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arXiv:2510.17019 · Physical Review A

Modified Langevin noise formalism for multiple quantum emitters in dispersive electromagnetic environments out of equilibrium

Giovanni Miano, Loris Maria Cangemi, Carlo Forestiere

Published Jan 26, 2026• 2 citations
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Abstract

The control of interactions among quantum emitters through nanophotonic structures offers significant opportunities for quantum technologies. However, a rigorous theoretical description of the interaction of multiple quantum emitters with complex, dispersive dielectric objects remains challenging. Here, we introduce an approach based on the modified Langevin noise formalism that unveils the roles of both the noise polarization currents of the dielectrics and the vacuum fluctuations of the electromagnetic field scattered by the dielectrics. This work extends Refs. \cite{miano_quantum_2025} and \cite{miano_spectral_2025} to the general case of an arbitrary number of emitters. The proposed approach allows us to describe the dynamics of the quantum emitters for arbitrary initial quantum states of the electromagnetic environment, consisting of two independent bosonic reservoirs, a medium-assisted reservoir and a scattering-assisted reservoir, each characterized by its own spectral density matrix. Specifically, we examine situations where both reservoirs are initially in thermal quantum states but have different temperatures. Understanding how these reservoirs shape the dynamics of the emitters is crucial for understanding light-matter interactions in complex electromagnetic environments and for improving intrinsic emitter properties within structured environments.

DOI
10.1103/ps9g-1b4d

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The control of interactions among quantum emitters through nanophotonic structures offers significant opportunities for quantum technologies. However, a rigorous theoretical description of the interaction of multiple quantum emitters with complex, dispersive dielectric objects remains challenging. Here, we introduce an approach based on the modified Langevin noise formalism that unveils the roles of both the noise polarization currents of the dielectrics and the vacuum fluctuations of the electromagnetic field scattered by the dielectrics. This work extends Refs. \cite{miano_quantum_2025} and \cite{miano_spectral_2025} to the general case of an arbitrary number of emitters. The proposed approach allows us to describe the dynamics of the quantum emitters for arbitrary initial quantum states of the electromagnetic environment, consisting of two independent bosonic reservoirs, a medium-assisted reservoir and a scattering-assisted reservoir, each characterized by its own spectral density matrix. Specifically, we examine situations where both reservoirs are initially in thermal quantum states but have different temperatures. Understanding how these reservoirs shape the dynamics of the emitters is crucial for understanding light-matter interactions in complex electromagnetic environments and for improving intrinsic emitter properties within structured environments.
In this paper, we model the interaction of a quantum emitter with a finite-size dispersive dielectric object in unbounded space within the framework of macroscopic quantum electrodynamics, using the modified Langevin noise formalism. The quantized electromagnetic field consists of two contributions: the medium-assisted field, which accounts for the electromagnetic field generated by the noise polarization currents of the dielectric, and the scattering-assisted field, which takes into account the electromagnetic field incoming from infinity and scattered by the dielectric. We show that the emitter couples to two distinct bosonic reservoirs: a medium-assisted reservoir and a scattering-assisted reservoir, each characterized by its own spectral density. We then use emitter-centered modes to reduce the degrees of freedom of both reservoirs. Eventually, we identify the conditions under which the electromagnetic environment composed of these two reservoirs can be effectively replaced by a single bosonic reservoir so that the reduced time evolution of the quantum emitter remains unchanged. In particular, when the initial states of the medium- and scattering-assisted reservoirs are thermal quantum states at the same temperature, we find that a single bosonic bath with a spectral density equal to the sum of the medium- and scattering-assisted spectral densities is equivalent to the original electromagnetic environment.
In this paper, we model the interaction of a quantum emitter with a finite-size dispersive dielectric object in an unbounded space within the framework of macroscopic quantum electrodynamics, using the modified Langevin noise formalism, without any restrictions on the emitter level structure or dipole operator. The quantized electromagnetic field consists of two contributions: the medium-assisted field, which accounts for the electromagnetic field generated by the noise polarization currents of the dielectric, and the scattering-assisted field, which takes into account the electromagnetic field incoming from infinity and scattered by the dielectric. We show that the emitter couples to two distinct bosonic baths: a medium-assisted bath and a scattering-assisted bath, each characterized by its own spectral density. We identify the conditions under which the electromagnetic environment composed of these two baths can be effectively replaced by a single bosonic bath, so that the reduced dynamics of the quantum emitter remain unchanged. In particular, when the initial states of the medium- and scattering-assisted baths are thermal states with the same temperature, we find that a single bosonic bath with a spectral density equal to the sum of the medium-assisted and scattering-assisted spectral densities is equivalent to the original electromagnetic environment.
The modified Langevin noise formalism (MLNF) models the interaction of the quantized electromagnetic field with an arbitrary lossy magneto-dielectric object placed in vacuum using three types of non-interacting bosonic polaritons: scattering, electric, and magnetic. These respectively represent free-space photons scattered by the object, and photons radiated by quantized electric and magnetic dipolar sources embedded within its volume. Recently [A. Ciattoni, Phys. Rev. A 110, 013707 (2024)], this formalism was justified from the canonical quantization of macroscopic electromagnetism (CQME) [Philbin, New J. Phys. 12, 123008 (2010)] in the Heisenberg picture. This was achieved by identifying the polariton operators within the formal solution of the macroscopic Maxwell equations, assuming they obey bosonic commutation relations to retrieve the canonical ones, and showing they diagonalize the CQME Hamiltonian. However, the explicit functional dependence of these polaritons on the underlying canonical field operators remained undetermined. In this paper, we derive the exact analytical expressions for the polariton operators in terms of the canonical CQME field operators. Using these mappings, we provide a direct and rigorous derivation of the MLNF from the canonical theory in the Schrödinger picture. Our derivation is structured in three foundational steps: 1) adopting the derived analytical expressions as the constitutive definitions of the polariton operators; 2) mathematically proving that these operators are strictly bosonic as a direct consequence of the canonical commutation relations; and 3) demonstrating that they exactly diagonalize the macroscopic CQME Hamiltonian.
This work presents a full-wave Green's function framework for modeling collective and coherent single-photon emission from multiple quantum emitters embedded in complex electromagnetic structures. Starting from a transverse modal completeness relation of modified Langevin noise formalism, we derive a closed set of coupled equations for population dynamics and frequency-resolved field amplitudes in the single-excitation regime. Since the electromagnetic reservoir is not traced out at the level of the dynamical amplitudes, the emitted single-photon dynamics can be modeled within the same closed set of equations without Markovian approximation in open and dissipative environments. We demonstrate that finite-bandwidth truncation of the spectral density leads to systematic deviations in coherent dispersive interactions, even when dissipative rates appear converged. To restore causal consistency, we introduce a counter-term compensation scheme that restores the missing dispersive contributions without modifying the retained non-Markovian memory kernel. To validate the scheme and demonstrate the practicality of the proposed framework, we present numerical examples ranging from benchmark configurations to a three-dimensional dispersive ring-resonator structure via finite element method. These capabilities provide a practical route for rigorously incorporating full-wave electromagnetic simulations into non-Markovian multi-emitter quantum electrodynamics, enabling predictive modeling of collective emission, coherent energy exchange, and single-photon radiation in realistic open structures.
In recent years, Born-Markov master equations based on tracing out the electromagnetic degrees of freedom have been extensively employed in the description of quantum optical phenomena originating from photon-mediated interactions in quantum emitter ensembles. The breakdown of these effective models, built upon assumptions such as ensemble spectral homogeneity, an unstructured photonic density of states, and weak light-matter coupling, has also recently attracted considerable attention. Here, we investigate the accuracy of this well-established framework beyond the most conventional, and extensively explored, spontaneous emission configuration. Specifically, we consider a system comprising two coherently driven and detuned quantum emitters, embedded within a hybrid photonic-plasmonic cavity, formed by a metallic nanorod integrated into a high-refractive-index dielectric microresonator. The local density of photonic states in this structure exhibits a complex frequency dependence, making it a compelling platform for exploring photon-mediated interactions beyond the assumptions above. We benchmark this modeling approach for the quantum dynamics of the emitter pair against exact calculations based on a macroscopic field quantization formalism, providing an illustrative assessment of its validity in significantly structured and dispersive photonic environments. Our analysis reveals four distinct regimes of laser driving and frequency splitting that lead to markedly different levels of accuracy in the effective model.