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arXiv:2510.09164

High-Fidelity Single-Shot Readout and Selective Nuclear Spin Control for a Spin-1/2 Quantum Register in Diamond

Prithvi Gundlapalli, Philipp J. Vetter, Genko T. Genov, Michael Olney‐Fraser, Peng Wang, Matthias M. Müller, Katharina Senkalla, Fedor Jelezko

Published Oct 10, 2025• 0 citations
arXivHTMLPDF

Abstract

Quantum networks offer a way to overcome the size and complexity limitations of single quantum devices by linking multiple nodes into a scalable architecture. Group-IV color centers in diamond, paired with long-lived nuclear spins, have emerged as promising building blocks demonstrating proof-of-concept experiments such as blind quantum computing and quantum-enhanced sensing. However, realizing a large-scale electro-nuclear register remains a major challenge. Here we establish the germanium-vacancy (GeV) center as a viable platform for such network nodes. Using correlation spectroscopy, we identify single nuclear spins within a convoluted spin environment, overcoming limitations imposed by the color center's spin-$1/2$ nature and thereby enabling indirect control of these nuclear spins. We further demonstrate high-fidelity single-shot readout of both the GeV center ($95.8\,\%$) and a neighboring ${}^{13}\text{C}$ nuclear spin ($93.7\,\%$), a key tool for feed-forward error correction. These critical advances position the GeV center as a compelling candidate for next-generation quantum network nodes.

DOI
10.48550/arxiv.2510.09164

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Quantum networks offer a way to overcome the size and complexity limitations of single quantum devices by linking multiple nodes into a scalable architecture. Group-IV color centers in diamond, paired with long-lived nuclear spins, have emerged as promising building blocks demonstrating proof-of-concept experiments such as blind quantum computing and quantum-enhanced sensing. However, realizing a large-scale electro-nuclear register remains a major challenge. Here we establish the germanium-vacancy (GeV) center as a viable platform for such network nodes. Using correlation spectroscopy, we identify single nuclear spins within a convoluted spin environment, overcoming limitations imposed by the color center's spin-1/21/21/2 nature and thereby enabling indirect control of these nuclear spins. We further demonstrate high-fidelity single-shot readout of both the GeV center (95.8 %95.8\,\%95.8%) and a neighboring 13C{}^{13}\text{C}13C nuclear spin (93.7 %93.7\,\%93.7%), a key tool for feed-forward error correction. These critical advances position the GeV center as a compelling candidate for next-generation quantum network nodes.
Abstract Solid-state spin defects, such as color centers in diamond, are among the most promising candidates for scalable and integrated quantum technologies. In particular, the good optical properties of silicon-vacancy centers in diamond, combined with naturally occurring and exceptionally coherent nuclear spins, serve as a building block for quantum networking applications. Here, we show that leveraging an ultra-high-strained silicon-vacancy center inside a nanodiamond allows us to coherently and efficiently control its electron spin, while mitigating phonon-induced dephasing at liquid helium temperature. Moreover, we indirectly control and characterize a 13C nuclear spin and establish a quantum register. We overcome limited nuclear spin initialization by implementing single-shot nuclear spin readout. Lastly, we demonstrate coherent optical control with GHz rates, thus opening a potential connection of the register to the optical domain. Our work paves the way for future integration of quantum network registers into conventional, well-established photonics and hybrid quantum communication systems.
Color centers associated with group-IV dopants in diamond with long-lived nuclear spins have emerged as major candidates for distributed quantum computing nodes and quantum repeaters. Several proof-of-principle experiments have already been demonstrated. A key operation for long-distance entanglement-distribution protocols are fast and robust gates between the electron spin and a nuclear spin. Here, we investigate numerically for an existing experimental platform of a Germanium-vacancy (GeV) center with a strongly-coupled 13{}^{13}13C spin, how such gates can be implemented via quantum optimal control. In the presence of realistic noise we investigate different parameter regimes and gate operations and obtain robust two-qubit gates with fidelities exceeding 99.9%99.9 \%99.9%. The framework provides a scalable strategy for group-IV quantum nodes and can be adapted to related architectures.
Solid-state spin defects, such as color centers in diamond, are among the most promising candidates for scalable and integrated quantum technologies. In particular, the good optical properties of silicon-vacancy centers in diamond combined with naturally occurring and exceptionally coherent nuclear spins serve as a building block for quantum networking applications. Here, we show that leveraging an ultra-high strained silicon-vacancy center inside a nanodiamond allows us to coherently and efficiently control its electron spin, while mitigating phonon-induced dephasing at liquid helium temperature. Moreover, we indirectly control and characterize a 13C nuclear spin and establish a quantum register. We overcome limited nuclear spin initialization by implementing single-shot nuclear spin readout. Lastly, we demonstrate coherent optical control with GHz rates, thus connecting the register to the optical domain. Our work paves the way for future integration of quantum network registers into conventional, well-established photonics and hybrid quantum communication systems.
Long distance quantum networking requires combining efficient spin-photon interfaces with long-lived local memories. Group-IV color centers in diamond (SiV, GeV, and SnV) are promising candidates for this application, containing an electronic spin-photon interface and dopant nuclear spin memory. Recent work has demonstrated state-of-the-art performance in spin-photon coupling and spin-spin entanglement. However, coupling between the electron and nuclear spins introduces a phase kickback during optical excitation that limits the utility of the nuclear memory. Here, we propose using the large hyperfine coupling of SnV-117 to operate the device at zero magnetic field in a regime where the memory is insensitive to optical excitation. We further demonstrate ground state spin control of a SnV-117 color center integrated in a photonic integrated circuit, showing 97.8% gate fidelity and 2.5 ms coherence time for the memory spin level. This shows the viability of the zero-field protocol for high fidelity operation, and lays the groundwork for building quantum network nodes with SnV-117 devices.
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The germanium vacancy in diamond (GeV) is a promising candidate for color center based quantum networking. Yet, like for other group-IV vacancy defects in diamond, achieving fast, high-fidelity qubit operations using traditional magnetic resonance techniques is experimentally challenging due to a weak magnetic dipole and susceptibility to thermally induced decoherence. Here, we perform all-optical control of the GeV and realize Rabi frequencies exceeding ∼ 20 MHz. We do so by driving the two Λ -systems of the GeV simultaneously and apply this to probe the spin coherence ( T 2 * = 224 ± 14 ns, T 2 H = 11.9 ± 0.3 µ s ). Our control scheme is applicable to other color centers and particularly, other group-IV defects for which the scheme may be optimized to improve all-optical control in these systems.