We present a scalable method for electrically tuning multiple spatially separated quantum dots embedded in photonic crystal waveguides. Ion implantation into the top p-doped layer of a p-i-n diode creates high-resistivity tracks, providing electrical isolation between adjacent regions. Unlike physical etching, this method preserves the guided-mode profile of the photonic crystal without introducing significant scattering, limiting refractive index perturbations to below 0.001 with 0.01% additional loss. In contrast, physical etching can reduce single-band transmission by more than 30% for an etch width of 100 nm. We demonstrate the applicability of our approach using quantum dots embedded in a glideplane photonic crystal waveguide, controlling the detuning between different spin-state combinations of two highly chiral quantum dots coupled to the same mode. Second-order photon correlation measurements provide a sensitive probe of the chirality-dependent photon statistics, which are in good agreement with a waveguide-QED master equation model. Our results mark an important step towards scalable, multi-emitter architectures for chiral quantum networks.
We present a scalable method for electrically tuning multiple spatially separated quantum dots embedded in photonic crystal waveguides. Ion implantation into the top p-doped layer of a p-i-n diode creates high-resistivity tracks, providing electrical isolation between adjacent regions. Unlike physical etching, this method preserves the guided-mode profile of the photonic crystal without introducing significant scattering, limiting refractive index perturbations to below 0.001 with 0.01% additional loss. In contrast, physical etching can reduce single-band transmission by more than 30% for an etch width of 100 nm. We demonstrate the applicability of our approach using quantum dots embedded in a glideplane photonic crystal waveguide, controlling the detuning between different spin-state combinations of two highly chiral quantum dots coupled to the same mode. Second-order photon correlation measurements provide a sensitive probe of the chirality-dependent photon statistics, which are in good agreement with a waveguide-QED master equation model. Our results mark an important step towards scalable, multi-emitter architectures for chiral quantum networks.
Radiative coupling between quantum emitters leads to a range of spectacular emission phenomena. Dicke studied the foundations of collectively enhanced and suppressed decay, commonly referred to as super- and subradiance. Collective effects can further result in directionality of the emission, thus offering a complimentary implementation of chiral quantum optics. Waveguide quantum electrodynamics (QED) allows coupling between spatially separated emitters, enabling selective driving. In this work, we control the emission direction for a pair of quantum dots embedded in a bidirectional photonic crystal waveguide offering independent electrical tuning. Notably the emitters are 13 \micro m apart, which corresponds to 26 effective wavelengths, but are nevertheless radiatively coupled. The directionality arises from a dispersive dipole-dipole interaction, which shifts the energy of the collective states, so that the emitter pair effectively forms an artificial molecule. We show that the emission direction can be switched from left- to rightwards by manipulating the relative driving phase while collectively exciting the emitters. In addition, we observe directional photon statistics under continuous driving, with, for example, single photons detected on one output port, and photon pairs on the other. With pulsed excitation, both emitters are fully inverted and correlated photon pairs are observed in time-resolved intensity correlation measurements. This work demonstrates a novel implementation of chiral quantum optics using quantum dots coupled via a non-chiral waveguide, and reports key steps for scaling up as a multi-emitter waveguide QED platform.
Quantum photonics is a rapidly developing platform for future quantum network applications. Waveguide-based architectures, in which embedded quantum emitters act as both nonlinear elements to mediate photon–photon interactions and as highly coherent single-photon sources, offer a highly promising route to realize such networks. A key requirement for the scale-up of the waveguide architecture is local control and tunability of individual quantum emitters. Here, we demonstrate electrical control, tuning, and switching of the nonlinear photon–photon interaction arising due to a quantum dot embedded in a single-mode nano-photonic waveguide. A power-dependent waveguide transmission extinction as large as 40±2% is observed on resonance. Photon statistics measurements show clear, voltage-controlled bunching of the transmitted light and antibunching of the reflected light, demonstrating the single-photon, quantum character of the nonlinearity. Importantly, the same architecture is also shown to act as a source of highly coherent, electrically tunable single photons. Overall, the platform presented addresses the essential requirements for the implementation of photonic gates for scalable nano-photonic-based quantum information processing.
The generation of indistinguishable single photons and control of photon-photon interactions are key requirements for photonic quantum networks. Nano-photonic waveguide-based architectures, in which few-level solid state systems provide both single photon generation and the nonlinearity through which two or more photons interact, offer a scalable route to such networks. However, it is a challenge to maintain the optical quality of the embedded photon sources whilst also providing fine-tuning of the emission frequency and optical nonlinearity in a waveguide geometry. We demonstrate a tunable solid-state platform for scalable photonic quantum networks which allows local electrical control of both single photon generation and optical nonlinearity at the single photon level. Electrical tuning and switching of coherent photon scattering from a quantum dot embedded in a nano-photonic waveguide is demonstrated, with a transmission extinction as large as 40±2% measured on resonance. Observation of a clear, voltage-controlled bunching signal in the photon statistics of the transmitted light demonstrates the single photon character of the nonlinearity. The deterministic nature of the nonlinearity is particularly attractive for the future realization of photonic gates for scalable nano-photonic waveguide-based quantum information processing.
We identify chiral inversion points in slow-light, glide-plane-symmetric, photonic-crystal waveguides, defined as fixed locations where the local optical chirality changes sign over a narrow wavelength range. We experimentally access this behaviour using a waveguide-embedded InAs/InGaAs quantum dot. The slow-light spectral region is determined from time-integrated and time-resolved photoluminescence, and the dot exciton is electrically tuned across the slow-light bandwidth via the quantum-confined Stark effect. As the emission wavelength is swept through the slow-light region, the directional emission contrast shows a strong wavelength dependence and a sign reversal, consistent with the identified chiral inversion point. Numerical simulations attribute the switching primarily to the pronounced spectral variation of the local optical chirality for emitters displaced from the waveguide center. These results demonstrate on-demand electrical switching of chiral light-matter coupling in nanophotonic waveguides and enable tunable chiral interfaces for integrated quantum photonic devices.
The ability to engineer chiral light-matter interactions is a valuable resource for realizing quantum networks and non-reciprocal quantum optics. Here, we demonstrate chiral coupling between light and a negatively charged exciton state, i.e., a four-level system, embedded in a standard photonic-crystal waveguide. By controlling the orientation and strength of an external magnetic field, we tune the polarization of the individual optical transition dipoles relative to the fixed elliptically polarized waveguide mode. In a two-sided waveguide, an optimized oblique magnetic field allows a selected transition to decay exclusively into a single propagation direction, enabling near-unity directional emission (0.99−0.02+0.01), despite the waveguide exhibiting imperfect polarization for chiral coupling. We further observe two tunable chiral branching ratios, the directional analogue of optical cyclicity, for two Λ-systems, with one reaching 134−77+∞. The magnetic-field-dependent spectroscopy also allows reconstruction of the local guided-mode polarization at the emitter via the Stokes parameters relative to the emitter's dipole moments. Finally, we demonstrate that this local chirality enables coherent control of an electron spin via an optical Raman process mediated by waveguide driving. Building on the simultaneous realization of a large branching ratio, directionality and spin control achieved at the same oblique magnetic-field angle, we propose a protocol with high tolerance to photon loss for generating high-fidelity remote spin-spin entanglement. Our magnetic control opens a reconfigurable and generic route for enhancing on-chip chiral spin-photon coupling in standard nanophotonic interfaces without the need to carefully engineer the polarization of the waveguide.
Abstract Chiral quantum optics has attracted considerable interest in the field of quantum information science. Exploiting the spin‐polarization properties of quantum emitters and engineering rational photonic nanostructures has made it possible to transform information from spin to path encoding. Here, compact chiral photonic circuits with deterministic circularly polarized chiral routing and beamsplitting are demonstrated using two laterally adjacent waveguides coupled with quantum dots. Chiral routing arises from the electromagnetic field chirality in waveguide, and beamsplitting is obtained via the evanescent field coupling. The spin‐ and position‐dependent directional spontaneous emission are achieved by spatially selective micro‐photoluminescence measurements, with a chiral contrast of up to 0.84 in the chiral photonic circuits. This makes a significant advancement for broadening the application scenarios of chiral quantum optics and developing scalable quantum photonic networks.