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arXiv:2512.24472

Three-Axis Spin Squeezed States Associated with Excited-State Quantum Phase Transitions

Chon-Fai Kam

quant-phSubmitted Dec 30, 2025• Announced Jan 1, 2026• 0 citations
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Abstract

Spin squeezing in collective atomic ensembles enables quantum-enhanced metrology by reducing noise below the standard quantum limit through nonlinear interactions. Extending the one-axis and two-axis twisting paradigms of Kitagawa and Ueda, we introduce a general class of three-axis spin squeezed states within the anisotropic Lipkin-Meshkov-Glick model. The model features direction-dependent quadratic couplings that interpolate between uniaxial and biaxial regimes and can be interpreted as an asymmetric quantum rotor. Using semiclassical dynamics, Majorana representations, and Husimi-Q distributions, we analyze the structure and metrological properties of the resulting states. The three-axis framework reproduces the known N^(-2/3) scaling of one-axis twisting and the Heisenberg-limited N^(-1) scaling of two-axis twisting, while allowing additional tunability and enhanced entanglement generation in low-spin systems. We further show that tuning the anisotropy parameters induces ground-state and excited-state quantum phase transitions, including a second-order transition associated with level clustering and critical dynamics. These results unify spin squeezing, quantum criticality, and rotor analogies, and suggest implementations in Rydberg arrays and cavity-QED platforms for precision sensing and quantum simulation.

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•Apr 25, 2022•14 citations
Spin squeezing in collective atomic ensembles enables quantum-enhanced metrology by reducing noise below the standard quantum limit through nonlinear interactions. Extending the one-axis and two-axis twisting paradigms of Kitagawa and Ueda, we introduce a general class of three-axis spin squeezed states within the anisotropic Lipkin-Meshkov-Glick model. The model features direction-dependent quadratic couplings that interpolate between uniaxial and biaxial regimes and can be interpreted as an asymmetric quantum rotor. Using semiclassical dynamics, Majorana representations, and Husimi-Q distributions, we analyze the structure and metrological properties of the resulting states. The three-axis framework reproduces the known N^(-2/3) scaling of one-axis twisting and the Heisenberg-limited N^(-1) scaling of two-axis twisting, while allowing additional tunability and enhanced entanglement generation in low-spin systems. We further show that tuning the anisotropy parameters induces ground-state and excited-state quantum phase transitions, including a second-order transition associated with level clustering and critical dynamics. These results unify spin squeezing, quantum criticality, and rotor analogies, and suggest implementations in Rydberg arrays and cavity-QED platforms for precision sensing and quantum simulation.
Spin squeezing, as a crucial quantum resource, plays a pivotal role in quantum metrology, enabling us to achieve high-precision parameter estimation schemes. Here, we investigate the spin squeezing and the quantum phase transition in an anisotropic central spin system. We find that this kind of central spin system can be mapped to the anisotropic Lipkin-Meshkov-Glick model in the limit where the ratio of transition frequencies between the central spin and the spin bath tends towards infinity. This property can induce a one-axis twisting interaction and provides another possibility for generating spin squeezing. We consider the generation of spin-squeezed states through the ground state and the dynamical evolution of the central spin model, respectively. The results show that the dynamical approach is more effective, and the spin-squeezing parameter improves as the anisotropy parameter decreases, while its value scales with system size as ${N}^{\ensuremath{-}2/3}$. Furthermore, we obtain the critical exponent of the quantum Fisher information around the critical point by numerical simulation, and find its value tends to 4/34/34/3 as the frequency ratio and the system size approach infinity. This paper offers a promising scheme for generating spin-squeezed state and paves the way for potential advancements in quantum sensing.
Spin squeezing is vitally important in quantum metrology and quantum information science. The noise reduction resulting from spin squeezing can surpass the standard quantum limit and even reach the Heisenberg limit (HL) in some special circumstances. However, systems that can reach the HL are very limited. Here, we study the spin squeezing in atomic systems with a generic form of the quadratic collective-spin interaction, which can be described by the Lipkin-Meshkov-Glick model. We find that the squeezing properties are determined by the initial states and the anisotropic parameters. Moreover, we propose a pulse rotation scheme to transform the model into a two-axis twisting model with Heisenberg-limited spin squeezing. Our study paves the way for reaching HL in a broad variety of systems.
Squeezed spin states have important applications in quantum metrology and sensing. It has been shown by S\o{}rensen and M\o{}lmer [Phys. Rev. A 66, 022314 (2002)] that an effective one-axis-twisting interaction can be realized in a cavity setup via a double off-resonance stimulated Raman scattering, resulting in a noise reduction scaling $\ensuremath{\propto}1/{N}^{2/3}$ with NNN being the atom number. Here, we show that, by making an appropriate change of the initial input spin state, it is possible to produce a one-axis-twisting spin squeezing via a single off-resonance stimulated Raman scattering, which thus can greatly simplify the realistic implementation. We also show that the one-axis-twisting interaction can be transformed into a more efficient two-axis-twisting interaction by rotating the collective spin while coupling to the cavity, yielding a Heisenberg limited noise reduction $\ensuremath{\propto}1/N$. Considering the noise effects due to atomic decoherence and cavity decay, we find that substantial squeezing is still attainable with current laboratory techniques.
We study the generation of metrologically useful entanglement in a three-level (spin-1) system naturally realized in arrays of dipole-interacting Rydberg atoms confined in optical tweezers. In the spin-quadrupolar operator basis, the interaction Hamiltonian decomposes into effective SU(2) subspaces, within which quench dynamics from product initial states generate scalable spin-nematic squeezing. For symmetric interactions, we identify a mapping to effective one-axis twisting within bright and dark manifolds and demonstrate that the squeezing parameter scales as ξ2∝N−2/3ξ^{2}\propto N^{-2/3}ξ2∝N−2/3 (ξ2∝N−0.5ξ^{2}\propto N^{-0.5}ξ2∝N−0.5) with system size for all-to-all (two-dimensional dipolar) couplings. In both cases the quantum Fisher information reaches FQ∝N2F_Q\propto N^{2}FQ​∝N2. For antisymmetric interactions supplemented by a microwave drive we find a distinct two-axis countertwisting mechanism. This results in squeezing ξ2∝N−0.7ξ^{2}\propto N^{-0.7}ξ2∝N−0.7 for all-to-all interactions and moderate squeezing for dipolar interactions in 2D. Our results constitute a first theoretical step beyond the well-studied qubit setting toward scalable entanglement generation in qudit systems with dipolar interactions, directly relevant to current Rydberg tweezer experiments.
Ultracold atoms in an ultrahigh-finesse optical cavity are a powerful platform to produce spin squeezing since photon of cavity mode can induce nonlinear spin-spin interaction and thus generate a one-axis twisting Hamiltonian HOAT=qJx2H_{\text{OAT}}=qJ_{x}^{2}HOAT​=qJx2​, whose corresponding maximal squeezing factor scales as N−2/3N^{-2/3}N−2/3, where NNN is the atomic number. On the contrary, for the other two-axis twisting Hamiltonian HTAT=q(Jx2−Jy2)H_{\text{TAT}}=q(J_{x}^{2}-J_{y}^{2})HTAT​=q(Jx2​−Jy2​), the maximal squeezing factor scales as N−1N^{-1}N−1, approaching the Heisenberg limit. In this paper, inspired by recent experiments of cavity-assisted Raman transitions, we propose a scheme, in which an ensemble of ultracold six-level atoms interacts with two quantized cavity fields and two pairs of Raman lasers, to realize a tunable two-axis spin Hamiltonian %H=q(J_{x}^{2}+χJ_{y}^{2})+ω_{0}J_{z}. For proper parameters, the above one- and two- axis twisting Hamiltonians are recovered, and the scaling of N−1N^{-1}N−1 of the maximal squeezing factor can occur naturally. On the other hand, in the two-axis twisting Hamiltonian, spin squeezing is usually reduced when increasing the effective atomic resonant frequency ω0ω_{0}ω0​. Surprisingly, we find that by combined with the dimensionless parameter χ(>−1)χ(>-1)χ(>−1), the effective atomic resonant frequency ω0ω_{0}ω0​ can enhance spin squeezing largely. These results are benefit for achieving the required spin squeezing in experiments.
In an ensemble of two-level atoms that can be described in terms of a collective spin, entangled states can be used to enhance the sensitivity of interferometric precision measurements. While non-Gaussian spin states can produce larger quantum enhancements than spin-squeezed Gaussian states, their use requires the measurement of observables that are nonlinear functions of the three components of the collective spin. In this paper we develop strategies that achieve the optimal quantum enhancements using non-Gaussian states produced by a nonlinear one-axis-twisting Hamiltonian, and show that measurement-after-interaction techniques, known to amplify the output signals in quantum parameter estimation protocols, are effective in measuring nonlinear spin observables. Including the presence of the relevant decoherence processes from atomic experiments, we determine analytically the quantum enhancement of non-Gaussian over-squeezed states as a function of the noise parameters for arbitrary atom numbers.