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arXiv:2509.11585 · Physical Review Research

Strong photon antibunching and photon pair emission in a two-atom cavity QED system with van der Waals interaction

Z. Y. Yu, J. P. Xu, C. J. Zhu, Z. Y. Bai, Y. P. Yang

Published Oct 27, 2025• 1 citation
arXivHTMLPDF

Abstract

We investigate the generation of strong antibunching photons/photon pairs in a two-atom cavity QED system leveraging interatomic van der Waals (vdW) interaction. We show that the vdW interaction shifts the energy of double excited state, enabling the suppression of two-photon excitation via destructive interference in a diamond configuration. This leads to antibunching photon emission with extremely high purity. Furthermore, by tuning the vdW interaction strength, the conditions for conventional and unconventional photon blockades can be satisfied simultaneously, which significantly enhances the generation of single photon. Conversely, at the antiblockade excitation frequency, quantum Monte Carlo simulations demonstrate the feasibility of generating antibunching photon pairs with a high purity and reasonable leaking rate by selecting appropriate driving field Rabi frequency and vdW interaction strength. These findings on enhanced photon antibunching and photon pair emission may lead to more efficient and brighter quantum light sources, which is a key mechanism for optical quantum devices.

DOI
10.1103/3v2q-7g6r

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We investigate the generation of strong antibunching photons/photon pairs in a two-atom cavity QED system leveraging interatomic van der Waals (vdW) interaction. We show that the vdW interaction shifts the energy of double excited state, enabling the suppression of two-photon excitation via destructive interference in a diamond configuration. This leads to antibunching photon emission with extremely high purity. Furthermore, by tuning the vdW interaction strength, the conditions for conventional and unconventional photon blockades can be satisfied simultaneously, which significantly enhances the generation of single photon. Conversely, at the antiblockade excitation frequency, quantum Monte Carlo simulations demonstrate the feasibility of generating antibunching photon pairs with a high purity and reasonable leaking rate by selecting appropriate driving field Rabi frequency and vdW interaction strength. These findings on enhanced photon antibunching and photon pair emission may lead to more efficient and brighter quantum light sources, which is a key mechanism for optical quantum devices.
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We theoretically study the quantum-interference-induced photon blockade and antiblockade phenomenon in an atom-cavity QED system, where the destructive [constructive] interference between two different transition pathways prohibits [enhances] two-photon excitation. To begin with, we study a single-atom--cavity QED system where the atom or cavity is driven by a coherent pump field. We show that the cavity-driven case will lead to the quantum-interference-induced photon blockade under a specific condition, but such an interference-induced photon blockade cannot be realized in the atom-driven case. This is an important consequence of the pathways possible for the two types of drives. Then, we investigate the two-atom case, and find that an additional transition pathway appears in the atom-driven case. We show that this additional transition pathway results in the quantum-interference-induced photon blockade only when the atomic resonant frequency is different from the cavity mode frequency otherwise antiblockade occurs. Moreover, in this case, the condition for realizing the interference-induced photon blockade is independent of the system's intrinsic parameters, which can be used to generate antibunched photons in both weak and strong coupling regimes.
The antibunching effect generated in a cavity containing first a single two-level atomic system and then two identical atoms is explored for off-resonant interactions, in strong- and weak-coupling regimes. The cavity is driven by coherent and squeezed sources. Using the second-order correlation function analytically derived in the weak-excitation regime, we show that squeezed light achieves and improves strong antibunching, leading to a photon blockade. This enhancement is due to a destructive quantum interference mechanism induced by the nonclassical light, creating a supplementary transition pathway. The best effect is obtained for equal frequency detunings in the strong-coupling regime. More interestingly, our investigation reveals that the two-atom-cavity system can further improve the antibunching effect compared to the single-atom cavity. It turns out that the additional couplings appearing in the cavity due to the implementation of the two atoms, combined with the squeezed light, could substantially enhance the photon-blockade effect.
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We theoretically investigate the quantum-interference-induced photon blockade effect in a single two-level atom-cavity quantum electrodynamics (QED) system with degenerate parametric amplification. The analytical calculations reveal the optimal parametric gain and phase parameters for achieving optimum unconventional photon blockade conditions. Under the optimal parameter regime, the numerical results of the second-order correlation function demonstrate strong photon antibunching consistent with the analytical results. Furthermore, the numerical results corroborate that coherently driving the atom leads to a stronger photon blockade than a coherently driven cavity with the optimal parameters. We numerically demonstrate that the UPB effect is compromised by a non-zero cavity-atom coupling in the cavity-driven configuration. However, stronger photon antibunching can be attained with a non-zero cavity-atom coupling in the atom-driven configuration. This work may be suitable for experimentally realising a strongly antibunched single-photon source for applications in quantum technology.
We investigate a hybrid photon blockade (HPB) scheme in a driven two-qubit cavity QED system arising from the combination of eigenenergy-level anharmonicity (ELA) and quantum destructive interference (QDI). By tuning the detuning of a single qubit and pumping field, we identify precise parametric regimes that fully integrate the advantages of high brightness in ELA-based conventional photon blockade and strong antibunching in QDI-based unconventional photon blockade. Interestingly, these regimes are accompanied by hyperradiance, indicating that inter-emitter correlations give rise to enhanced collective emission. The HPB mechanism exhibits parametric generality across varying coupling asymmetries and remains accessible via detuning control, offering a feasible route for generating high-quality single-photon source in diverse quantum platforms.