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arXiv:2509.06946 · Physical Review A

Mechanisms of anomalous three-body loss in a population-imbalanced three-component Fermi gas

Kajsa-My Tempest, Chris H. Greene

Published Dec 16, 2025• 0 citations
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Abstract

Achieving precise control of ultracold atomic gases requires a detailed understanding of atom loss mechanisms. Motivated by the anomalous three-body decay in a three-component Fermi gas reported in Ref. [1], this work investigates mechanisms that possibly contribute to the observed loss. The three-body Schrödinger equation is solved in the hyperspherical adiabatic representation with pairwise van der Waals interactions, and the $S$-matrix is obtained via the eigenchannel $R$-matrix method to compute recombination rate coefficients $K_3$ and two-body cross sections. At the magnetic field strength where the anomalous decay occurs, $K_3$ is unitary limited, exhibiting the threshold energy scaling $K_3(E)\propto E^{-1}$. Consequently, the thermally averaged $\langle K_3 \rangle$ acquires a temperature dependence. Because the experiment is performed in the degenerate regime, $\langle K_3 \rangle$ also explicitly depends on the per-spin densities through the per-spin Fermi energies $E_{F}^{(i)}\propto n_i^{2/3}$. As the gas is diluted and degeneracy is reduced, $\langle K_3 \rangle$ approaches the non-degenerate value and becomes a function of temperature only. Channel-resolved branching ratios and cross sections are folded into a Monte Carlo cascade simulation of secondary collisions and trap escape. The analysis indicates that typical three-body recombination events remove fewer than three atoms on average, and that the atom losses are primarily due to the ejection of secondary collision products, rather than the initial three-body recombination products. Therefore, a significant fraction of the released binding energy remains in the trapped ensemble as kinetic energy. Retained energy drives evaporative loss, offering a plausible, partial explanation for the anomalous decay.

DOI
10.1103/h2bq-msgx

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Achieving precise control of ultracold atomic gases requires a detailed understanding of atom loss mechanisms. Motivated by the anomalous three-body decay in a three-component Fermi gas reported in Ref. [1], this work investigates mechanisms that possibly contribute to the observed loss. The three-body Schrödinger equation is solved in the hyperspherical adiabatic representation with pairwise van der Waals interactions, and the SSS-matrix is obtained via the eigenchannel RRR-matrix method to compute recombination rate coefficients K3K_3K3​ and two-body cross sections. At the magnetic field strength where the anomalous decay occurs, K3K_3K3​ is unitary limited, exhibiting the threshold energy scaling K3(E)∝E−1K_3(E)\propto E^{-1}K3​(E)∝E−1. Consequently, the thermally averaged ⟨K3⟩\langle K_3 \rangle⟨K3​⟩ acquires a temperature dependence. Because the experiment is performed in the degenerate regime, ⟨K3⟩\langle K_3 \rangle⟨K3​⟩ also explicitly depends on the per-spin densities through the per-spin Fermi energies EF(i)∝ni2/3E_{F}^{(i)}\propto n_i^{2/3}EF(i)​∝ni2/3​. As the gas is diluted and degeneracy is reduced, ⟨K3⟩\langle K_3 \rangle⟨K3​⟩ approaches the non-degenerate value and becomes a function of temperature only. Channel-resolved branching ratios and cross sections are folded into a Monte Carlo cascade simulation of secondary collisions and trap escape. The analysis indicates that typical three-body recombination events remove fewer than three atoms on average, and that the atom losses are primarily due to the ejection of secondary collision products, rather than the initial three-body recombination products. Therefore, a significant fraction of the released binding energy remains in the trapped ensemble as kinetic energy. Retained energy drives evaporative loss, offering a plausible, partial explanation for the anomalous decay.
In several experiments with ultracold trapped atoms, a narrow loss feature has been observed near an atom-dimer resonance, at which there is an Efimov trimer at the atom-dimer threshold. The conventional interpretation of these loss features is that they are produced by the avalanche mechanism, in which the energetic atom and dimer from three-body recombination undergo secondary elastic collisions that produce additional atoms with sufficient energy to escape from the trapping potential. We use Monte Carlo methods to calculate the average number of atoms lost and the average heat generated by recombination events in a Bose-Einstein condensate and in a thermal gas. We improve on previous models by taking into account the energy dependence of the cross sections, the spatial structure of the atom cloud, and the elastic scattering of the atoms. We show that the avalanche mechanism cannot produce a narrow loss feature near the atom-dimer resonance. The number of atoms lost from a recombination event can be more than twice as large as the three that would be obtained in the absence of secondary collisions. However, the resulting loss feature is broad and its peak is at a scattering length that is larger than the atom-dimer resonance and depends on the trap depth.
This thesis reports on experimental studies of few-body physics in ultracold Fermi gases. The main part is devoted to the first realisation of an ultracold three-component Fermi gas in thermal equilibrium that consists of atoms in the three lowest spin states of 6Li. In first experiments the collisional stability of the gas was investigated in dependence of the interparticle interaction. The interaction strength was tuned by an external magnetic field employing Feshbach resonances in all three two-body scattering channels. At two magnetic field values a resonant enhancement of three-body loss was observed that can be explained by an Efimov-like trimer consisting of one atom in each of the three states which crosses the continuum twice in the studied magnetic field region. The behaviour of three-body loss rates could be understood by taking into account a variation of the lifetime of the trimer with the magnetic field. These experiments were performed with large ensembles of atoms. A finite deeply degenerate Fermi gas consisting of a controlled number of atoms may serve as a clean model for finite Fermi systems as for example atomic nuclei. An approach for the preparation of such a gas is discussed and first experimental steps are presented.
Fermionic systems with multiple internal states, such as quarks in quantum chromodynamics and nucleons in nuclear matter, are at the heart of some of the most complex quantum many-body problems. The stability of such many-body multi-component systems is crucial to understanding, for instance, baryon formation and the nuclear structure, but these problems are typically challenging to tackle theoretically. Versatile experimental platforms on which to study analogous problems are thus sought-after. Here, we create a uniform three-component Fermi gas with controllable polarization, and observe anomalous decay of the polarized gas, in which the loss rates of each component unexpectedly differ, contradicting generic assumptions of three-body losses in this system. We introduce a generalized three-body rate equation which captures the decay dynamics, but the underlying microscopic mechanism is unknown. Three-component Fermi gases represent a versatile platform for quantum simulation, including quantum chromodynamics-like physics, pairing and few-body effects. Here the authors demonstrate control of spin imbalances and an unexpected asymmetric decay due to different three-body losses for each component, and whose microscopic mechanism remains to be understood.
Three-body recombination of identical, spin-polarized fermionic atoms in the ultracold limit is investigated using model interactions. The mechanisms for recombination are parametrized by the "scattering volume" V(p) and described in the framework of the adiabatic hyperspherical representation. We have calculated the recombination rate K3 as a function of V(p) and have found K3 proportional, variant |V(p)|(8/3) for small |V(p)|. Recombination near a two-body Feshbach resonance can thus be significant.
The aim of this thesis was to measure the three-body contact in the unitary Fermi gas for the first time. The three-body contact is a physical observable that quantifies the three-body short-range correlations. Our probe, sensitive to three fermions with spins ↑↑↓ or ↓↓↑ at short distances, is three-body loss from the optical trap, caused by recombination into a deeply bound molecule and a free atom. In our system, the two spins signify two different hyperfine states of 6Li. We calibrate that recombination process by measuring three-body loss in the motional ground state of three fermions in an optical tweezer at unitarity. The numerically determined three-body contact C_3 (3) 3 of the three fermion system and the experimentally obtained loss rate allow us to extract Im[a_3], which quantifies the coupling to the deeply bound molecular state. Depending on the initial spin configuration ↑↑↓ or ↓↓↑, we find two different values, differing by almost a factor of two. This difference can only be explained by microscopic details of the interatomic coupling. In the many-body unitary Fermi gas, we use the coupling parameter Im[a_3] to extract the zero-temperature dimensionless three-body contact density ζ3\zeta_3ζ3​ from three-body loss measurements. We obtain a value of ζ3\zeta_3ζ3​ = 0.22(4) and observe that the loss rate scales with a characteristic three-body constant s = 1.77, which stems from an underlying SO(2,1) symmetry. We heat the gas and determine ζ3\zeta_3ζ3​ in the thermal regime, observing agreement with the theoretical prediction based on the virial expansion. The extracted value of ζ3\zeta_3ζ3​ > 0, which eludes theory, indicates three-body correlations. At the same time, the experimentally confirmed constant s proves the existence of irreducible three-body correlations that cannot be explained by two-body correlations alone.
Hybrid atom-ion experiments have recently entered the few-partial wave regime in which magnetically tunable Feshbach resonances dominate the three-body loss dynamics. This necessitates a treatment of three-body recombination that can incorporate the role of the resonant dimer channel. Here, we develop a two-step Lindemann-type model for resonant atom-atom-ion three-body recombination that combines multichannel quantum-defect theory for the long-range polarization potential with a universal quantum-capture treatment of the inelastic atom-dimer step. We show that within our model, rate competition can lead to a peak in the three-body-recombination cross section of higher partial-wave channels at energies well below their corresponding centrifugal barrier. Investigating the resulting loss rates under numerically obtained non-thermal collision-energy distributions, we find that these effects survive the energy averaging and can be observed in state-of-the-art hybrid experimental setups. Our findings pave the way for a detailed characterization of atom-ion Feshbach resonances via the analysis of inelastic three-body-recombination processes.