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arXiv:2510.22615 · Physical Review Applied

Sensitive detection of the Rydberg transition in trapped electrons on liquid helium using radio-frequency reflectometry

J.-Y. Lin, Tomoyuki Tani, Mikhail Belianchikov, Denis Konstantinov

Published Jul 13, 2026• 0 citations
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Abstract

Radio-frequency reflectometry, which probes small changes in the electrical impedance of a device, provides a useful method for sensitive and fast detection of dynamic processes in quantum systems. We use this method to detect excitation of the quantized motional (Rydberg) states of trapped electrons on liquid helium. The Rydberg transition in an ensemble of electrons is detected by a change in the impedance of an rf circuit coupled to the microwave-excited electrons. To elucidate the origin of the observed response, the result is compared with an independent impedance measurement on the same electron system modulated by an electrostatic potential and with a numerical simulation using the Green's function method. Additionally, it is found that the rf response to the Rydberg resonance can be strongly enhanced by a resonant mode of the electron collective motion. Our results suggest that the observed response to the Rydberg resonance must be attributed to the lateral motion of the many-electron system rather than the vertical displacement of the individually excited electrons, as was explicate earlier. A theoretical analysis of the expected response due to the vertical displacement is given.

DOI
10.1103/4fx7-fk1z

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Radio-frequency reflectometry, which probes small changes in the electrical impedance of a device, provides a useful method for sensitive and fast detection of dynamic processes in quantum systems. We use this method to detect excitation of the quantized motional (Rydberg) states of trapped electrons on liquid helium. The Rydberg transition in an ensemble of electrons is detected by a change in the impedance of an rf circuit coupled to the microwave-excited electrons. To elucidate the origin of the observed response, the result is compared with an independent impedance measurement on the same electron system modulated by an electrostatic potential and with a numerical simulation using the Green's function method. Additionally, it is found that the rf response to the Rydberg resonance can be strongly enhanced by a resonant mode of the electron collective motion. Our results suggest that the observed response to the Rydberg resonance must be attributed to the lateral motion of the many-electron system rather than the vertical displacement of the individually excited electrons, as was explicate earlier. A theoretical analysis of the expected response due to the vertical displacement is given.
Electrons trapped on the surface of superfluid helium have been thought of as a useful resource for quantum computing. Such electrons show long coherence of their surface-bound (Rydberg) states combined with their easy electrostatic manipulation. Recent proposals have explored the possibility of coupling the spin state of an electron and the state of its quantized motion, with the promise of a highly scalable two-dimensional architecture for a quantum computer. However, despite recent progress in the detection of quantized lateral motion of electrons using a circuit-QED setup, manipulation of a small number of electrons and their quantum state detection remains a challenging problem. Here, we report on the detection of the Rydberg transition of electrons on superfluid helium in an on-chip microchannel device in which electrons are moved and trapped by a set of electrostatic gates. A highly sensitive image-charge detection system allows us to not only resolve the transition spectra of such electrons, but also perform the device characterization. The demonstrated sensitivity shows the feasibility of detecting the Rydberg transition of a single electron, which can open an alternate pathway for a nondestructive spin-state readout.
Many important phenomena in quantum devices are dynamic, meaning that they cannot be studied using time-averaged measurements alone. Experiments that measure such transient effects are collectively known as fast readout. One of the most useful techniques in fast electrical readout is radio-frequency reflectometry, which can measure changes in impedance (both resistive and reactive) even when their duration is extremely short, down to a microsecond or less. Examples of reflectometry experiments, some of which have been realized and others so far only proposed, include projective measurements of qubits and Majorana devices for quantum computing, real-time measurements of mechanical motion, and detection of non-equilibrium temperature fluctuations. However, all of these experiments must overcome the central challenge of fast readout: the large mismatch between the typical impedance of quantum devices (set by the resistance quantum) and of transmission lines (set by the impedance of free space). Here, we review the physical principles of radio-frequency reflectometry and its close cousins, measurements of radio-frequency transmission and emission. We explain how to optimize the speed and sensitivity of a radio-frequency measurement and how to incorporate new tools, such as superconducting circuit elements and quantum-limited amplifiers into advanced radio-frequency experiments. Our aim is threefold: to introduce the readers to the technique, to review the advances to date, and to motivate new experiments in fast quantum device dynamics. Our intended audience includes experimentalists in the field of quantum electronics who want to implement radio-frequency experiments or improve them, together with physicists in related fields who want to understand how the most important radio-frequency measurements work.
The quantized lateral motional states and the spin states of electrons trapped on the surface of superfluid helium have been proposed as basic building blocks of a scalable quantum computer.Circuit quantum electrodynamics allows strong dipole coupling between electrons and a high-Q superconducting microwave resonator, enabling such sensitive detection and manipulation of electron degrees of freedom.Here, we present the first realization of a hybrid circuit in which a large number of electrons are trapped on the surface of superfluid helium inside a coplanar waveguide resonator.The high finesse of the resonator allows us to observe large dispersive shifts that are many times the linewidth and make fast and sensitive measurements on the collective vibrational modes of the electron ensemble, as well as the superfluid helium film underneath.Furthermore, a large ensemble coupling is observed in the dispersive regime during experiment, and it shows excellent agreement with our numeric model.The coupling strength of the ensemble to the cavity is found to be ≈1 MHz per electron, indicating the feasibility of achieving single electron strong coupling.
Abstract Electrons trapped on the surface of liquid helium is an extremely clean system which holds promise for a scalable qubit platform. However, the superfluid surface is not free from fluctuations which might cause the decay and dephasing of the electron’s quantized states. Understanding and mitigating these fluctuations is essential for the advancement of electrons-on-helium qubit technology. Some work has been recently done to investigate surface oscillations due to the mechanical vibration of the cryostat using a superconducting coplanar waveguide resonator. In the present work, we focus on a sub-hertz frequency range and observe a strong effect of surface oscillations on the temporal dynamics of the Rydberg transition of electrons confined in a microchannel trapping device. We suggest possible origin of such oscillations and find a reasonable agreement between the corresponding estimation of the oscillation frequency and the observed result.
Dipole-dipole interactions between helium atoms in Rydberg-Stark states with principal quantum number n=53n=53n=53 and approximately linear Stark energy shifts, resulting from induced electric dipole moments of approximately 7900 D, have been investigated experimentally. The experiments were performed in pulsed supersonic metastable helium beams, with particle number densities of up to $\ensuremath{\sim}{10}^{9}\phantom{\rule{4pt}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3}$. In the presence of amplitude-modulated, radio-frequency electric fields, changes in the spectral intensity distributions associated with the transitions to these states that are attributed to dipole-dipole interactions within the ensembles of excited atoms have been observed. The experimental results are in excellent agreement with calculations of the Rydberg energy level structure carried out using Floquet methods, and excitations shared by up to four atoms. The use of these Rydberg-Stark states as sensors for nonresonant broadband radio-frequency electrical noise is also discussed.
Rydberg atoms show significant promise as the basis for highly sensitive detectors of continuous radio-frequency (rf) electric fields (E fields). Here, we study their time-dependent response to pulse-modulated rf E fields at 19.4 GHz using a cesium vapor cell at room temperature. We use density-matrix simulations to explain the timescales that shape the transient atomic response under different laser conditions, finding them to be limited by dephasing mechanisms, including transit-time broadening, Rydberg-Rydberg collisions, and ionization. Using a matched filter, we demonstrate the detection of individual pulses with durations from 10 \textmu{}s down to 50 ns and amplitudes from 15 000 \textmu{}V ${\mathrm{cm}}^{\ensuremath{-}1}$ down to about 170 \textmu{}V ${\mathrm{cm}}^{\ensuremath{-}1}$, corresponding to a sensitivity of about 240 nV ${\mathrm{cm}}^{\ensuremath{-}1}$ ${\mathrm{Hz}}^{\ensuremath{-}1/2}$. Finally, we highlight the potential of a Rydberg vapor cell as a receiver by detecting pulse trains from a rotating emitter on a simulated passing aircraft.