We study the ground-state and low-lying metastable phases of repulsive binary Bose-Einstein condensates confined in twisted, spin-dependent periodic optical lattices. For balanced mixtures, weak intercomponent interactions yield a fourfold momentum-space symmetry dictated by the lattice geometry. Increasing the coupling strength leads to the emergence of additional momentum peaks that combine with the lattice-induced structure to produce an eightfold rotationally symmetric pattern, signaling quasicrystalline order. At intermediate interactions, global phase separation suppresses this quasicrystalline state; however, at stronger coupling, local phase separation gives rise to a long-lived metastable phase in which the eightfold symmetry is restored. In this regime, a secondary ring of dominant momentum peaks appears at smaller wave vectors, indicating longer-wavelength density modulations and a crossover from lattice-dominated to interaction-driven quasicrystalline order. In contrast, imbalanced mixtures form partially miscible density clusters with eightfold-symmetric aperiodic patterns only at intermediate coupling, while stronger interactions drive global phase separation and permanently destroy quasicrystalline order. Real-time simulations demonstrate that these aperiodic structures are dynamically stable and experimentally accessible. Our results show that quasicrystalline order can emerge in binary condensates without explicitly aperiodic lattices and reveal population balance as a key ingredient for stabilizing quantum quasicrystals.
We study the ground-state and low-lying metastable phases of repulsive binary Bose-Einstein condensates confined in twisted, spin-dependent periodic optical lattices. For balanced mixtures, weak intercomponent interactions yield a fourfold momentum-space symmetry dictated by the lattice geometry. Increasing the coupling strength leads to the emergence of additional momentum peaks that combine with the lattice-induced structure to produce an eightfold rotationally symmetric pattern, signaling quasicrystalline order. At intermediate interactions, global phase separation suppresses this quasicrystalline state; however, at stronger coupling, local phase separation gives rise to a long-lived metastable phase in which the eightfold symmetry is restored. In this regime, a secondary ring of dominant momentum peaks appears at smaller wave vectors, indicating longer-wavelength density modulations and a crossover from lattice-dominated to interaction-driven quasicrystalline order. In contrast, imbalanced mixtures form partially miscible density clusters with eightfold-symmetric aperiodic patterns only at intermediate coupling, while stronger interactions drive global phase separation and permanently destroy quasicrystalline order. Real-time simulations demonstrate that these aperiodic structures are dynamically stable and experimentally accessible. Our results show that quasicrystalline order can emerge in binary condensates without explicitly aperiodic lattices and reveal population balance as a key ingredient for stabilizing quantum quasicrystals.
The discovery of quasicrystals with crystallographically forbidden rotational symmetries has changed the notion of the ordering in materials, yet little is known about the dynamical emergence of such exotic forms of order. Here we theoretically study a nonequilibrium cavity-QED setup realizing a zero-temperature quantum phase transition from a homogeneous Bose-Einstein condensate to a quasicrystalline phase via collective superradiant light scattering. Across the superradiant phase transition, collective light scattering creates a dynamical, quasicrystalline optical potential for the atoms. Remarkably, the quasicrystalline potential is "emergent" as its eightfold rotational symmetry is not present in the Hamiltonian of the system, rather appears solely in the low-energy states. For sufficiently strong two-body contact interactions between atoms, a quasicrystalline order is stabilized in the system, while for weakly interacting atoms the condensate is localized in one or few of the deepest minima of the quasicrystalline potential.
We investigate the formation of moire quasicrystal patterns in Bose gasses confined in twisted bilayer optical lattices via Floquet-engineered intralayer atomic interactions. Dynamical evolutions of the total density wave amplitude exhibit the stage for the emergence of moire quasicrystal patterns, where the pattern formation is closely associated with the momenta of collective modes excited by the weak periodic drive. Through analyzing the radial and angular density wave amplitude, we find that these new collective modes are only coupled radially and cannot be decoupled eventually. The symmetry of quasicrystal patterns can be easily manipulated by the modulation frequencies and amplitudes. Reducing the frequencies and increasing the amplitudes can both facilitate lattice symmetry breaking and the subsequent emergence of rotational symmetry. Notably, a twelve-fold quasicrystal pattern emerges under specific parameters, closely resembling the moire quasicrystal in twisted bilayer graphene. The momentum-space distributions also exhibit high rotational symmetry, which is consistent with the real-space patterns at specific evolution times. Our findings establish a new quantum platform for exploring quasicrystals and their symmetry properties in ultracold bosonic systems.
Quasicrystals are long-range ordered and yet non-periodic. This interplay results in a wealth of intriguing physical phenomena, such as self-similarity, the inheritance of topological properties from higher dimensions, and the presence of non-trivial structure on all lengthscales. However, quasicrystalline materials are notoriously hard to synthesise, as defects and impurities may greatly alter their final microscopic composition. The field of quantum simulation with ultracold atoms offers a solution to this problem, namely the use of optical lattices – standing waves of light. Optical lattices are free of impurities and therefore ideally suited to study quasicrystals, enabling unprecedented access to observables that are unattainable in condensed matter systems. This study presents the first experimental realisation of a two-dimensional quasicrystalline potential for ultracold atoms, based on an eightfold symmetric optical lattice. Features pertaining to both ordered and disordered phases are observed, from sharp diffraction peaks in the matter-wave interference pattern, to a disorder-induced localised phase emerging at a critical lattice depth V_loc ~ 1.78 E_rec. The localised phase seems to be resilient against moderate interactions, which would make this the first experimental realisation of a 2D Bose glass.
This thesis concerns the physics of ultracold bosons in quasicrystalline lattices, studied by means of quantum simulation using ultracold 39K atoms loaded to an eight-fold rotationally symmetric optical quasicrystal. Quasicrystalline and quasiperiodic systems, thanks to their long-range order and lack of periodicity, exhibit a wealth of interesting properties such as a dense and self-similar momentum space, and a localization transition to Anderson insulator or Bose glass states (in non-interacting or interacting cases respectively) reminiscent of that in disordered systems, whilst lacking the rare regions that typically exist in such systems. Here we will cover experiments into this system’s behaviour in both equilibrium and non-equilibrium settings. First, we focus on mapping out its phase diagram in both weakly and strongly interacting regimes. We observe consistency with numerical predictions for the superfluid-Bose glass phase transition using coherence measurements, as well as finding a region of roughly zero compressibility around where the numerics predicts the existence of a Mott insulator ground state. We also study which regimes of the phase diagram can be ramped through adiabatically, finding that entropy is created upon traversing the Bose glass phase irrespective of ramp duration, which we attribute to its localized nature. Next we look into the dynamics of the system after a quench of the lattice depth in the weakly interacting regime. Upon quenching from the superfluid regime to the Bose glass regime, we observe a quantum walk to higher order diffraction peaks in momentum space whose maximum order is unbounded by kinetic energy thanks to the dense, self-similar nature of the quasicrystal’s momentum space. Quenching in the opposite direction we observe instead a walk between sites in real space for short times by looking at the position (as opposed to momentum) space autocorrelation function of the cloud, finding an expansion rate in agreement with an intuitive estimate based on the Lieb-Robinson bounds of a periodic system. We also look into the timescales of these dynamics in the context of what we might expect from the underlying Hamiltonian, before finally investigating the loss of coherence exhibited by the system after a slower quench of the lattice depth from an initially superfluid cloud. We observe that coherence is lost sooner after the quench for deeper final lattices, with the loss becoming almost instantaneous for quenches that cross the localization transition across the whole cloud. After this we explore the system’s transport dynamics by means of a quench to an excited state at the same time as an additional confining potential is switched off. We observe that unlike in the case of a periodic square lattice, where ballistic expansion that scales with the tunnelling strength occurs in the non-interacting case before becoming slower upon the introduction of interactions thanks to diffusion, in the quasicrystal the transport rate no longer scales with tunnelling strength. Instead we observe a drop relative to the tunnelling rate by 2 − 3 orders of magnitude as the lattice depth is increased from 1Er to 5Er with little dependence on the interaction strength. We also note that the finite rate measured for the deeper lattices is potentially an overestimate since the finite loss rate of atoms makes mass transport indistinguishable from density-dependent losses at that point. Finally, we discuss use of a quantum gas magnification scheme with which to magnify the real space density distribution of our atoms such that it can be measured with single-site resolution. Some preliminary results are presented regarding how the density distribution changes with lattice depth in the weakly interacting regime, in which we observe that as lattice depth increases a higher proportion of atoms occupy deeper sites close to the centre of the quasicrystal’s configuration space, as we might expect.
We study the low-temperature phases of interacting bosons on a two-dimensional quasicrystalline lattice. By means of numerically exact path integral Monte Carlo simulations, we show that for sufficiently weak interactions the system is a homogeneous Bose-Einstein condensate that develops density modulations for increasing filling factor. The simultaneous occurrence of sizeable condensate fraction and density modulation can be interpreted as the analogous, in a quasicrystalline lattice, of supersolid phases occurring in conventional periodic lattices. For sufficiently large interaction strength and particle density, global condensation is lost and quantum exchanges are restricted to specific spatial regions. The emerging quantum phase is therefore a Bose glass, which here is stabilized in the absence of any source of disorder or quasidisorder, purely as a result of the interplay between quantum effects, particle interactions and quasicrystalline substrate. This finding clearly indicates that (quasi)disorder is not essential to observe Bose glass physics. Our results are of interest for ongoing experiments on (quasi)disorder-free quasicrystalline lattices.
We investigate the properties of Bose–Einstein condensates (BECs) in a two-dimensional quasi-periodic optical lattice (OL) with eightfold rotational symmetry by numerically solving the Gross–Pitaevskii equation. In a stationary external harmonic trapping potential, we first analyze the evolution of matter-wave interference pattern from periodic to quasi-periodic as the OL is changed continuously from four-fold periodic to eight-fold quasi-periodic. We also investigate the transport properties during this evolution for different interatomic interaction and lattice depth, and find that the BEC crosses over from ballistic diffusion to localization. Finally, we focus on the case of eightfold symmetric lattice and consider a global rotation imposed by the external trapping potential. The BEC shows vortex pattern with eightfold symmetry for slow rotation, becomes unstable for intermediate rotation, and exhibits annular solitons with approximate axial symmetry for fast rotation. These results can be readily demonstrated in experiments using the same configuration as in Phys. Rev. Lett. 122 110404 (2019).