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arXiv:2511.00570

Quantum-coherent optical isolation and circulation using frequency conversion on a chip

Jierui Hu, Hao Yuan, Joshua Akin, Shanhui Fan, Kejie Fang

Published Nov 1, 2025• 0 citations
arXivHTMLPDF

Abstract

Breaking optical reciprocity enables new regimes of light--matter interaction with broad implications for fundamental physics and emerging quantum technologies. Although various approaches have been explored to achieve optical nonreciprocity, realizing it at the single-photon level has remained a major challenge. Here, we demonstrate nonmagnetic optical nonreciprocity -- including both isolation and circulation -- in the quantum regime, enabled by efficient and noiseless all-optical frequency conversion on an integrated III-V photonic chip. Our device preserves the quantum coherence and entanglement of the input photons while delivering exceptional performance parameters, including a high extinction ratio of 34 dB, low insertion loss of 0.8 dB, broad bandwidth of 44 GHz, high operational fidelity of 97%, and widely tunable operation wavelength. This realization of quantum optical nonreciprocity in a scalable photonic platform opens a pathway toward directional quantum communication and noise-resilient quantum networks.

DOI
10.48550/arxiv.2511.00570

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Breaking optical reciprocity enables new regimes of light--matter interaction with broad implications for fundamental physics and emerging quantum technologies. Although various approaches have been explored to achieve optical nonreciprocity, realizing it at the single-photon level has remained a major challenge. Here, we demonstrate nonmagnetic optical nonreciprocity -- including both isolation and circulation -- in the quantum regime, enabled by efficient and noiseless all-optical frequency conversion on an integrated III-V photonic chip. Our device preserves the quantum coherence and entanglement of the input photons while delivering exceptional performance parameters, including a high extinction ratio of 34 dB, low insertion loss of 0.8 dB, broad bandwidth of 44 GHz, high operational fidelity of 97%, and widely tunable operation wavelength. This realization of quantum optical nonreciprocity in a scalable photonic platform opens a pathway toward directional quantum communication and noise-resilient quantum networks.
Breaking electromagnetic reciprocity enables directional control of light and is essential for both classical and quantum photonic systems. However, realizing integrated optical nonreciprocity that simultaneously combines low loss, broad bandwidth, and compatibility with quantum states of light remains a major challenge. Here, we demonstrate optical nonreciprocity based on quantum frequency conversion in an integrated [Formula: see text] nonlinear waveguide. Operating from classical power levels down to the single-photon level, the device preserves quantum coherence and entanglement of the input photons. We achieve an isolation of 34 decibels with a low on-chip insertion loss of 0.8 decibels and a broad isolation bandwidth, together with a four-port circulator exhibiting an operational fidelity of up to 0.97. Our results establish parametric frequency conversion as a scalable and quantum-compatible route toward integrated nonreciprocal photonic devices for applications in quantum communication and noise-resilient photonic networks.
Nonreciprocal devices operating at the single-photon level are fundamental elements for quantum technologies. Because magneto-optical nonreciprocal devices are incompatible for magnetic-sensitive or on-chip quantum information processing, all-optical nonreciprocal isolation is highly desired, but its realization at the quantum level is yet to be accomplished at room temperature. Here, we propose and experimentally demonstrate two regimes, using electromagnetically induced transparency (EIT) or a Raman transition, for all-optical isolation with warm atoms. We achieve an isolation of 22.52 ± 0.10 dB and an insertion loss of about 1.95 dB for a genuine single photon, with bandwidth up to hundreds of megahertz. The Raman regime realized in the same experimental setup enables us to achieve high isolation and low insertion loss for coherent optical fields with reversed isolation direction. These realizations of single-photon isolation and coherent light isolation at room temperature are promising for simpler reconfiguration of high-speed classical and quantum information processing.
Optical nonreciprocity is an essential property for a wide range of applications, such as building nonreciprocal optical devices that include isolators and circulators. The realization of optical nonreciprocity relies on breaking the symmetry associated with Lorentz reciprocity, which typically requires stringent conditions such as introducing a strong magnetic field or a high-finesse cavity with nonreciprocal coupling geometry. Here we discover that the collision effect of thermal atoms, which is undesirable for most studies, can induce broadband optical nonreciprocity. By exploiting the thermal atomic collision, we experimentally observe magnet-free and cavity-free optical nonreciprocity, which possesses a high isolation ratio, ultrabroad bandwidth, and low insertion loss simultaneously. The maximum isolation ratio is close to 40 dB, while the insertion loss is less than 1 dB. The bandwidth for an isolation ratio exceeding 20 dB is over 1.2 GHz, which is 2 orders of magnitude broader than typical resonance-enhanced optical isolators. Our work paves the way for the realization of high-performance optical nonreciprocal devices and provides opportunities for applications in integrated optics and quantum networks.
We propose an all-optical approach to achieve optical nonreciprocity on a chip by quantum squeezing one of two coupled resonator modes. By parametric pumping a χ^{(2)}-nonlinear resonator unidirectionally with a classical coherent field, we squeeze the resonator mode in a selective direction due to the phase-matching condition, and induce a chiral photon interaction between two resonators. Based on this chiral interresonator coupling, we achieve an all-optical diode and a three-port quasicirculator. By applying a second squeezed-vacuum field to the squeezed resonator mode, our nonreciprocal device also works for single-photon pulses. We obtain an isolation ratio of >40 dB for the diode and fidelity of >98% for the quasicirculator, and insertion loss of <1 dB for both. We also show that nonreciprocal transmission of strong light can be switched on and off by a relative weak pump light. This achievement implies a nonreciprocal optical transistor. Our protocol opens up a new route to achieve integrable all-optical nonreciprocal devices permitting chip-compatible optical isolation and nonreciporcal quantum information processing.
A scheme for magnetic-free optical nonreciprocity in an ensemble of four-level cold atoms is proposed by exploiting the directional four-wave mixing effect. Using experimentally achievable parameters, the nonreciprocal optical responses of the system can be observed and the conversion on nonreciprocal transmission and nonreciprocal phase shift can be implemented. These nonreciprocal phenomena originate from the directional phase matching, which breaks the time-reversal symmetry and dynamic reciprocity of the cold atomic system. Moreover, by embedding the cold atoms into a Mach-Zehnder interferometer and choosing proper parameters, a two-port optical isolator with an isolation ratio of 79.70 dB and an insertion loss of 0.35 dB and a four-port optical circulator with a fidelity of 0.9985 and a photon survival probability of 0.9278 can be realized, which shows the high performance of isolation and circulation. The proposal may enable a new class of optically controllable cavity-free nonreciprocal devices in optical signal processing at the low light level.
On-chip single-photon nonreciprocal devices with high isolation and low insertion loss become a key element in quantum information processing. Based on electromagnetically induced transparency in chiral quantum systems, a single-photon isolator and a single-photon circulator are obtained without requiring unbalanced coupling. These devices have high isolation and low insertion loss. Moreover, their bandwidths are significantly broadened with the assistance of electromagnetically induced transparency.