Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2511.08285 · Physical Review A

Nonexistence of maximally entangled mixed states for a fixed spectrum

Gonzalo Camacho, Julio I. de Vicente

quant-phSubmitted Nov 11, 2025• Announced Nov 12, 2025• 0 citations
arXivHTMLPDF

Abstract

The existence of a maximally entangled pure state is a cornerstone result of entanglement theory that has paramount consequences in quantum information theory. A natural generalization of this property is to consider whether a notion of maximal entanglement is possible among all states with the same spectrum (where the aforementioned case of pure states corresponds to the particular choice in which the spectrum is a delta distribution, i.e., rank-1 states). Despite positive evidence in the past that such a notion might exist at least in the case of two-qubit states, it was recently shown in [Phys. Rev. Lett. 133, 050202 (2024)] that the answer to the above question is negative. This reference proved this for particular choices of the spectrum in the case of rank-2 two-qubit density matrices. While this settles the problem in general, it still leaves open whether there are other choices of the spectrum outside the case of pure states where a maximally entangled state for a fixed spectrum might exist. In this work we extend this impossibility result to all rank-2 and rank-3 two-qubit states as well as for a large class of eigenvalue distributions in the case where the rank equals four.

Journal reference
Phys. Rev. A 113, 022416 (2026)
DOI
10.1103/2m8l-kfnm
Comments
11 pages, 1 figure

Related papers

Maximally Entangled Mixed States for a Fixed Spectrum Do Not Always Exist

Julio I. de Vicente

Entanglement is a resource under local operations assisted by classical communication (LOCC). Given a set of states S, if there is one state in S that can be transformed by LOCC into all other states in S, then this state is maximally entangled in S. It is a well-known result that the d-dimensional Bell state is the maximally entangled state in the set of all bipartite states of local dimension d. Since in practical applications noise renders every state mixed, it is interesting to study whether sets of mixed states of relevance enable the notion of a maximally entangled state. A natural choice is the set of all states with the same spectrum. In fact, for any given spectrum distribution on two-qubit states, previous work has shown that several entanglement measures are all maximized by one particular state in this set. This has led us to consider the possibility that this family of states could be the maximally entangled states in the set of all states with the same spectrum, which should then maximize all entanglement measures. In this work, I answer this question in the negative: There are no maximally entangled states for a fixed spectrum in general, i.e., for every possible choice of the spectrum. In order to do so, I consider the case of rank-2 states and show that for particular values of the eigenvalues there exists no state that can be transformed to all other isospectral states not only under LOCC but also under the larger class of nonentangling operations. This in particular implies that in these cases the state that maximizes a given entanglement measure among all states with the same spectrum depends on the choice of entanglement measure; i.e., it cannot be that the aforementioned family of states maximizes all entanglement measures.

arXiv:2402.05673•Physical Review Letters•Jul 30, 2024•11 citations

Maximally entangled mixed states for qubit-qutrit systems

Paulo E. M. F. Mendonça, Marcelo A. Marchiolli, Samuel R. Hedemann

We consider the problems of maximizing the entanglement negativity of X-form qubit-qutrit density matrices with (i) a fixed spectrum and (ii) a fixed purity. In the first case, the problem is solved in full generality whereas, in the latter, partial solutions are obtained by imposing extra spectral constraints such as rank deficiency and degeneracy, which enable a semidefinite programming treatment for the optimization problem at hand. Despite the technically motivated assumptions, we provide strong numerical evidence that threefold degenerate X states of purity $P$ reach the highest entanglement negativity accessible to arbitrary qubit-qutrit density matrices of the same purity, hence characterizing a sparse family of likely qubit-qutrit maximally entangled mixed states.

arXiv:1612.01214•Physical Review A•Feb 21, 2017•23 citations

Extremal maximal entanglement

Wanchen Zhang, Yu Ning, Fei Shi +1 more

A pure multipartite quantum state is called absolutely maximally entangled if all reductions of no more than half of the parties are maximally mixed. However, an $n$-qubit absolutely maximally entangled state exists only when $n$ equals 2, 3, 5, and 6. A natural question arises when it does not exist: Which $n$-qubit pure state has the largest number of maximally mixed $\ensuremath{\lfloor}n/2\ensuremath{\rfloor}$-party reductions? We denote this number by $\mathrm{Qex}(n)$. It was shown that $\mathrm{Qex}(4)=4$ by Higuchi and Sudbery [Phys. Lett. A 273, 213 (2000)] and $\mathrm{Qex}(7)=32$ by Huber et al. [Phys. Rev. Lett. 118, 200502 (2017)]. In this paper, we give a general upper bound of $\mathrm{Qex}(n)$ by linking the well-known Tur\'an problem in graph theory and provide lower bounds using constructive and probabilistic methods. In particular, we show that $\mathrm{Qex}(8)=56$, which is the third known value for this problem.

arXiv:2411.12208•Physical Review A•May 7, 2025•3 citations

Nonlocality and entanglement in qubit systems

Josep Amengual i Batle, M. Casas

Nonlocality and quantum entanglement constitute two special aspects of the quantum correlations existing in quantum systems, which are of paramount importance in quantum-information theory. Traditionally, they have been regarded as identical (equivalent, in fact, for pure two qubit states, that is, Gisin's Theorem ), yet they constitute different resources. Describing nonlocality by means of the violation of several Bell inequalities, we obtain by direct optimization those states of two qubits that maximally violate a Bell inequality, in terms of their degree of mixture as measured by either their participation ratio R = 1/Tr(ρ 2 ) or their maximum eigenvalue λ max . This optimum value is obtained as well, which coincides with previous results. Comparison with entanglement is performed too. An example of an application is given in the XY model. In this novel approximation, we also concentrate on the nonlocality for linear combinations of pure states of two qubits, providing a closed form for their maximal nonlocality measure. The case of Bell diagonal mixed states of two qubits is also extensively studied. Special attention concerning the connection between nonlocality and entanglement for mixed states of two qubits is paid to the so-called maximally entangled mixed states. Additional aspects for the case of two qubits are also described in detail. Since we deal with qubit systems, we will perform an analogous study for three qubits, employing similar tools. Relation between distillability and nonlocality is explored quantitatively for the whole space of states of three qubits. We finally extend our analysis to four-qubit systems, where nonlocality for generalized Greenberger–Horne–Zeilinger states of arbitrary number of parties is computed.

arXiv:1102.4653•Journal of Physics A Mathematical and Theoretical•Oct 14, 2011•61 citations

Entangled symmetric states of N qubits with all positive partial transpositions

Remigiusz Augusiak, Jordi Tura, Jan Samsonowicz +1 more

From both theoretical and experimental points of view symmetric states constitute an important class of multipartite states. Still, entanglement properties of these states, in particular those with positive partial transposition (PPT), lack a systematic study. Aiming at filling in this gap, we have recently affirmatively answered the open question of existence of four-qubit entangled symmetric states with PPT and thoroughly characterized entanglement properties of such states [J. Tura et al., Phys. Rev. A 85, 060302(R) (2012)]. With the present contribution we continue on characterizing PPT entangled symmetric states. On the one hand, we present all the results of our previous work in a detailed way. On the other hand, we generalize them to systems consisting of an arbitrary number of qubits. In particular, we provide criteria for separability of such states formulated in terms of their ranks. Interestingly, for most of the cases, the symmetric states are either separable or typically separable. Then, edge states in these systems are studied, showing in particular that to characterize generic PPT entangled states with four and five qubits, it is enough to study only those that assume few (respectively, two and three) specific configurations of ranks. Finally, we numerically search for extremal PPT entangled states in such systems consisting of up to 23 qubits. One can clearly notice regularity behind the ranks of such extremal states, and, in particular, for systems composed of odd numbers of qubits we find a single configuration of ranks for which there are extremal states.

arXiv:1206.3088•Physical Review A•Oct 15, 2012•47 citations

Bound Entangled States With Negative Partial Transpose Exist

Indrani Chattopadhyay, D. Sarkar

We prove the existence of bound entangled states with negative partial transpose (NPT) in any d × d(d ≥ 3) Hilbert space with a simple assumption on Schmidt rank two states. Obviously they belong to the class of conjectured to be bound entangled states by Divincenzo et.al [Phys. Rev. A, 61, 062312(2000)] and by Dür et.al [Phys. Rev. A, 61, 062313(2000)]. PACS number(s): 03.67.Hk, 03.65.Ud. The basic issue on the classification of mixed state entanglement at least on the level of bipartite systems solely depends upon whether there exist bound entangled states or not. The existence of PPT-bound (PPT means positive partial transpose) entangled states [1] and also the existence of NPT N−copy undistillable states [2, 3] for every positive integer N naturally indicates there may exist NPT-bound entangled states. In this work we are able to show the existence of NPT-bound entangled states with a simple assumption on Schmidt rank two states. We first briefly describe the issue and the importance of the problem. In recent years it is found that quantum entanglement is an useful resource in performing several tasks in quantum information theory and quantum communication [4]. Maximally entangled states shared between two parties are essential ingredients in this respect [5]. Now due to the interaction with environment, states are in practice found to be mixed. However there is a process called distillation by which we can distill sometimes maximally entangled

•Sep 6, 2006•0 citations
The existence of a maximally entangled pure state is a cornerstone result of entanglement theory that has paramount consequences in quantum information theory. A natural generalization of this property is to consider whether a notion of maximal entanglement is possible among all states with the same spectrum (where the aforementioned case of pure states corresponds to the particular choice in which the spectrum is a delta distribution, i.e., rank-1 states). Despite positive evidence in the past that such a notion might exist at least in the case of two-qubit states, it was recently shown in [Phys. Rev. Lett. 133, 050202 (2024)] that the answer to the above question is negative. This reference proved this for particular choices of the spectrum in the case of rank-2 two-qubit density matrices. While this settles the problem in general, it still leaves open whether there are other choices of the spectrum outside the case of pure states where a maximally entangled state for a fixed spectrum might exist. In this work we extend this impossibility result to all rank-2 and rank-3 two-qubit states as well as for a large class of eigenvalue distributions in the case where the rank equals four.
Entanglement is a resource under local operations assisted by classical communication (LOCC). Given a set of states S, if there is one state in S that can be transformed by LOCC into all other states in S, then this state is maximally entangled in S. It is a well-known result that the d-dimensional Bell state is the maximally entangled state in the set of all bipartite states of local dimension d. Since in practical applications noise renders every state mixed, it is interesting to study whether sets of mixed states of relevance enable the notion of a maximally entangled state. A natural choice is the set of all states with the same spectrum. In fact, for any given spectrum distribution on two-qubit states, previous work has shown that several entanglement measures are all maximized by one particular state in this set. This has led us to consider the possibility that this family of states could be the maximally entangled states in the set of all states with the same spectrum, which should then maximize all entanglement measures. In this work, I answer this question in the negative: There are no maximally entangled states for a fixed spectrum in general, i.e., for every possible choice of the spectrum. In order to do so, I consider the case of rank-2 states and show that for particular values of the eigenvalues there exists no state that can be transformed to all other isospectral states not only under LOCC but also under the larger class of nonentangling operations. This in particular implies that in these cases the state that maximizes a given entanglement measure among all states with the same spectrum depends on the choice of entanglement measure; i.e., it cannot be that the aforementioned family of states maximizes all entanglement measures.
We consider the problems of maximizing the entanglement negativity of X-form qubit-qutrit density matrices with (i) a fixed spectrum and (ii) a fixed purity. In the first case, the problem is solved in full generality whereas, in the latter, partial solutions are obtained by imposing extra spectral constraints such as rank deficiency and degeneracy, which enable a semidefinite programming treatment for the optimization problem at hand. Despite the technically motivated assumptions, we provide strong numerical evidence that threefold degenerate X states of purity PPP reach the highest entanglement negativity accessible to arbitrary qubit-qutrit density matrices of the same purity, hence characterizing a sparse family of likely qubit-qutrit maximally entangled mixed states.
A pure multipartite quantum state is called absolutely maximally entangled if all reductions of no more than half of the parties are maximally mixed. However, an nnn-qubit absolutely maximally entangled state exists only when nnn equals 2, 3, 5, and 6. A natural question arises when it does not exist: Which nnn-qubit pure state has the largest number of maximally mixed $\ensuremath{\lfloor}n/2\ensuremath{\rfloor}$-party reductions? We denote this number by Qex(n)\mathrm{Qex}(n)Qex(n). It was shown that Qex(4)=4\mathrm{Qex}(4)=4Qex(4)=4 by Higuchi and Sudbery [Phys. Lett. A 273, 213 (2000)] and Qex(7)=32\mathrm{Qex}(7)=32Qex(7)=32 by Huber et al. [Phys. Rev. Lett. 118, 200502 (2017)]. In this paper, we give a general upper bound of Qex(n)\mathrm{Qex}(n)Qex(n) by linking the well-known Tur\'an problem in graph theory and provide lower bounds using constructive and probabilistic methods. In particular, we show that Qex(8)=56\mathrm{Qex}(8)=56Qex(8)=56, which is the third known value for this problem.
Nonlocality and quantum entanglement constitute two special aspects of the quantum correlations existing in quantum systems, which are of paramount importance in quantum-information theory. Traditionally, they have been regarded as identical (equivalent, in fact, for pure two qubit states, that is, Gisin's Theorem ), yet they constitute different resources. Describing nonlocality by means of the violation of several Bell inequalities, we obtain by direct optimization those states of two qubits that maximally violate a Bell inequality, in terms of their degree of mixture as measured by either their participation ratio R = 1/Tr(ρ 2 ) or their maximum eigenvalue λ max . This optimum value is obtained as well, which coincides with previous results. Comparison with entanglement is performed too. An example of an application is given in the XY model. In this novel approximation, we also concentrate on the nonlocality for linear combinations of pure states of two qubits, providing a closed form for their maximal nonlocality measure. The case of Bell diagonal mixed states of two qubits is also extensively studied. Special attention concerning the connection between nonlocality and entanglement for mixed states of two qubits is paid to the so-called maximally entangled mixed states. Additional aspects for the case of two qubits are also described in detail. Since we deal with qubit systems, we will perform an analogous study for three qubits, employing similar tools. Relation between distillability and nonlocality is explored quantitatively for the whole space of states of three qubits. We finally extend our analysis to four-qubit systems, where nonlocality for generalized Greenberger–Horne–Zeilinger states of arbitrary number of parties is computed.
From both theoretical and experimental points of view symmetric states constitute an important class of multipartite states. Still, entanglement properties of these states, in particular those with positive partial transposition (PPT), lack a systematic study. Aiming at filling in this gap, we have recently affirmatively answered the open question of existence of four-qubit entangled symmetric states with PPT and thoroughly characterized entanglement properties of such states [J. Tura et al., Phys. Rev. A 85, 060302(R) (2012)]. With the present contribution we continue on characterizing PPT entangled symmetric states. On the one hand, we present all the results of our previous work in a detailed way. On the other hand, we generalize them to systems consisting of an arbitrary number of qubits. In particular, we provide criteria for separability of such states formulated in terms of their ranks. Interestingly, for most of the cases, the symmetric states are either separable or typically separable. Then, edge states in these systems are studied, showing in particular that to characterize generic PPT entangled states with four and five qubits, it is enough to study only those that assume few (respectively, two and three) specific configurations of ranks. Finally, we numerically search for extremal PPT entangled states in such systems consisting of up to 23 qubits. One can clearly notice regularity behind the ranks of such extremal states, and, in particular, for systems composed of odd numbers of qubits we find a single configuration of ranks for which there are extremal states.
We prove the existence of bound entangled states with negative partial transpose (NPT) in any d × d(d ≥ 3) Hilbert space with a simple assumption on Schmidt rank two states. Obviously they belong to the class of conjectured to be bound entangled states by Divincenzo et.al [Phys. Rev. A, 61, 062312(2000)] and by Dür et.al [Phys. Rev. A, 61, 062313(2000)]. PACS number(s): 03.67.Hk, 03.65.Ud. The basic issue on the classification of mixed state entanglement at least on the level of bipartite systems solely depends upon whether there exist bound entangled states or not. The existence of PPT-bound (PPT means positive partial transpose) entangled states [1] and also the existence of NPT N−copy undistillable states [2, 3] for every positive integer N naturally indicates there may exist NPT-bound entangled states. In this work we are able to show the existence of NPT-bound entangled states with a simple assumption on Schmidt rank two states. We first briefly describe the issue and the importance of the problem. In recent years it is found that quantum entanglement is an useful resource in performing several tasks in quantum information theory and quantum communication [4]. Maximally entangled states shared between two parties are essential ingredients in this respect [5]. Now due to the interaction with environment, states are in practice found to be mixed. However there is a process called distillation by which we can distill sometimes maximally entangled