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arXiv:2511.06097

Quantum Optimal Control of a Lambda System in the Density Matrix Formulation

Julia Cen, Domenico D'Alessandro

quant-phSubmitted Nov 8, 2025• Announced Nov 11, 2025• 0 citations
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Abstract

In various physical implementations of quantum information processing, qubits are realized in a Lambda type system configuration as two stable lower energy levels coupled indirectly via an unstable higher energy level, that is, in comparison, a lot more susceptible to decoherence. We consider the quantum control problem of optimal state transfer between two isospectral density matrices, over an arbitrary finite time horizon, for the quantum Lambda system. The cost considered is a compromise between the energy of the control field and the average occupancy in the highest energy level. We apply a geometric approach that combines the use of the Pontryagin Maximum Principle, a symmetry reduction technique to reduce the number of parameters in the resulting optimization problem, and several auxiliary techniques to bound the parameter space in the search for the optimal solution. We prove several properties of the optimal control and trajectories for this problem, including their normality and smoothness. We obtain a system of differential equations that must be satisfied by the optimal pair of control and trajectory we treat in detail, with numerical simulations, and solve a case study involving a Hadamard-like transformation. Our techniques can be adapted to other contexts and promise to push to a more consequential level, the application of geometric control in quantum systems.

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In various physical implementations of quantum information processing, qubits are realized in a Lambda type system configuration as two stable lower energy levels coupled indirectly via an unstable higher energy level, that is, in comparison, a lot more susceptible to decoherence. We consider the quantum control problem of optimal state transfer between two isospectral density matrices, over an arbitrary finite time horizon, for the quantum Lambda system. The cost considered is a compromise between the energy of the control field and the average occupancy in the highest energy level. We apply a geometric approach that combines the use of the Pontryagin Maximum Principle, a symmetry reduction technique to reduce the number of parameters in the resulting optimization problem, and several auxiliary techniques to bound the parameter space in the search for the optimal solution. We prove several properties of the optimal control and trajectories for this problem, including their normality and smoothness. We obtain a system of differential equations that must be satisfied by the optimal pair of control and trajectory we treat in detail, with numerical simulations, and solve a case study involving a Hadamard-like transformation. Our techniques can be adapted to other contexts and promise to push to a more consequential level, the application of geometric control in quantum systems.
We study the time-optimal robust control of a two-level quantum system subjected to field inhomogeneities. We apply the Pontryagin maximum principle and we introduce a reduced space onto which the optimal dynamics is projected down. This reduction leads to a complete analytical derivation of the optimal solution in terms of elliptic functions and elliptic integrals. Necessary optimality conditions are then obtained for the original system. These conditions are verified numerically and lead to the optimal control protocol. Various examples, ranging from state-to-state transfer to the generation of a NOT gate, illustrate this study. The connection with other geometric optimization approaches that have been used to solve this problem is also discussed. Finally, we show how this method can be combined with numerical optimization algorithms to design robust control for higher-dimensional quantum systems, as illustrated by a Bose-Einstein condensate in an optical lattice.
In this work, we address the problem of maximizing fidelity in a quantum state transformation process controlled in such a way as to keep decoherence within given bounds. We consider a three-level Λ-type atom subjected to Markovian decoherence characterized by non-unital decoherence channels. We introduce fidelity as the performance index for the quantum state transformation process since the goal is to maximize the similarity of the final state density operator with the one of the desired target state. We formulate the quantum optimal control problem with state constraints where the latter reflect the fact that the decoherence level remains within a pre-defined bound. Optimality conditions of Pontryagin’s Maximum Principle in Gamkrelidze’s form are given. These provide a complete set of relations enabling the computation of the optimal control strategy. This is a novel approach in the context of quantum systems.
In this paper, we demonstrate an approach to quantum robust control based on the tools of geometric optimal control. The central objects of interest are the sensitivity functions defined as the coefficients in the Taylor expansion of the trajectory with respect to the (unknown, small) parameters which describe the deviation of the actual model from nominal one. In terms of these quantities, we formalize an optimal control problem where one searches for the optimal nominal trajectory which minimizes the size of the sensitivity while taking into account other aspects of the control design such as the energy of the control field. We consider in detail the case of a single qubit with a dephasing Hamiltonian term, and the optimal control problem of obtaining a state transfer by minimizing the weighted sum of the energy of the controlling field and the first order sensitivity. At the limit of a very large weight on the sensitivity, we obtain the optimal control which zeros the sensitivity and minimizes the control field energy. This problem has a rich mathematical structure which enables its solution in terms of elliptic integrals. For this problem, we obtain an explicit solution which is particularly simple and also smooth, avoiding discontinuities which are present in other approaches. We extend the results to the robust control of two quantum bits minimizing cross-talk contamination, as we show that such a problem decouples in two independent one qubit problems.
We consider the problem of time-optimal control for a three-level quantum system where one level is coupled by the control field to the lowest two, which are not coupled to each other. A bound is assumed on the norm of the control at every time. Such a problem belongs to the class of KP sub-Riemannian problems for which we can perform a symmetry reduction and reduce to a Riemannian problem on the associated quotient space. We prove several properties of such a quotient space in our case, including the fact that it is an example of an almost-Kähler manifold that is not Kähler. We provide the explicit form of the optimal controls for any unitary transformation on the lowest two levels and discuss the geometric and practical implications of this result.
We address a control-constrained optimal control problem pertaining to the transformation of quantum states. Our objective is to steer a quantum system from an initial state to a desired target state while adhering to the principles of the Liouville-von Neumann equation. To achieve this, we introduce a cost functional that balances the dual goals of fidelity maximization and energy consumption minimization. We derive optimality conditions in the form of the Pontryagin Maximum Principle (PMP) for the matrix-valued dynamics associated with this problem. Subsequently, we present a time discretized computational scheme designed to solve the optimal control problem. This computational scheme is rooted in an indirect method grounded in the PMP, showcasing its versatility and efficacy. To illustrate the practicality and applicability of our methodology, we employ it to address the case of a spin ½ particle subjected to interaction with a magnetic field. Our findings shed light on the potential of this approach to tackle complex quantum control scenarios and contribute to the broader field of quantum state transformations.
Optimal Control Theory is a powerful mathematical tool, which has known a rapid development since the 1950s, mainly for engineering applications. More recently, it has become a widely used method to improve process performance in quantum technologies by means of highly efficient control of quantum dynamics. This tutorial aims at providing an introduction to key concepts of optimal control theory which is accessible to physicists and engineers working in quantum control or in related fields. The different mathematical results are introduced intuitively, before being rigorously stated. This tutorial describes modern aspects of optimal control theory, with a particular focus on the Pontryagin Maximum Principle, which is the main tool for determining open-loop control laws without experimental feedback. The different steps to solve an optimal control problem are discussed, before moving on to more advanced topics such as the existence of optimal solutions or the definition of the different types of extremals, namely normal, abnormal, and singular. The tutorial covers various quantum control issues and describes their mathematical formulation suitable for optimal control. The connection between the Pontryagin Maximum Principle and gradient-based optimization algorithms used for high-dimensional quantum systems is described. The optimal solution of different low-dimensional quantum systems is presented in detail, illustrating how the mathematical tools are applied in a practical way.