricted Hilbert space of two isolated spin states among the 2 F + 1 = 10 possible states. These manipulations correspond to engineering unitary operations derived from generators of the s u ( N ) algebra beyond what can be done by simple spin precession. We present Ramsey interferometers involving an isolated pair of Zeeman states with no measurable decoherence after 3 s. We also demonstrate that one can harness the large spin degrees of freedom as a qudit resource by implementing two interferometer schemes over four states. The first scheme senses in parallel multiple external fields acting on the atoms, and the second scheme simultaneously measures multiple observables of a collective atomic state—including noncommuting ones. Engineering unitary transformations of the large spin driven by other generators than the usual spin- F representation of the s u ( 2 ) group offers new possibilities from the point of view of quantum metrology and quantum many-body physics, notably for the quantum simulation of large-spin s u ( N ) -symmetric quantum magnetism with fermionic alkaline-earth atoms.
The development of quantum-gas microscopes has brought novel ways of probing quantum degenerate many-body systems at the single-atom level. Until now, most of these setups have focused on alkali atoms. Expanding quantum-gas microscopy to alkaline-earth elements will provide new tools, such as SU( N )-symmetric fermionic isotopes or ultranarrow optical transitions, to the field of quantum simulation. Here we demonstrate the site-resolved imaging of a 84 Sr bosonic quantum gas in a Hubbard-regime optical lattice. The quantum gas is confined by a two-dimensional in-plane lattice and a light-sheet potential, which operate at the strontium clock-magic wavelength of 813.4 nm. We realize fluorescence imaging using the broad 461-nm transition, which provides high spatial resolution. Simultaneously, we perform attractive Sisyphus cooling with the narrow 689-nm intercombination line. We reconstruct the atomic occupation from the fluorescence images, obtaining imaging fidelities above 94 % . Finally, we realize a 84 Sr superfluid in the Bose-Hubbard regime. We observe its interference pattern upon expansion, a probe of phase coherence, with single-atom resolution. Our strontium quantum-gas microscope provides a new platform to study dissipative Hubbard models, quantum optics in atomic arrays, and SU( N ) fermions at the microscopic level. Published by the American Physical Society 2024
High-resolution fluorescence imaging of ultracold atoms and molecules is paramount to performing quantum simulation and computation in optical lattices and tweezers. Imaging durations in these experiments typically range from a millisecond to a second, significantly limiting the cycle time. In this work, we present fast, 2.4 μs single-atom imaging in lattices, with 99.4% fidelity - pushing the readout duration of neutral atom quantum platforms to be close to that of superconducting qubit platforms. Additionally, we thoroughly study the performance of accordion lattices. We also demonstrate number-resolved imaging without parity projection, which will facilitate experiments such as the exploration of high-filling phases in the extended Bose-Hubbard models, multi-band or SU(N) Fermi-Hubbard models, and quantum link models. High-resolution imaging is essential for quantum simulation and computation in optical lattices and tweezers. Here, authors achieve fast 2.4-microsecond single-atom imaging with 99.4% fidelity and demonstrate number-resolved imaging without parity projection, advancing quantum readout capabilities.
Few-level systems consisting of a certain number of spin states have provided the basis of a wide range of cold atom researches. However, more developments are still needed for better preparation of isolated few-spin systems. In this work, we demonstrate a highly nonlinear spin-discriminating (HNSD) method for isolating an arbitrary few-level manifold out of a larger total number of spin ground states in fermionic alkaline-earth atoms. With this method, we realize large and tunable energy shifts for unwanted spin states while inducing negligible shifts for the spin states of interest, which leads to a highly isolated few-spin system under minimal perturbation. Furthermore, the isolated few-spin system exhibits a long lifetime on the hundred-millisecond scale. Using the HNSD method, we demonstrate a characteristic Rabi oscillation between the two states of an isolated two-spin Fermi gas. Our method has wide applicability for realizing long-lived two-spin or high-spin quantum systems based on alkaline-earth fermions.
Imagine a new generation of computers that dramatically surpasses the most powerful supercomputers, being able to tackle the most challenging of computational problems. These problems arise, for example, in quantum physics where the computational power required to model a many-particle system increases exponentially with the number of its constituents, and as a consequence the calculations become prohibitively time-consuming. Nobel laureate Richard Feynman proposed this new type of computer in the early 1980s: ‘Let the computer itself be built of quantum mechanical elements which obey quantum mechanical laws.’ Such a quantum simulator would allow researchers to tackle challenging problems in condensed-matter physics. In particular many-body fermionic quantum systems are very difficult to compute due to the antisymmetric nature of the wave function, and the resulting sign problem for quantum Monte Carlo methods. This is why a quantum simulator will be an excellent test bed to investigate phenomena and properties of strongly correlated fermionic quantum systems. A powerful experimental platform to realize a quantum simulator is laser-cooled atoms [1] held in an artificial crystal of light, generated by superimposing laser beams. The atoms are kept in this optical lattice similar to marbles in the hollows of an egg carton, and they can mimic the behaviour of electrons in a real crystal. These systems interface atomic physics with condensed matter physics in a new way, as the tools of atomic physics allow for exquisite control of many experimental parameters, which are often inaccessible in solid state experiments. In-situ imaging techniques [2] using ‘quantum-gas microscopes’ constitute a new approach to the study of many-body quantum systems in an optical lattice with unprecedented resolution at the single-particle and single-site level [3,4]. This new method is complementary to earlier optical lattice experiments measuring distributions in momentum space after a time-of-flight expansion. A quantum-gas microscope uses an optical imaging system (Fig. 1a) for collecting the fluorescence light of ultracold atoms in an optical lattice with high spatial resolution comparable to the lattice spacing of ≈ 500 nm. (a) Atoms in optical lattice atoms are imaged with a high-resolution microscope objective [4]. (b) Single-site addressing is achieved by focussing a laser beam through the microscope onto selected atoms, bringing them into resonance with microwave radiation which produces spin flips [12]. (c) and (d) Single-atom-resolved fluorescence images of bosonic Mottinsulators [4,9]. (e) Deterministically prepared atom distribution using single-site addressing [12]. (f) Direct observation of single-atom quantum walks [15]. Fluorescence imaging of atoms in a quantum-gas microscope has made it possible to directly observe bosonic Mott insulators with single-atom resolution [4–6], giving access to in-situ measurements of temperature and entropy distributions. Subsequently, ground-breaking experiments in many-body quantum dynamics have been performed, such as the first direct observation of correlation spreading after quenches of the system to lower lattice depths [7]. Other experiments include the quantum simulation of an antiferromagnetic spin-1/2 chain [8], the realization of algorithmic cooling [9], the direct measurement of correlations across the superfluid-to-Mott-insulator transition [10], or the observation of the ‘Higgs’ amplitude mode [11]. The high-resolution imaging system is also capable of optically addressing individual atoms with sub-diffraction-limited resolution. For this purpose, a laser beam is focussed though the microscope objective onto selected lattice sites, bringing the atoms into resonance with microwave radiation which produces spin flips [12,13]. The preparation of arbitrary atom distributions in the lattice not only opens perspectives for neutral-atom quantum information processing, but also allows the deterministic creation of specific out-of-equilibrium situations, and their ensuing system dynamics can be studied with single-atom resolution. Examples include the creation of spin impurities and the study of their dynamics in a many-body system [14], the observation of quantum walks [15] and magnon-bound states [16], and the measurement of entanglement entropy [17]. The technique used for single-site-resolved detection of individual atoms in the optical lattice is fluorescence imaging. It requires laser cooling of the atoms to sub-Doppler temperatures while detecting the fluorescence photons emitted during this process. A challenge is to achieve a low particle loss rate and to prevent the atoms from hopping between lattice sites. In the case of the first quantum-gas microscopes, this has been implemented with bosonic rubidium-87 atoms, and also recently for ytterbium-174. However, it has proven more challenging for fermionic alkaline species such as potassium-40 and lithium-6, as their low mass and small excited state hyperfine splitting-prevented standard sub-Doppler cooling from working. As a result, it took several years to extend the quantum-gas microscope technique to fermionic species, and in 2015 several groups have demonstrated single-atom-resolved imaging of fermions [18]. In these setups, the direct observation of band insulators [19], fermionic Mott insulators [20,21] and even antiferromagnetic correlations [22] has been reported most recently. These developments provide fascinating opportunities to study many-body fermionic quantum systems with single-particle access. The fermionic nature of the electron is vital to understanding a range of phenomena within solid-state physics, such as electron pairing in superconductivity, and quantum magnetism. In this context, the quantum simulator will allow, e.g. for direct measurement of ordered quantum phases and out-of-equilibrium dynamics, with access to quantities such as spin--spin correlation functions and the growth of many-body entanglement. The high-resolution imaging systems could also be used to project tailored time-varying light fields onto the atoms, allowing the removal of high-entropy regions by locally modifying the confining potential to attain very low-entropy states. Attaining these low-entropy many-particle states is one of the key challenges in our field. In summary, quantum-gas microscopes offer unprecedented access to many-body quantum systems, and they will allow us to gain an even deeper insight into the intriguing world of quantum physics that governs the properties of strongly correlated materials. Using a well-controlled quantum system to simulate other quantum systems could help resolve some of the most challenging problems scientists face in condensed matter physics and materials science, but it will also provide new insights in quantum chemistry, high-energy physics and biology. SK acknowledges funding from the EU (ERC FERMILATT, SIQS, QuProCs) and SUPA.