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arXiv:2602.10873 · Physical Review A

Experimental study of matter-wave four-wave mixing in K 39 Bose-Einstein condensates with tunable interaction

Yue Zhang, Liangchao Chen, Zekui Wang, Yazhou Wang, Pengjun Wang, Lianghui Huang, Zengming Meng, Zhuxiong Ye, Wei Han, Jing Zhang

Published Dec 23, 2025• 0 citations
arXivHTMLPDF

Abstract

We experimentally investigate four-wave mixing (FWM) of matter waves in two geometric configurations in $^{39}$K Bose-Einstein condensates with the atomic interaction tuned via Feshbach resonances. For one configuration with the single-spin component, the FWM yield increases with a larger scattering length. For the two-spin component configuration, we specifically investigate FWM in both the droplet and gas parameter regimes. We find that the FWM yield reaches its maximum near the critical parameter region between the gas and droplet phases. Our research can help to optimize the FWM yield for matter-wave amplification and entangled atom pair generation, making it conducive to applications in quantum information processing and precision measurement.

DOI
10.1103/btrx-c77h

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We experimentally investigate four-wave mixing (FWM) of matter waves in two geometric configurations in 39^{39}39K Bose-Einstein condensates with the atomic interaction tuned via Feshbach resonances. For one configuration with the single-spin component, the FWM yield increases with a larger scattering length. For the two-spin component configuration, we specifically investigate FWM in both the droplet and gas parameter regimes. We find that the FWM yield reaches its maximum near the critical parameter region between the gas and droplet phases. Our research can help to optimize the FWM yield for matter-wave amplification and entangled atom pair generation, making it conducive to applications in quantum information processing and precision measurement.
Abstract We describe possibilities of spontaneous, degenerate four-wave mixing (FWM) processes in spin–orbit coupled Bose–Einstein condensates. Phase matching conditions (i.e., energy and momentum conservation laws) in such systems allow one to identify four different configurations characterized by involvement of distinct spinor states in which such a process can take place. We derived these conditions from first principles and then illustrated dynamics with direct numerical simulations. We found, among others, the unique configuration, where both probe waves have smaller group velocity than pump wave and proved numerically that it can be observed experimentally under proper choice of the parameters. We also reported the case when two different FWM processes can occur simultaneously. The described resonant interactions of matter waves is expected to play an important role in the experiments of BEC with artificial gauge fields. Beams created by FWM processes are an important source of correlated particles and can be used in the experiments testing quantum properties of atomic ensembles.
A recent experiment [Deng et al., Nature (London) 398, 218 (1999)] demonstrated four-wave mixing of matter wave packets created from a Bose-Einstein condensate. The experiment utilized light pulses to create two high-momentum wave packets via Bragg diffraction from a stationary Bose-Einstein condensate. The high-momentum components and the initial low-momentum condensate interact to form a new momentum component due to the nonlinear self-interaction of the bosonic atoms. We develop a three-dimensional quantum- mechanical description, based on the slowly-varying-envelope approximation, for four-wave mixing in Bose-Einstein condensates using the time-dependent Gross-Pitaevskii equation. We apply this formulation to describe the experimental observations and to make predictions. We examine the role of phase-modulation, momentum, and energy conservation (i.e., phase matching), and particle number conservation in four-wave mixing of matter waves, and develop simple models for understanding our numerical results.
The advent of the laser as an intense, coherent light source gave birth to nonlinear optics, which now plays an important role in many areas of science and technology. One of the first applications of nonlinear optics was the production of coherent light of a new frequency by multi-wave mixing of several optical fields in a nonlinear medium. Until the experimental realization of Bose-Einstein Condensation (BEC) there had been no intense coherent source of matter-waves analogous to the optical laser. BEC has already been exploited to produce a matter-wave 'laser' atom optics was reported: the observation of coherent four wave mixing in which three sodium matter waves mix to produce a fourth. The experiment utilized light pulses to create two high-momentum wavepackets via Bragg diffraction from a stationary Bose- Einstein condensate. The high-momentum components and the remaining zero momentum condensate component interact to form a new momentum component due to the nonlinear self- interaction of the bosonic atoms. We develop a quantum mechanical description, based on the slowly-varying-envelope approximation to the time-dependent nonlinear Schroedinger equation, to describe four-wave mixing in Bose-Einstein condensates and apply this description to understand the experimental observations and to make new predictions. We examine the role of phase-modulation, momentum and energy conservation, and particle number conservation in four-wave mixing of matter waves.
We calculate the four-wave mixing (FWM) in a Bose-Einstein condensate system having multiple spin wave packets that are initially overlapping in physical space, but have nonvanishing relative momentum that causes them to recede from one another. Three receding condensate atom wave packets can result in production of a fourth wave packet by the process of FWM due to atom-atom interactions. We consider cases where the four final wave packets are composed of one, two, three, and four different internal spin components. FWM with one or two-spin state wave packets is much stronger than three- or four-spin state FWM, wherein two of the coherent moving Bose-Einstein condensate wave packets form a spin-polarization grating that rotates the spin projection of the third wave into that of the fourth diffracted wave (as opposed to the one- or two-spin state case where a regular density grating is responsible for the diffraction). Calculations of FWM for 87Rb^{87}\mathrm{Rb}87Rb and 23Na^{23}\mathrm{Na}23Na condensate systems are presented.
The advent of the laser as an intense, coherent light source gave birth to nonlinear optics, which now plays an important role in many areas of science and technology. One of the first applications of nonlinear optics was the production of coherent light of a new frequency by multi-wave mixing of several optical fields in a nonlinear medium. Until the experimental realization of Bose-Einstein Condensation (BEC) there had been no intense coherent source of matter-waves analogous to the optical laser. FEC has already been exploited to produce a matter-wave `laser' leading to the threshold of a new field of physics: nonlinear atom optics. Recently the first experiment in nonlinear atom optics was reported: the observation of coherent four wave mixing in which three sodium matter waves mix to produce a fourth. The experiment utilized light pulses to create two high-momentum wavepackets via Bragg diffraction from a stationary Bose- Einstein condensate. The high-momentum components and the remaining zero momentum condensate component interact to form a new momentum component due to the nonlinear self- interaction of the bosonic atoms. We develop a quantum mechanical description, based on the slowly-varying-envelope approximation to the time-dependent nonlinear Schrodinger equation (also called the Gross-Pitaevskii equation), to describe four-wave mixing in Bose-Einstein condensates and apply this description to understand the experimental observations and to make new predictions. We examine the role of phase-modulation, momentum and energy conservation (i.e., phase-matching), and particle number conservation in four-wave mixing of matter waves.
This thesis presents the development of an experimental apparatus to produce Bose-Einstein condensates (BECs) with tunable interparticle interactions. The ability to precisely control the strength of these interactions, and even to switch them from repulsive to attractive, allows one to probe novel regimes of condensate physics, from the collapse of attractively interacting BECs and the formation of solitary matter-waves to the observation of beyond mean-field effects in strongly repulsive condensates. The construction and characterisation of both a single and crossed beam optical dipole trap is presented. In the single beam case we develop a technique allowing the guided transport of atoms along the beam and up to a room-temperature surface; a technique which can be used to evaporatively cool the trapped atomic cloud. We produce Bose-Einstein condensates of 87Rb in the F=1, mF=-1 state in this trap, comparing the effect of beam waist on the evaporation trajectory. In the crossed beam trap Bose-Einstein condensation of 87Rb is realised in three distinct trapping configurations, along with a 1D optical lattice formed by changing the polarisation of the beams. A method of direct cooling of 85Rb atoms in the crossed trap is developed using a magnetic Feshbach resonance to precisely tune both the elastic and inelastic scattering properties of the atoms. The resonance used for this work occurs at 155G in collisions between atoms in the F=2, mF=-2 state of 85Rb. Bose-Einstein condensates of up to 40,000 85Rb atoms are formed in this trap and we demonstrate the presence of tunable interatomic interactions, exploring the collapse phenomenon associated with attractive condensates. By loading the 85Rb condensate into a quasi-1D waveguide we show that stable attractive condensates can be created, taking the form of bright solitary matter-waves. We observe a solitary wave of ~2,000 atoms which propagates, without dispersion, along the waveguide over a distance of ~1.1mm. The particle-like nature of the solitary wave is demonstrated by classical reflection of the wavepacket from a repulsive Gaussian barrier.