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arXiv:2601.18541

Formation Dynamics of Quantum Droplets for Homonuclear and Heteronuclear Mixtures

Enrique Calderoli, Gerardo Martinez

Published Jan 26, 2026• 0 citations
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Abstract

Significant efforts have been devoted to studying the properties of quantum droplets, an ultra low-temperature phase of bosonic quantum matter that emerges as a consequence of the Lee-Huang-Yang fluctuating correction. However, the temporal dynamics of droplet formation for heteronuclear bosonic mixtures is only partially understood. Here, we numerically analyze the droplet formation process for homonuclear and heteronuclear binary bosonic mixtures in one dimension, using a tight-binding model and real-time evolution with a novel, highly robust integration algorithm. We proceed with a systematic scan of interaction intensities, mass ratios, and initial conditions that allows us to characterize quantitative criteria for droplet formation and equilibrium prospects. Noticeably, most droplets readily form across the entire parameter space, although only a small fraction achieves a stable equilibrium configuration within the simulation horizon. We attribute this equilibrium deficiency to damping from a breathing mode, which we extract directly from the width oscillations at late times. The Lee-Huang-Yang contribution supplies essentially the entire binding energy, while, at late times, the density profile of the equilibrated subset is better described by a soliton-like shape rather than the flat-topped profiles characteristic of larger droplets. Referring to the energy of the free-atom band, the binding energy grows super-extensively with the number of atoms as $E_{\text{bind}} \propto N^{1.6}$. Heteronuclear droplets bind more strongly as the mass ratio between their components increases and exhibit breathing oscillations that are greater than those of their homonuclear counterparts, which is consistent with the role of mass-imbalanced kinetic terms. Our analysis provides a methodological framework for interpreting real-time quantum droplet simulations.

DOI
10.48550/arxiv.2601.18541

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Significant efforts have been devoted to studying the properties of quantum droplets, an ultra low-temperature phase of bosonic quantum matter that emerges as a consequence of the Lee-Huang-Yang fluctuating correction. However, the temporal dynamics of droplet formation for heteronuclear bosonic mixtures is only partially understood. Here, we numerically analyze the droplet formation process for homonuclear and heteronuclear binary bosonic mixtures in one dimension, using a tight-binding model and real-time evolution with a novel, highly robust integration algorithm. We proceed with a systematic scan of interaction intensities, mass ratios, and initial conditions that allows us to characterize quantitative criteria for droplet formation and equilibrium prospects. Noticeably, most droplets readily form across the entire parameter space, although only a small fraction achieves a stable equilibrium configuration within the simulation horizon. We attribute this equilibrium deficiency to damping from a breathing mode, which we extract directly from the width oscillations at late times. The Lee-Huang-Yang contribution supplies essentially the entire binding energy, while, at late times, the density profile of the equilibrated subset is better described by a soliton-like shape rather than the flat-topped profiles characteristic of larger droplets. Referring to the energy of the free-atom band, the binding energy grows super-extensively with the number of atoms as Ebind∝N1.6E_{\text{bind}} \propto N^{1.6}Ebind​∝N1.6. Heteronuclear droplets bind more strongly as the mass ratio between their components increases and exhibit breathing oscillations that are greater than those of their homonuclear counterparts, which is consistent with the role of mass-imbalanced kinetic terms. Our analysis provides a methodological framework for interpreting real-time quantum droplet simulations.
We study the impact of beyond Lee-Huang-Yang (LHY) physics, especially due to intercomponent correlations, in the ground state and the quench dynamics of one-dimensional quantum droplets with an ab initio nonperturbative approach. It is found that the droplet Gaussian-shaped configuration arising for intercomponent attractive couplings becomes narrower for stronger intracomponent repulsion and transits towards a flat-top structure either for larger particle numbers or weaker intercomponent attraction. Additionally, a harmonic trap prevents the flat-top formation. At the balance point where mean-field interactions cancel out, we show that a correlation hole is present in the few-particle limit of LHY fluids as well as for flat-top droplets. Introducing mass imbalance, droplets experience intercomponent mixing and excitation signatures are identified for larger masses. Monitoring the droplet expansion (breathing motion) upon considering interaction quenches to stronger (weaker) attractions, we explicate that beyond LHY correlations result in a reduced velocity (breathing frequency). Strikingly, the droplets feature two-body anticorrelations (correlations) at the same position (longer distances). Our findings pave the way for probing correlation-induced phenomena of droplet dynamics in current ultracold-atom experiments.
Abstract The static and dynamic properties of self-bound quantum droplets in a one-dimensional Bose-Bose mixture are discussed in the spirit of the Hartree–Fock-Bogoliubov theory. This latter enables us to provide beyond the Lee-Huang-Yang (LHY) quantum corrections to the equation of state at both zero and finite temperatures. In the uniform case our results for the ground-state energy and the critical temperature are confirmed through comparison with Quantum Monte-Carlo simulation and with available theoretical results. The density profiles are supported by numerical simulations of the generalized Gross-Pitaevskii equation which selfconsistently includes higher-order terms originating from the normal and anomalous fluctuations under the local density approximation. We show that the density exhibits a dip near its center in the flat-top plateau region for large interspecies interactions. We exemplify the impact of the beyond LHY corrections on the spatiotemporal evolution of the self-bound droplet in the presence of excitation induced by periodic density modulation. It is found that higher-order corrections may lead to the formation of a train of small droplets. We then extend our study for the case of inhomogeneous droplets in quasi one-dimensional Bose mixtures.
We exemplify the impact of beyond Lee-Huang-Yang (LHY) physics, especially due to intercomponent correlations, in the ground state and the quench dynamics of one-dimensional so-called quantum droplets using an ab-initio nonperturbative approach. It is found that the droplet Gaussian-shaped configuration arising for intercomponent attractive couplings becomes narrower for stronger intracomponent repulsion and transits towards a flat-top structure either for larger particle numbers or weaker intercomponent attraction. Additionally, a harmonic trap prevents the flat-top formation. At the balance point where mean-field interactions cancel out, we show that quantum fluctuations prevent the collapse of LHY fluids for larger atom numbers and a correlation hole is present in the few particle limit of these fluids as well as for flat-top droplets. Introducing mass-imbalance, droplets experience intercomponent mixing and excitation signatures are identified for larger masses. Monitoring the droplet expansion (breathing motion) upon considering interaction quenches to stronger (weaker) attractions we explicate that beyond LHY correlations result in a reduced velocity (breathing frequency). Strikingly, the droplets feature two-body anti-correlations (correlations) at the same position (longer distances). Our findings pave the way for probing correlation-induced phenomena of droplet dynamics in current ultracold atom experiments.
We discuss the bulk and surface properties of ultradilute self-bound quantum droplets in a heteronuclear Bose-Bose mixture in the presence of higher-order quantum and thermal fluctuations. Within the realm of the Hartree-Fock-Bogoliubov theory, we calculate beyond the Lee-Huang-Yang corrections to the ground-state energy, the droplet equilibrium density, the surface tension, and the critical number of particles. Our predictions are compared with recent diffusion Monte Carlo simulation and density functional theory method and excellent agreement is found. We address in addition the effects of temperature on the formation and on the robustness of the heteronuclear self-bound mixtures.
In this paper, we present a systematic study on the ground state computation of quantum droplets in homonuclear Bose-Bose mixtures, governed by the extended Gross-Pitaevskii equations (eGPEs) with Lee-Huang-Yang (LHY) corrections. This model captures the formation of self-bound droplets stabilized by the delicate balance between the attractive mean-field interaction and the repulsive quantum fluctuations. We formulate dimensionless energy functionals for both the general two-component system and the reduced single-component density-locked model. To compute the ground states efficiently, we adapt and benchmark various gradient flow discretization schemes, identifying a backward-forward sine-pseudospectral scheme based on the gradient flow with Lagrange multiplier method (GFLM-BFSP) as the robust solver for our simulations. Utilizing this method, we report three main numerical observations: (i) the density-locked model is quantitatively validated as a reliable approximation for ground state properties; (ii) the dimension-dependent convergence rates of the Thomas-Fermi approximation are established in the strong-coupling regime; and (iii) the critical particle number for self-binding in free space is numerically determined, providing a precise correction to the analytical prediction by Petrov [Phys. Rev. Lett. 115, 155302 (2015)].
The ultracold and ultradilute bosonic heteronuclear mixture (41K - 87Rb) of Bose-Einstein condensates with tunable interspecies interaction at zero temperature is studied in the self-bound regime, using numerical simulations based on Density Functional Theory within the Local Density Approximation. In particular, the beyond mean-field effects embodied in the Lee-Huang-Yang energy contribution are explicitly included in the total energy functional. The thermodynamic properties of the homogeneous system are investigated to set the stability conditions of the self-bound droplet. The surface properties are discussed with (i) a variational approach, (ii) a numerical method and (iii) by solving the two coupled Gross-Pitaevskii equations associated to the two components of the mixture. The validity of the liquid-drop model is verified by computing the total ground state energy for systems with a different number of particles and, after the confinement in a quasi-1D configuration by means of an optical waveguide, we also discuss the transition between quantum droplets and bright solitons, two localized states of different nature.