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arXiv:2510.09262 · Advanced Quantum Technologies

Entangled Photon Pair Generator Via Biexciton–Exciton Cascade in Semiconductor Quantum Dots and its Simulation

Simon Sekavčnik, Paul R. Kohl, Janis Nötzel

Published Apr 1, 2026• 3 citations
arXivHTMLPDF

Abstract

ABSTRACT The generation of entangled photon pairs is highly useful for many types of quantum technologies. In this work an entangled photon pair generator that utilizes the biexciton–exciton cascade in semiconductor quantum dots is described on a physical, mathematical, and software level. The system is implemented and simulated as a self‐contained component in a framework for bigger quantum optical experiments. Thus, it is a description to further the holistic understanding of the system for interdisciplinary audiences in a hopefully simple yet sufficient manner. It is described from the condensed matter physics fundamentals, over the most important quantum optical properties, to a mathematical description of the used model, and finally a software description and simulation, making it an executable description of such a system. We provide a compact description in the Kraus operator formalism to seamlessly incorporate such an entangled photon pair generator simulation component into bigger simulations consisting of multiple components at a reasonable computational cost. The simulation accommodates a wide range of parameter regimes and makes it possible to simulate many different excitation strategies. This includes resonant two‐photon excitation, adiabatic rapid passage chirped excitation, and dichromatic pulsed excitation.

DOI
10.1002/qute.202500786

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ABSTRACT The generation of entangled photon pairs is highly useful for many types of quantum technologies. In this work an entangled photon pair generator that utilizes the biexciton–exciton cascade in semiconductor quantum dots is described on a physical, mathematical, and software level. The system is implemented and simulated as a self‐contained component in a framework for bigger quantum optical experiments. Thus, it is a description to further the holistic understanding of the system for interdisciplinary audiences in a hopefully simple yet sufficient manner. It is described from the condensed matter physics fundamentals, over the most important quantum optical properties, to a mathematical description of the used model, and finally a software description and simulation, making it an executable description of such a system. We provide a compact description in the Kraus operator formalism to seamlessly incorporate such an entangled photon pair generator simulation component into bigger simulations consisting of multiple components at a reasonable computational cost. The simulation accommodates a wide range of parameter regimes and makes it possible to simulate many different excitation strategies. This includes resonant two‐photon excitation, adiabatic rapid passage chirped excitation, and dichromatic pulsed excitation.
Resonant excitation of the biexciton state in an InAsP quantum dot by a phase-coherent pair of picosecond pulses allows preparing time-bin entangled pairs of photons via the biexciton–exciton cascade. We show that this scheme can be implemented for a dot embedded in an InP nanowire. The underlying physical mechanisms can be represented and quantitatively analyzed by an effective three-level open system master equation. Simulation parameters including decay and intensity dependent dephasing rates are extracted from experimental data, which in turn let us predict the resulting entanglement and optimal operating conditions.
A scheme for creating biexcitons without undesirable excitons is demonstrated in GaAs quantum dots (QDs) using an optical pumping method. This scheme utilizes resonant two-photon excitation processes for biexcitons with carefully set excitation conditions. In this scheme, biexcitons are directly created from the ground state while suppressing unnecessary exciton creation. Theoretical analysis confirms that our scheme works in actual QDs. Directly created biexcitons will make ideal entangled photons via cascade photoemission processes in a biexciton–exciton system with the reduction in the number of undesirable single photons from excitons that are not related to the cascade processes.
Semiconductor Quantum dots are potentially an attractive source of non-classical light. They can confine bound electron-hole pairs, excitons, in all three spatial dimensions giving them discrete optical emission energies, much like the electronic states in atomic systems. The semiconductor nature of the system allows quantum dots to be integrated into complicated device structures including optical cavities [1] and electrical injection [2]. The radiative exciton emission from a semiconductor quantum dot can provide the simplest form of quantum light, a single photon source [2]. The finite re-excitation time following the radiative decay of an exciton in a quantum dot prevents the dot from emitting more than one photon if excited with a short optical or electronic pulse. In a similar fashion excitation of the biexciton state, consisting of two electrons and holes, in the quantum dot results in the emission of a pair of photons at the energy of the biexciton and exciton transitions. The biexciton state was, in fact, proposed as a possible source of polarisation-entangled photons in 2000 by Benson et al. [3] as it consists of two polarisation-correlated decay paths which could potentially be indistinguishable. The condition of indistinguishability is fundamental to the generation of entangled photons and is, in general, not true of the two decay paths from the biexciton state in a quantum dot; physical anisotropy causes the intermediate exciton states to hybridise and separate in energy providing ‘which-path’ information about the route taken through the biexciton decay. We demonstrate how the splitting between the intermediate exciton states in a single InAs quantum dot can be controlled by growth [4], rapid thermal annealing [5] and the application of an external magnetic field [6]. Each of these three techniques can be used to make the intermediate exciton states degenerate allowing the biexciton decay to produce singe pairs of entangled photons triggered by short laser pulses [7,8]. Entangled photon pair sources are essential for applications such as entanglement based quantum key distribution, and optical quantum computing. For these applications it is important that no more than one entangled photon pair is generated in a cycle, a requirement met by our quantum dot source which is not possible with traditional methods for generating entangled pairs of photons. Entanglement also enables quantum interferometry and metrology, the basis of image resolution beyond that possible with equivalent classical light. Biphoton interferometry using entangled emission from the biexciton decay reveals fringes with half the period of classical light [9], and less that that of the laser. In addition, interferometry suggests that this type of entangled light source is not limited by decoherence, we fine the biphoton is surprising robust against dephasing, in stark contrast to the devastating effect of decoherence upon single photons emitted by similar structures.
For scalable applications of optical quantum information it is desirable to have a well controlled source of photons, producing single photons or entangled-pairs on-demand. The finite delay following decay of an exciton confined in a quantum dot makes them a good source of single photons, we demonstrate this, triggering the emission with a pulsed laser. Currently the most widely used techniques for generating entangled photon pairs are nonlinear optical processes, such as parametric down conversion, which produces a probabilistic number of pairs per excitation cycle. Such a source is of limited use in quantum information/processing applications where a regular stream of single entangled photon pairs is preferable. We produced such a triggered source from a semiconductor device for the first time, using the two-photon cascade from a biexciton confined in a single quantum dot. We demonstrate a fidelity of 70% for the emission from the biexciton cascade to the expected bell state. Single quantum dots could prove to be the first robust and compact triggered source of entangled photons.
Semiconductor quantum dots (QDs) have emerged as a premier solid-state platform for the deterministic generation of nonclassical light, offering a compelling pathway toward scalable quantum photonic systems. While single-photon emission from QDs has reached a high level of maturity, the realization of high-fidelity entangled photon-pair sources remains an active and rapidly evolving frontier. In this review, we survey the recent progress in QD-based entangled photon sources, highlighting the conceptual evolution from the established biexciton-exciton cascade to the emerging paradigm of spontaneous two-photon emission. We further examine how advances in nanophotonic architectures and coherent control strategies are redefining fundamental performance limits, enabling concurrent improvements in source brightness, coherence, and entanglement fidelity. Finally, we discuss the key physical and technological challenges that must be addressed to bridge the gap between laboratory demonstrations and large-scale deployment. We conclude by outlining the future opportunities for integrating QD-based entangled photon sources into practical quantum communication, computation, and sensing platforms.
Semiconductor quantum dots (QDs) have emerged as a premier solid-state platform for the deterministic generation of nonclassical light, offering a compelling pathway toward scalable quantum photonic systems. While single-photon emission from QDs has reached a high level of maturity, the realization of high-fidelity entangled photon-pair sources remains an active and rapidly evolving frontier. In this review, we survey the recent progress in QD-based entangled photon sources, highlighting the conceptual evolution from the established biexciton–exciton cascade to the emerging paradigm of spontaneous two-photon emission. We further examine how advances in nanophotonic architectures and coherent control strategies are redefining fundamental performance limits, enabling concurrent improvements in source brightness, coherence, and entanglement fidelity. Finally, we discuss the key physical and technological challenges that must be addressed to bridge the gap between laboratory demonstrations and large-scale deployment. We conclude by outlining the future opportunities for integrating QD-based entangled photon sources into practical quantum communication, computation, and sensing platforms.