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arXiv:2511.17420

Measuring Anyonic Exchange Phases Using Two-Dimensional Coherent Spectroscopy

Nico Kirchner, Wonjune Choi, Frank Pollmann

cond-mat.str-elquant-phSubmitted Nov 21, 2025• Announced Nov 24, 2025• 1 citation
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Abstract

Identifying experimental signatures of anyons, which exhibit fractional exchange statistics, remains a central challenge in the study of two-dimensional topologically ordered systems. Previous theoretical work has shown that the threshold behavior in linear response spectroscopy can reveal the fractional exchange statistics between an anyon and its antiparticle. In this work, we extend this framework to nonlinear, two-dimensional coherent spectroscopy. We demonstrate by analyzing time-ordered four-point correlation functions that the threshold behavior of nonlinear response functions encodes the fractional statistics between general pairs of anyons that can combine to any composite topological charge. This feature in particular provides a powerful probe for unambiguously distinguishing non-Abelian anyons, which can form multiple composite charges with distinct nontrivial braid statistics. Our approach is validated using numerical simulations that are consistent with the correct fractional exchange statistics for both the Abelian anyons in the toric code and non-Abelian Ising anyons.

Comments
12 pages, 3 figures

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Measuring Anyonic Exchange Phases Using Two-Dimensional Coherent Spectroscopy

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Identifying experimental signatures of anyons, which exhibit fractional exchange statistics, remains a central challenge in the study of two-dimensional topologically ordered systems. Previous theoretical work has shown that the threshold behavior in linear response spectroscopy can reveal the fractional exchange statistics between an anyon and its antiparticle. In this work, we extend this framework to nonlinear, two-dimensional coherent spectroscopy. We demonstrate by analyzing time-ordered four-point correlation functions that the threshold behavior of nonlinear response functions encodes the fractional statistics between general pairs of anyons that can combine to any composite topological charge. This feature in particular provides a powerful probe for unambiguously distinguishing non-Abelian anyons, which can form multiple composite charges with distinct nontrivial braid statistics. Our approach is validated using numerical simulations that are consistent with the correct fractional exchange statistics for both the Abelian anyons in the toric code and non-Abelian Ising anyons.
Identifying experimental signatures of anyons, which exhibit fractional exchange statistics, remains a central challenge in the study of two-dimensional topologically ordered systems. Previous theoretical work has shown that the threshold behavior in linear response spectroscopy can reveal the fractional exchange statistics between an anyon and its antiparticle. In this work, we extend this framework to nonlinear, two-dimensional coherent spectroscopy. We demonstrate by analyzing time-ordered four-point correlation functions that the threshold behavior of nonlinear response functions encodes the fractional statistics between general pairs of anyons that can combine to any composite topological charge. This feature in particular provides a powerful probe for unambiguously distinguishing non-Abelian anyons, which can form multiple composite charges with distinct nontrivial braid statistics. Our approach is validated using numerical simulations that are consistent with the correct fractional exchange statistics for both the Abelian anyons in the toric code and non-Abelian Ising anyons.
We study the behavior of linear and nonlinear spectroscopic quantities in two-dimensional topologically ordered systems, which host anyonic excitations exhibiting fractional statistics. We highlight the role that braiding phases between anyons have on the dynamics of such quasiparticles, which as we show dictates the behavior of both linear response coefficients at finite temperatures, as well as nonlinear pump-probe response coefficients. These quantities, which act as probes of temporal correlations in the system, are shown to obey distinctive universal forms at sufficiently long timescales. As well as providing an experimentally measurable fingerprint of anyonic statistics, the universal behavior that we find also demonstrates anomalously fast thermal relaxation: correlation functions decay as a “squished exponential” C ( t ) ∼ exp ( − [ t / τ ] 3 / 2 ) at long times. We attribute this unusual asymptotic form to the nonlocal nature of interactions between anyons, which allows relaxation to occur much faster than in systems with quasiparticles interacting via local, nonstatistical interactions. While our results apply to any Abelian or non-Abelian topological phase in two-dimensions, we discuss in particular the implications for candidate quantum spin liquid materials, wherein the relevant quantities can be measured using pre-existing time-resolved terahertz-domain spectroscopic techniques. Published by the American Physical Society 2024
Observation of Time-Domain Braiding of Non-Abelian Anyons at ν=5/2ν= 5/2ν=5/2 State
Unlike elementary particles, which obey either bosonic or fermionic exchange statistics, certain quasiparticles, known as anyons, are predicted to exhibit Abelian or non-Abelian braiding statistics. While braiding Abelian anyons modifies the wavefunction by a 'statistical phase', braiding non-Abelian anyons implements a unitary transformation of the state within a degenerate subspace of states. Experimental evidence of non-Abelian braiding has thus far remained elusive. Here, we report a 'time-domain braiding' signature of non-Abelian anyons in the ν=5/2ν= 5/2ν=5/2 fractional quantum Hall state, by extending our previously demonstrated approach with Abelian anyons at ν=1/3ν= 1/3ν=1/3. Our approach is based on measurements of the current fluctuations arising from weak partitioning of a highly dilute one-dimensional edge mode. We independently probe the partition noise of the downstream charged mode and also that of the upstream neutral mode. These independent measurements agree with our theoretical predictions for 'time-domain braiding' of the downstream Abelian and the upstream non-Abelian anyons, respectively, in the 'particle-hole Pfaffian' topological order. Together, these results provide evidence for the presence of non-Abelian anyons.
The hallmark of a two-dimensional (2d) topologically ordered phase is the existence of deconfined ``anyon'' excitations that have exotic braiding and exchange statistics, different from those of ordinary bosons or fermions. As opposed to conventional Landau-Ginzburg-Wilson phases, which are classified on the basis of the spontaneous breaking of an underlying symmetry, topologically ordered phases, such as those occurring in the fractional quantum Hall effect, are absolutely stable, not requiring any such symmetry. Recently, though, it has been realized that symmetries, which may still be present in such systems, can give rise to a host of new, distinct, many-body phases, all of which share the same underlying topological order. These ``symmetry enriched'' topological (SET) phases are distinguished not on the basis of anyon braiding statistics alone, but also by the symmetry properties of the anyons, such as their fractional charges, or the way that different anyons are permuted by the symmetry. Thus a useful approach to classifying SETs is to determine all possible such symmetry actions on the anyons that are algebraically consistent with the anyon statistics. Remarkably, however, there exist symmetry actions that, despite being algebraically consistent, cannot be realized in any physical system, and hence do not lead to valid 2d SETs. One class of such ``anomalous'' SETs, characterized by certain disallowed symmetry fractionalization patterns, finds a physical interpretation as an allowed surface state of certain three-dimensional (3d) short-range entangled phases, but another, characterized by some seemingly valid but anomalous permutation actions of the symmetry on the anyons and encoded in an H3(G,A){H}^{3}(G,\mathcal{A})H3(G,A) group cohomology class, has so far eluded a physical interpretation. In this work, we find a way to physically realize these anomalously permuting SETs at the surfaces of certain 3d long-range entangled phases, expanding our understanding of general anomalous SETs in two dimensions.
We show that the braiding of anyons in a quantum spin liquid leaves a distinct dynamical signature in the nonlinear pump–probe response. Using a combination of exact diagonalization and matrix product state techniques, we study the nonlinear pump–probe response of the toric code in a magnetic field, a model with mobile electric e and magnetic m anyonic excitations. While the linear response signal oscillates and decays with time like ∼ t − 1.3 , the amplitude of the nonlinear signal for χ XZZ ( 3 ) features a linear-in-time enhancement at early times and a stronger enhancement t α with α > 1 at later times. The comparison between χ XZZ ( 3 ) , which involves nontrivial braiding of e and m anyons, and χ XXX ( 3 ) that involves trivial braiding of the same types of anyons, distinguishes the braiding statistics of anyons. We support our analysis with a hard-core anyon model with statistical gauge fields to develop further insights into the time dependence of the pump–probe response. Pump–probe spectroscopy provides a distinctive new probe of quantum spin liquid states, beyond the inconclusive broad features observed in single spin-flip inelastic neutron scattering.
We study symmetries and defects of a wide class of two-dimensional Abelian topological phases characterized by Lie algebras. We formulate the symmetry group of all Abelian topological field theories. The symmetries relabel quasiparticles (or anyons) but leave exchange and braiding statistics unchanged. Within the class of ADEADEADE phases, in particular, these anyonic symmetries have a natural origin from the Lie algebra. We classify one-dimensional gapped phases along the interface between identical topological states according to symmetries. This classification also applies to gapped edges of a wide range of fractional quantum spin Hall (QSH) states. We show that the edge states of the ADEADEADE QSH systems can be gapped even in the presence of time-reversal and charge-conservation symmetries. We distinguish topological point defects according to anyonic symmetries and bound quasiparticles. Although in an Abelian system, they surprisingly exhibit non-Abelian fractional Majorana-like characteristics from their fusion behavior.