Extending classical synchronization to the quantum domain is of great interest both from the fundamental physics point of view and with a view toward quantum technology applications. This work characterizes phase synchronization of an effective spin-1 system, which is realized by coupling three quantum states with infinite lifetime to auxiliary excited states that have a finite lifetime. Integrating out the excited states, the effective spin-1 model features coherent and incoherent effective couplings. Our key findings are: (i) Phase synchronization can be controlled by adjusting the phases of the couplings to the excited states. (ii) Unlike in the paradigmatic spin-1 system studied in the literature, where the dissipative couplings describe decay into the limit cycle state, the effective spin-1 model investigated in this work is governed by a competition between dissipative decay into and out of the limit cycle state, with the dissipative decay out of the limit cycle state playing a critical role. (iii) We identify a parameter regime where phase synchronization of the effective spin-1 system is -- in the absence of coherent effective couplings -- governed entirely by the effective dissipators. The effective spin-1 model is benchmarked through comparisons with master equation calculations for the full Hilbert space. Physical insights are gained through analytical perturbation theory calculations. Our findings, which are expected to hold for a broad class of energy level and coupling schemes, are demonstrated using hyperfine states of $^{87}$Rb.
Extending classical synchronization to the quantum domain is of great interest both from the fundamental physics point of view and with a view toward quantum technology applications. This work characterizes phase synchronization of an effective spin-1 system, which is realized by coupling three quantum states with infinite lifetime to auxiliary excited states that have a finite lifetime. Integrating out the excited states, the effective spin-1 model features coherent and incoherent effective couplings. Our key findings are: (i) Phase synchronization can be controlled by adjusting the phases of the couplings to the excited states. (ii) Unlike in the paradigmatic spin-1 system studied in the literature, where the dissipative couplings describe decay into the limit cycle state, the effective spin-1 model investigated in this work is governed by a competition between dissipative decay into and out of the limit cycle state, with the dissipative decay out of the limit cycle state playing a critical role. (iii) We identify a parameter regime where phase synchronization of the effective spin-1 system is -- in the absence of coherent effective couplings -- governed entirely by the effective dissipators. The effective spin-1 model is benchmarked through comparisons with master equation calculations for the full Hilbert space. Physical insights are gained through analytical perturbation theory calculations. Our findings, which are expected to hold for a broad class of energy level and coupling schemes, are demonstrated using hyperfine states of 87Rb.
With growing interest in quantum technologies, possibilities of synchronizing quantum systems have garnered significant recent attention. In experiments with dilute ensemble of laser cooled spin-1 ^{87}Rb atoms, we observe phase difference of spin coherences to synchronize with phases of external classical fields. An initial limit-cycle state of a spin-1 atom localizes in phase space due to dark-state polaritons generated by classical two-photon tone fields. In particular, when the two couplings fields are out of phase, the limit-cycle state synchronizes only with two artificially engineered, anisotropic decay rates. Furthermore, we observe a blockade of synchronization due to quantum interference and emergence of Arnold-tongue-like features. Such anisotropic decay induced synchronization of spin-1 systems with no classical analog can provide insights in open quantum systems and find applications in synchronized quantum networks.
We experimentally investigate quantum synchronization for one of the simplest possible quantum systems, namely an externally driven few-level system with equally spaced energy levels effectively acting as a spin-1 system. Coupling to excited auxiliary states, we realize additive effective Lindblad operators that are associated with non-conventional dissipative pathways, which are shown to enhance, in certain parameter regimes, quantum synchronization. The experimental set-up, which utilizes cold 87Rb atoms in a MOT, and associated synchronization extraction protocol are benchmarked carefully through dedicated simulations. Convincing agreement is found between experiment and simulations. The dissipation engineering approach established in our work can be readily extended to systems with more energy levels, such as effective spin-3/2 or spin-2 systems, and has implications for quantum synchronization studies in higher-spin systems as well as for a wide range of quantum science studies and technology applications.
Synchronization is a collective phenomenon in which interacting nonlinear oscillators develop a persistent relation between their phases and frequencies. In quantum systems, its description requires connecting the classical dynamics of limit-cycle oscillators with quantum fluctuations, dissipation, and the notion of phase. In this tutorial review, we offer a systematic framework for analyzing synchronization in classical and quantum dynamical systems. Starting from amplitude-phase dynamics, we introduce successively topics of relevance, such as phase locking, the Adler equation, Arnold tongues, and the Kuramoto model, and use these concepts to analyze coupled oscillators and their stability. We then formulate the corresponding description for quantum limit-cycle oscillators using Lindblad master equations and phase-space methods, with explicit examples of two and many coupled oscillators. We further discuss noise, synchronization measures, and the extreme quantum regime, including synchronization in spin systems. The emphasis throughout is on analytical derivations and a practical methodology for identifying synchronized states, determining their stability, and characterizing synchronization in quantum systems. The review is designed as a self-contained guide from which we hope that students can learn the essential concepts and techniques, while researchers can readily find the analytical tools and methodological insights needed to approach new synchronization problems.
Recently, it was shown that dissipative quantum systems with three or more levels are able to synchronize to an external signal. Some researchers have stated that this is not possible for two-level systems, as those systems lack a stable limit cycle in unperturbed dynamics, but others have demonstrated, under a different definition of synchronization, that it is possible in qubits in models which include other elements. We show how a quantum two-level system can be understood as containing a valid limit cycle as the starting point of synchronization and that it can synchronize its dynamics to an external weak signal. This is demonstrated by analytically solving the Lindblad equation of a two-level system coupled to an environment, determining the steady state. This is a mixed state with contributions from many pure states, each of which provides a valid limit cycle. We show that this is sufficient to phase lock the dynamics to a weak external signal, hence clarifying synchronization in two-level systems. We use the Husimi Q representation to analyze the synchronization region, defining a synchronization measure which characterizes the strength of the phase locking. Also, we study the stability of the limit cycle and its deformation with the strength of the signal in terms of the components of the Bloch vector of the system. Finally, we generalize a model of the three-level system to illustrate how the stationary fixed point of that model can be changed into a limit cycle similar to the one that we describe for the two-level system.
Among the most iconic features of classical dissipative dynamics are persistent limit-cycle oscillations and critical slowing down at the onset of such oscillations, where the system relaxes purely algebraically in time. On the other hand, quantum systems subject to generic Markovian dissipation decohere exponentially in time, approaching a unique steady state. Here we show how coherent limit-cycle oscillations and algebraic decay can emerge in a quantum system governed by a Markovian master equation as one approaches the classical limit, illustrating general mechanisms using a single-spin model and a two-site lossy Bose-Hubbard model. In particular, we demonstrate that the fingerprint of a limit cycle is a slow-decaying branch with vanishing decoherence rates in the Liouville spectrum, while a power-law decay is realized by a spectral collapse at the bifurcation point. We also show how these are distinct from the case of a classical fixed point, for which the quantum spectrum is gapped and can be generated from the linearized classical dynamics.
The study of phase transitions in dissipative quantum systems based on the Liouvillian is often hindered by the difficulty of constructing a time-local master equation when the system-environment coupling is strong. To address this issue, the complex discretization approximation for the environment is proposed to study the quantum phase transition in the extended Jaynes-Cumming model with an infinite number of boson modes. This approach yields a non-Hermitian effective Hamiltonian that can be used to simulate the dynamics of the spin. It is found that the ground state of this effective Hamiltonian determines the spin dynamics in the single-excitation subspace. Depending on the opening of the energy gap and the maximum population of excitations on the spin degree of freedom, three distinct phases can be identified: fast decaying, localized, and stretched dynamics of the spin. This approach can be extended to multiple excitations, and similar dynamics were found in the double-excitation subspace, indicating the robustness of the single-excitation phase.