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arXiv:2601.06345

Controlling Rydberg atom-polariton interactions: from exceptional points to fast readout

Tamara Šumarac, Emily H. Qiu, Shai Tsesses, Peiran Niu, Adrian J. Menssen, Wenchao Xu, Valentin Walther, Uroš Delić, Soonwon Choi, Mikhail D. Lukin, Vladan Vuletić

physics.atom-phcond-mat.quant-gasquant-phSubmitted Jan 9, 2026• Announced Jan 13, 2026• 0 citations
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Abstract

Rydberg atoms represent a platform underpinning many recent developments in quantum computation, simulation, sensing, and metrology. They further facilitate optical nonlinearity at the single-photon level when coupled to photons propagating in atomic clouds, which form collective atomic excitations called Rydberg polaritons, strongly interacting with each other. Here, we experimentally explore interactions between a Rydberg polariton in an atomic ensemble and a single, adjacent, Rydberg atom. We discover three different regimes of quantum dynamics corresponding to polariton blockade, coherent exchange, and probabilistic hopping, which are defined by their distinct transmission characteristics, with a transition through an exceptional point occurring between blockade and coherent exchange. We investigate the applications of such interactions for fast, non-destructive detection of Rydberg atoms and present proof-of-principle demonstrations for their potential application in nonlinear photonic networks.

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Rydberg polaritons and Rydberg superatoms - novel tools for quantum nonlinear optics

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Mapping the strong interaction between Rydberg excitations in ultra-cold atomic ensembles onto single photons enables the realization of optical nonlinearities which can modify light on the level of individual photons.This novel approach forms the basis of a growing Rydberg quantum optics toolbox, which already contains photonic logic building-blocks such as single-photon sources, switches, transistors, and conditional π-phase shifts.This thesis reports on two experiments investigating strong photon-photon interactions mediated by Rydberg interactions.First, applying a ladder-type EIT scheme to Rydberg atoms in D-states with high principal quantum number results in the Rydberg interaction mediated nonlinearity accompanied by a time-dependent decay of transmission of probe light through the medium.In a joint experimental and theoretical analysis, this effect is attributed to the dephasing of propagating polaritons into stationary Rydberg excitations caused by the state mixing interaction occurring with Rydberg D-state atoms.Second, via a two-photon Raman excitation scheme Rydberg atoms are efficiently excited in a small atomic cloud.As the size of the Rydberg blockade exceeds the dimension of the medium, only a single Rydberg excitation can be present at a time.By fast engineered dephasing this Rydberg excitation is decoupled from the light field.Measurement of the transmitted light and the amount of excited Rydberg atoms gives evidence for the realization of a deterministic single-photon absorber.

•Jan 1, 2017•2 citations

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Photons are ideal carriers of quantum information: they are fast, low-loss, and compatible with mature photonic infrastructure.Linear optical quantum computing exploits these properties but relies on probabilistic measurements and post-selection, incurring an exponential resource overhead that limits scalability [1].Circumventing this bottleneck requires deterministic quantum logic gates, which in turn demand strong, controllable interactions between individual photons.Photons do not interact in free space or in linear optical media.The standard route to attain effective photonphoton interactions is to hybridise photons with interacting matter excitations, forming polaritons.The matter component introduces an interaction-induced anharmonic level shift U into the ladder of polariton states: when one polariton occupies a mode, the next photon sees a shifted resonance (Fig. 1a).The key figure of merit is U/γ, where γ is the total polariton decoherence rate.For U/γ ≪ 1 the nonlinearity is classical; for U/γ ≳ 1 the system enters the quantum nonlinear regime, enabling photon blockade, large conditional phase shifts, and deterministic photonic gates.Atomic Rydberg systems have provided the clearest demonstration of this regime.Atoms excited to Rydberg states -electronic states with large principal quantum numbers n ≫ 1 -possess unique properties [2].Their lifetimes scale as 1/γ ∝ n 3 and transition dipole moments as µ ∝ n 2 , leading to strong dipole-dipole (U ∝ n 4 /r 3 ) or van der Waals (U ∝ n 11 /r 6 ) interactions over long distances r.These interactions can be imprinted onto photons via electromagnetically induced transparency (EIT) [3]: photons hybridise with collective atomic excitations to form slowly propagating Rydberg polaritons that strongly interact with each other over distances of up to tens of micrometres [4].This mechanism has produced photon blockade [5]

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Abstract Quantum optics based on highly excited atoms, also known as Rydberg atoms, has cemented itself as a powerful platform for the manipulation of light at the few-photon level. The Rydberg blockade, resulting from the strong interaction between individual Rydberg atoms, can turn a large ensemble of atoms into a system which collectively resembles a single two-level emitter, a so-called Rydberg superatom. The coupling of this artificial emitter to a driving photonic mode is collectively enhanced by Rydberg interactions, enabling strong coherent coupling at the few-photon level in free-space. The exquisite level of control achievable through this has already demonstrated its utility in applications of quantum computing and information processing. Here, we review the derivation of the collective coupling between a Rydberg superatom and a single light mode and discuss the similarity of this free-space setup to waveguide quantum electrodynamics systems of quantum emitters coupled to photonic waveguides. We also briefly review applications of Rydberg superatoms to quantum optics such as single-photon generation and single-photon subtraction.

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Production and interaction of photons using atomic polaritons and Rydberg interactions

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Controllably producing optical photons and making them interact are two key requirements for the development of long-distance quantum communications, and more generally for photonic quantum information processing. This thesis presents experimental studies on possible solutions to these two problems, using the conversion of the photons into collective excitations (polaritons) in a cold atomic cloud, inside the mode of a low-finesse optical cavity (~100). Firstly, ground-state polaritons are used to store a single excitation in the cloud memory. This polariton is then efficiently converted into a single photon, whose field is characterized via homodyne tomography. The single photon state’s Wigner function is reconstructed from the experimental data and exhibits negative values, demonstrating that the photon’s degrees of freedom (spatio-temporal mode and quantum state) are well controlled. Secondly, photons can be coupled to polaritons involving Rydberg states. The strong dipolar interactions between these give rise to very strong optical dispersive nonlinearities, that are characterized in a classical excitation regime. These nonlinearities can be amplified until a single photon is enough to modify the entire system’s response, allowing in principle for the generation of effective photon-photon interactions.

•Dec 1, 2014•0 citations
Rydberg atoms represent a platform underpinning many recent developments in quantum computation, simulation, sensing, and metrology. They further facilitate optical nonlinearity at the single-photon level when coupled to photons propagating in atomic clouds, which form collective atomic excitations called Rydberg polaritons, strongly interacting with each other. Here, we experimentally explore interactions between a Rydberg polariton in an atomic ensemble and a single, adjacent, Rydberg atom. We discover three different regimes of quantum dynamics corresponding to polariton blockade, coherent exchange, and probabilistic hopping, which are defined by their distinct transmission characteristics, with a transition through an exceptional point occurring between blockade and coherent exchange. We investigate the applications of such interactions for fast, non-destructive detection of Rydberg atoms and present proof-of-principle demonstrations for their potential application in nonlinear photonic networks.
Mapping the strong interaction between Rydberg excitations in ultra-cold atomic ensembles onto single photons enables the realization of optical nonlinearities which can modify light on the level of individual photons.This novel approach forms the basis of a growing Rydberg quantum optics toolbox, which already contains photonic logic building-blocks such as single-photon sources, switches, transistors, and conditional π-phase shifts.This thesis reports on two experiments investigating strong photon-photon interactions mediated by Rydberg interactions.First, applying a ladder-type EIT scheme to Rydberg atoms in D-states with high principal quantum number results in the Rydberg interaction mediated nonlinearity accompanied by a time-dependent decay of transmission of probe light through the medium.In a joint experimental and theoretical analysis, this effect is attributed to the dephasing of propagating polaritons into stationary Rydberg excitations caused by the state mixing interaction occurring with Rydberg D-state atoms.Second, via a two-photon Raman excitation scheme Rydberg atoms are efficiently excited in a small atomic cloud.As the size of the Rydberg blockade exceeds the dimension of the medium, only a single Rydberg excitation can be present at a time.By fast engineered dephasing this Rydberg excitation is decoupled from the light field.Measurement of the transmitted light and the amount of excited Rydberg atoms gives evidence for the realization of a deterministic single-photon absorber.
Photons are ideal carriers of quantum information: they are fast, low-loss, and compatible with mature photonic infrastructure.Linear optical quantum computing exploits these properties but relies on probabilistic measurements and post-selection, incurring an exponential resource overhead that limits scalability [1].Circumventing this bottleneck requires deterministic quantum logic gates, which in turn demand strong, controllable interactions between individual photons.Photons do not interact in free space or in linear optical media.The standard route to attain effective photonphoton interactions is to hybridise photons with interacting matter excitations, forming polaritons.The matter component introduces an interaction-induced anharmonic level shift U into the ladder of polariton states: when one polariton occupies a mode, the next photon sees a shifted resonance (Fig. 1a).The key figure of merit is U/γ, where γ is the total polariton decoherence rate.For U/γ ≪ 1 the nonlinearity is classical; for U/γ ≳ 1 the system enters the quantum nonlinear regime, enabling photon blockade, large conditional phase shifts, and deterministic photonic gates.Atomic Rydberg systems have provided the clearest demonstration of this regime.Atoms excited to Rydberg states -electronic states with large principal quantum numbers n ≫ 1 -possess unique properties [2].Their lifetimes scale as 1/γ ∝ n 3 and transition dipole moments as µ ∝ n 2 , leading to strong dipole-dipole (U ∝ n 4 /r 3 ) or van der Waals (U ∝ n 11 /r 6 ) interactions over long distances r.These interactions can be imprinted onto photons via electromagnetically induced transparency (EIT) [3]: photons hybridise with collective atomic excitations to form slowly propagating Rydberg polaritons that strongly interact with each other over distances of up to tens of micrometres [4].This mechanism has produced photon blockade [5]
Most phenomena around us can be explained by classical optics since photons interact weakly with atoms. When the interaction is strong enough where one photon affects the properties of other photons, we go to the regime of quantum photon-photon nonlinear optics. The work in this thesis explores this regime of physics. This paves the path to exploring strongly interacting many-body physics with photons which is still a largely unexplored domain. The ability to control strongly interacting photons is also of central importance in quantum science and engineering. We use the approach of Electromagnetically Induced Transparency (EIT) in atomic ensembles to create strong interactions and demonstrate coherent control between single photons. Using EIT, we coherently map single photons onto the atoms which travel as coupled excitations of light and matter called dark-state polaritons. When the medium is optically dense, the polariton propagates as a massive particle with a velocity that is much smaller than the speed of light. These polaritons interact with each other via their atomic component. In this thesis, we show robust symmetry-protected collisions between photons that imprint a large phase of π/2 with little loss and extend the nature of photon-photon interactions to the repulsive regime, which are essential for quantum communication and metrology. We use the technique of photon blockade to make a fast optical detector of Rydberg states, directly demonstrating the use of quantum nonlinear optics for quantum computation. We also study the extensions of the attractive and repulsive photons for three particles shedding light into the formation of bound states and crystals of photons and paving the way to studying many-body physics of photons.
Interacting Rydberg excitations in cold atomic ensembles can exhibit large quantum nonlinearities that enable engineering of strong interactions between individual photons. Consequently, Rydberg ensembles are a promising platform for quantum information applications and the study of more fundamental physics of few- and many-body phenomena with interacting photons. This thesis presents a series of experiments that study and exploit different regimes of Rydberg-mediated interactions. We report the realization of an efficient on-demand single-photon source. The strong long-range Rydberg interactions allow the excitation of only a single collective Rydberg state within the entire atomic medium. The collective excitation can be subsequently retrieved as a single-photon. We use this scheme to generate highly pure and highly indistinguishable photons, which are suitable for scalable quantum information applications. These photons can be compatible with other atomic systems due to their narrow bandwidth, which makes building practical hybrid quantum systems feasible. Here, we demonstrate high visibility two-photon quantum interference between our Rydberg-produced photons, and photons emitted by a remote single-trapped ion. We also study Rydberg atoms under electromagnetically induced transparency conditions, where coherent superpostions of photons and Rydberg excitations propagate through the atomic medium as lossless dark-state polaritons. In the experiment, we use the external control fields to tune the interactions to a many-body regime where we can observe resonant scattering of dark-state polaritons to lossy channels. We show that the enhanced scattering process arises as a pure three-body effect.
Abstract Quantum optics based on highly excited atoms, also known as Rydberg atoms, has cemented itself as a powerful platform for the manipulation of light at the few-photon level. The Rydberg blockade, resulting from the strong interaction between individual Rydberg atoms, can turn a large ensemble of atoms into a system which collectively resembles a single two-level emitter, a so-called Rydberg superatom. The coupling of this artificial emitter to a driving photonic mode is collectively enhanced by Rydberg interactions, enabling strong coherent coupling at the few-photon level in free-space. The exquisite level of control achievable through this has already demonstrated its utility in applications of quantum computing and information processing. Here, we review the derivation of the collective coupling between a Rydberg superatom and a single light mode and discuss the similarity of this free-space setup to waveguide quantum electrodynamics systems of quantum emitters coupled to photonic waveguides. We also briefly review applications of Rydberg superatoms to quantum optics such as single-photon generation and single-photon subtraction.
Controllably producing optical photons and making them interact are two key requirements for the development of long-distance quantum communications, and more generally for photonic quantum information processing. This thesis presents experimental studies on possible solutions to these two problems, using the conversion of the photons into collective excitations (polaritons) in a cold atomic cloud, inside the mode of a low-finesse optical cavity (~100). Firstly, ground-state polaritons are used to store a single excitation in the cloud memory. This polariton is then efficiently converted into a single photon, whose field is characterized via homodyne tomography. The single photon state’s Wigner function is reconstructed from the experimental data and exhibits negative values, demonstrating that the photon’s degrees of freedom (spatio-temporal mode and quantum state) are well controlled. Secondly, photons can be coupled to polaritons involving Rydberg states. The strong dipolar interactions between these give rise to very strong optical dispersive nonlinearities, that are characterized in a classical excitation regime. These nonlinearities can be amplified until a single photon is enough to modify the entire system’s response, allowing in principle for the generation of effective photon-photon interactions.