We introduce a quantity called the free mutual information (FMI), adapted from concepts in free probability theory, as a new physical measure of quantum chaos. This quantity captures the spreading of a time-evolved operator in the space of all possible operators on the Hilbert space, which is doubly exponential in the number of degrees of freedom. It thus provides a finer notion of operator spreading than the well-understood phenomenon of operator growth in physical space. We derive two central results which apply in any physical system: first, an explicit “Coulomb gas” formula for the FMI of two observables A ( t ) and B in terms of the eigenvalues of the product operator A ( t ) B ; and second, a general relation expressing the FMI as a weighted sum of all higher-point out-of-time-ordered correlators (OTOCs). This second result provides a precise information-theoretic interpretation for the higher-point OTOCs as collectively quantifying operator ergodicity and the approach to freeness. This physical interpretation is particularly useful in light of recent progress in experimentally measuring higher-point OTOCs. We identify universal behaviors of the FMI and higher-point OTOCs across a variety of chaotic systems, including random unitary circuits and chaotic spin chains, which indicate that spreading in the doubly exponential operator space is a generic feature of quantum many-body chaos. At the same time, the non-generic behavior of the FMI in various non-chaotic systems, including certain unitary designs, shows that there are cases where an operator spreads in physical space but remains localized in operator space. The FMI is thus a sharper diagnostic of chaos than the standard four-point OTOC.
We introduce a quantity called the free mutual information (FMI), adapted from concepts in free probability theory, as a new physical measure of quantum chaos. This quantity captures the spreading of a time-evolved operator in the space of all possible operators on the Hilbert space, which is doubly exponential in the number of degrees of freedom. It thus provides a finer notion of operator spreading than the well-understood phenomenon of operator growth in physical space. We derive two central results which apply in any physical system: first, an explicit “Coulomb gas” formula for the FMI of two observables A ( t ) and B in terms of the eigenvalues of the product operator A ( t ) B ; and second, a general relation expressing the FMI as a weighted sum of all higher-point out-of-time-ordered correlators (OTOCs). This second result provides a precise information-theoretic interpretation for the higher-point OTOCs as collectively quantifying operator ergodicity and the approach to freeness. This physical interpretation is particularly useful in light of recent progress in experimentally measuring higher-point OTOCs. We identify universal behaviors of the FMI and higher-point OTOCs across a variety of chaotic systems, including random unitary circuits and chaotic spin chains, which indicate that spreading in the doubly exponential operator space is a generic feature of quantum many-body chaos. At the same time, the non-generic behavior of the FMI in various non-chaotic systems, including certain unitary designs, shows that there are cases where an operator spreads in physical space but remains localized in operator space. The FMI is thus a sharper diagnostic of chaos than the standard four-point OTOC.
Operator spreading under unitary time evolution has attracted a lot of attention recently as a way to probe many-body quantum chaos. While quantities such as out-of-time-ordered correlators (OTOCs) do distinguish interacting from noninteracting systems, it has remained unclear to what extent they can truly diagnose chaotic vs integrable dynamics in many-body quantum systems. Here, we analyze operator spreading in generic one-dimensional many-body quantum systems using a combination of matrix product operator (MPO) and analytical techniques, focusing on the operator right weight. First, we show that while small bond dimension MPOs allow one to capture the exponentially decaying tail of the operator front, in agreement with earlier results, they lead to significant quantitative and qualitative errors for the actual front---defined by the maximum of the right weight. We find that while the operator front broadens diffusively in both integrable and chaotic interacting spin chains, the precise shape and scaling of the height of the front in integrable systems is anomalous for all accessible times. We interpret these results using a quasiparticle picture. This provides a sharp, although rather subtle, signature of many-body quantum chaos in the operator front.
Unitary randomness underpins both fundamental tasks in quantum information and the modern theory of quantum chaos. On one side, a central concept is that of approximate unitary designs: circuits that look random according to small moments and for forward-in-time protocols. In a distinct setting, out-of-time-ordered correlators (OTOCs), intensely studied as a measure of information scrambling, have recently been shown to probe freeness between Heisenberg operators, the noncommutative generalization of statistical independence. Bridging these two concepts, we study the emergence of freeness in a random matrix product unitary ensemble. We prove that, with only polynomial bond dimension, these unitaries reproduce Haar values of higher-order OTOCs for local, finite-trace observables, while traceless observables instead require exponential resources. Indeed, local observables are precisely those predicted to thermalize in chaotic many-body systems according to the eigenstate thermalization hypothesis. Moreover, adding to previous literature, we show how random matrix product unitaries constitute approximate designs: we exactly compute the frame potential of the ensemble, showing convergence to the Haar value with polynomial deviations and so indicating that global observables are freely independent on-average. Our results highlight the need to refine previous notions of unitary design in the context of operator dynamics, guiding us towards protocols for quantum advantage and shedding light on the emergent complexity of chaotic many-body systems.
Out-of-time-ordered correlators (OTOCs) measure the scrambling of information and are a powerful diagnostic of chaos. In chaotic quantum systems with a classical analog, their relaxation towards equilibrium is dictated by the classical Ruelle--Pollicott resonances. We investigate higher-order OTOCs in quantum maps, prototypical one-body systems with a classical limit showing all the essential features of chaotic dynamics. We demonstrate numerically that in the intermediate-time regime they decay exponentially at a rate that depends only on the parity of the order: odd-order OTOCs decay at the same rate as classical correlations, given by the leading Ruelle--Pollicott resonance, and even-order ones at twice that rate. Both are far slower than the naive expectation, under which the rate would grow in proportion to the order. We then mimic the effect of an environment by defining a coarse-grained superoperator whose effect is to introduce decoherence into the system, and find that the expected proportionality between rate and order is thereby restored. Finally, we show that at long times each higher-order OTOC becomes dominated by a single free cumulant, whose saturation value falls off inversely with the dimension of the Hilbert space, signalling the emergence of asymptotic freeness and highlighting the relevance of free probability theory as a framework for the study of quantum chaos.
Thermalization of chaotic quantum many-body systems under unitary time evolution is related to the growth in complexity of initially simple Heisenberg operators.Operator growth is a manifestation of information scrambling and can be diagnosed by out-of-time-order correlators (OTOCs).However, the behavior of OTOCs of local operators in generic chaotic local Hamiltonians remains poorly understood, with some semiclassical and large-N models exhibiting exponential growth of OTOCs and a sharp chaos wave front and other random circuit models showing a diffusively broadened wave front.In this paper, we propose a unified physical picture for scrambling in chaotic local Hamiltonians.We construct a random time-dependent Hamiltonian model featuring a large-N limit where the OTOC obeys a Fisher-Kolmogorov-Petrovsky-Piskunov (FKPP) type equation and exhibits exponential growth and a sharp wave front.We show that quantum fluctuations manifest as noise (distinct from the randomness of the couplings in the underlying Hamiltonian) in the FKPP equation and that the noise-averaged OTOC exhibits a crossover to a diffusively broadened wave front.At small N, we demonstrate that operator growth dynamics, averaged over the random couplings, can be efficiently simulated for all time using matrix product state techniques.To show that time-dependent randomness is not essential to our conclusions, we push our previous matrix product operator methods to very large size and show that data for a timeindependent Hamiltonian model are also consistent with a diffusively broadened wave front.
We investigate the integrability-to-chaos transition and information scrambling in Ising spin networks via a graph-theoretic formulation. Modeling spins as vertices and interactions as edges encoded by adjacency matrices across path, Erdos-Renyi, and Watts-Strogatz topologies, we demonstrate that long-range couplings and heterogeneous degree distributions markedly accelerate quantum information propagation. The Hamiltonian comprises local and normalized non-local interactions; tuning the non-local coupling and field heterogeneity drives integrability breaking. To quantify scrambling, we employ bipartite mutual and tripartite information. Increasing non-local interactions drives tripartite information to large negative values, signaling deep information scrambling. The squared commutators constructed from out-of-time-order correlators (OTOCs) exhibit early-time exponential growth; equivalently, the OTOC four-point functions themselves decay exponentially, yielding quantum Lyapunov exponents that scale systematically with parameters governing the chaotic regime. Complementing this, Krylov complexity reveals rapid operator growth in the chaotic phase, synchronizing with OTOC and mutual information dynamics. Spectrally, the transition manifests as a shift from Poissonian to Wigner-Dyson level spacing statistics. The spectral form factor (SFF) exhibits the characteristic slope-dip-ramp-plateau structure, enabling the extraction of Thouless and Heisenberg times. Crucially, a reduced Thouless time strongly correlates with accelerated information and operator scrambling. Ultimately, this work establishes a unified framework bridging network topology with information-theoretic, operator, and spectral diagnostics, offering insights into thermalization and non-equilibrium dynamics in quantum many-body systems.
We adopt a continuous weak measurement tomography protocol to explore the signatures of chaos in the quantum system(s). We generate the measurement record as a series of expectation values of an observable evolving under the desired dynamics, which can show a transition from integrability to chaos. We find that the rate of information gain depends on the degree of chaos in the dynamics, the choice of initial observable, and how well the operator is aligned along the density matrix. The amount of operator spreading in the Krylov subspace, as quantified by the fidelity in quantum tomography and various other metrics of information gain, increases with the degree of chaos in the system. We study operator spreading in many-body quantum systems by its potential to generate an informationally complete measurement record. Our quantifiers for operator spreading are more consistent indicators of quantum chaos than Krylov complexity. Our study gives an operational interpretation for operator spreading in terms of fidelity gain in quantum tomography. Continuing in our journey of finding the footprints of chaos in the quantum domain, we explore the growth of errors in noisy tomography. For random states, when the measurement record is obtained from a random operator, the subsequent drop in the fidelity obtained is inversely correlated to the degree of chaos in the dynamics. This gives us an operational interpretation of Loschmidt echo for operators by connecting it to the performance of quantum tomography. We find a quantity to capture the scrambling of errors, an out-of-time-ordered correlator (OTOC) between two operators under perturbed and unperturbed dynamics that serves as a signature of chaos. Our results demonstrate a fundamental link between Loschmidt echo and scrambling of errors, as captured by OTOCs, with operational consequences in quantum information processing.